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Title: Ultrafast x-ray-induced nuclear dynamics in diatomic molecules using femtosecond x-ray-pump–x-ray-probe spectroscopy

Authors:
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Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1272654
Grant/Contract Number:  
AC02-06CH11357; FG02-86ER13491; SC0012376; AC02-76SF00515
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Physical Review A
Additional Journal Information:
Journal Name: Physical Review A Journal Volume: 94 Journal Issue: 1; Journal ID: ISSN 2469-9926
Publisher:
American Physical Society
Country of Publication:
United States
Language:
English

Citation Formats

Lehmann, C. S., Picón, A., Bostedt, C., Rudenko, A., Marinelli, A., Moonshiram, D., Osipov, T., Rolles, D., Berrah, N., Bomme, C., Bucher, M., Doumy, G., Erk, B., Ferguson, K. R., Gorkhover, T., Ho, P. J., Kanter, E. P., Krässig, B., Krzywinski, J., Lutman, A. A., March, A. M., Ray, D., Young, L., Pratt, S. T., and Southworth, S. H. Ultrafast x-ray-induced nuclear dynamics in diatomic molecules using femtosecond x-ray-pump–x-ray-probe spectroscopy. United States: N. p., 2016. Web. doi:10.1103/PhysRevA.94.013426.
Lehmann, C. S., Picón, A., Bostedt, C., Rudenko, A., Marinelli, A., Moonshiram, D., Osipov, T., Rolles, D., Berrah, N., Bomme, C., Bucher, M., Doumy, G., Erk, B., Ferguson, K. R., Gorkhover, T., Ho, P. J., Kanter, E. P., Krässig, B., Krzywinski, J., Lutman, A. A., March, A. M., Ray, D., Young, L., Pratt, S. T., & Southworth, S. H. Ultrafast x-ray-induced nuclear dynamics in diatomic molecules using femtosecond x-ray-pump–x-ray-probe spectroscopy. United States. doi:10.1103/PhysRevA.94.013426.
Lehmann, C. S., Picón, A., Bostedt, C., Rudenko, A., Marinelli, A., Moonshiram, D., Osipov, T., Rolles, D., Berrah, N., Bomme, C., Bucher, M., Doumy, G., Erk, B., Ferguson, K. R., Gorkhover, T., Ho, P. J., Kanter, E. P., Krässig, B., Krzywinski, J., Lutman, A. A., March, A. M., Ray, D., Young, L., Pratt, S. T., and Southworth, S. H. Tue . "Ultrafast x-ray-induced nuclear dynamics in diatomic molecules using femtosecond x-ray-pump–x-ray-probe spectroscopy". United States. doi:10.1103/PhysRevA.94.013426.
@article{osti_1272654,
title = {Ultrafast x-ray-induced nuclear dynamics in diatomic molecules using femtosecond x-ray-pump–x-ray-probe spectroscopy},
author = {Lehmann, C. S. and Picón, A. and Bostedt, C. and Rudenko, A. and Marinelli, A. and Moonshiram, D. and Osipov, T. and Rolles, D. and Berrah, N. and Bomme, C. and Bucher, M. and Doumy, G. and Erk, B. and Ferguson, K. R. and Gorkhover, T. and Ho, P. J. and Kanter, E. P. and Krässig, B. and Krzywinski, J. and Lutman, A. A. and March, A. M. and Ray, D. and Young, L. and Pratt, S. T. and Southworth, S. H.},
abstractNote = {},
doi = {10.1103/PhysRevA.94.013426},
journal = {Physical Review A},
number = 1,
volume = 94,
place = {United States},
year = {2016},
month = {7}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: 10.1103/PhysRevA.94.013426

Citation Metrics:
Cited by: 7 works
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Works referenced in this record:

Observation of Time-Domain Modulation of Free-Electron-Laser Pulses by Multipeaked Electron-Energy Spectrum
journal, September 2013


Symmetry-dependent vibrational excitation in N 1s photoionization of N2: Experiment and theory
journal, March 2006

  • Ehara, M.; Nakatsuji, H.; Matsumoto, M.
  • The Journal of Chemical Physics, Vol. 124, Issue 12
  • DOI: 10.1063/1.2181144

Two-colour hard X-ray free-electron laser with wide tunability
journal, December 2013

  • Hara, Toru; Inubushi, Yuichi; Katayama, Tetsuo
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3919

Doppler-free kinetic energy release spectrum of
journal, April 1996

  • Lundqvist, M.; Edvardsson, D.; Baltzer, P.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 29, Issue 8
  • DOI: 10.1088/0953-4075/29/8/013

Two-colour pump–probe experiments with a twin-pulse-seed extreme ultraviolet free-electron laser
journal, September 2013

  • Allaria, E.; Bencivenga, F.; Borghes, R.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3476

Ultrafast Extreme Ultraviolet Induced Isomerization of Acetylene Cations
journal, December 2010


Tracing nuclear-wave-packet dynamics in singly and doubly charged states of N 2 and O 2 with XUV-pump–XUV-probe experiments
journal, July 2012


Time-resolved Coulomb-explosion imaging of nuclear wave-packet dynamics induced in diatomic molecules by intense few-cycle laser pulses
journal, January 2011


Ultrafast isomerization initiated by X-ray core ionization
journal, September 2015

  • Liekhus-Schmaltz, Chelsea E.; Tenney, Ian; Osipov, Timur
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms9199

Time-Resolved Imaging and Manipulation of H 2 Fragmentation in Intense Laser Fields
journal, August 2005


Investigating two-photon double ionization of D 2 by XUV-pump–XUV-probe experiments
journal, May 2010


Exploring few-photon, few-electron reactions at FLASH: from ion yield and momentum measurements to time-resolved and kinematically complete experiments
journal, September 2010

  • Rudenko, A.; Jiang, Y. H.; Kurka, M.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 43, Issue 19
  • DOI: 10.1088/0953-4075/43/19/194004

Imaging charge transfer in iodomethane upon x-ray photoabsorption
journal, July 2014


Catching Conical Intersections in the Act: Monitoring Transient Electronic Coherences by Attosecond Stimulated X-Ray Raman Signals
journal, November 2015


Attosecond Electron Dynamics
journal, May 2008


Soft X-ray-Driven Femtosecond Molecular Dynamics
journal, September 2007


Transient lattice contraction in the solid-to-plasma transition
journal, January 2016

  • Ferguson, Ken R.; Bucher, Maximilian; Gorkhover, Tais
  • Science Advances, Vol. 2, Issue 1
  • DOI: 10.1126/sciadv.1500837

Electron localization following attosecond molecular photoionization
journal, June 2010

  • Sansone, G.; Kelkensberg, F.; Pérez-Torres, J. F.
  • Nature, Vol. 465, Issue 7299
  • DOI: 10.1038/nature09084

Oscillatory behavior of charge transfer cross sections as a function of the charge of projectiles in low-energy collisions
journal, March 1980

  • Ryufuku, Hiroshi; Sasaki, Ken; Watanabe, Tsutomu
  • Physical Review A, Vol. 21, Issue 3
  • DOI: 10.1103/PhysRevA.21.745

Auger decay of 1 σ g and 1 σ u hole states of the N 2 molecule: Disentangling decay routes from coincidence measurements
journal, April 2010


Potential for biomolecular imaging with femtosecond X-ray pulses
journal, August 2000

  • Neutze, Richard; Wouts, Remco; van der Spoel, David
  • Nature, Vol. 406, Issue 6797
  • DOI: 10.1038/35021099

Synchronized pulses generated at 20 eV and 90 eV for attosecond pump–probe experiments
journal, May 2015


Hetero-site-specific X-ray pump-probe spectroscopy for femtosecond intramolecular dynamics
journal, May 2016

  • Picón, A.; Lehmann, C. S.; Bostedt, C.
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms11652

Determination of the K—LL Auger Spectra of N 2 , O 2 , CO, NO, H 2 O, and CO 2
journal, September 1971

  • Moddeman, W. E.; Carlson, Thomas A.; Krause, Manfred O.
  • The Journal of Chemical Physics, Vol. 55, Issue 5
  • DOI: 10.1063/1.1676411

Radiation damage in protein serial femtosecond crystallography using an x-ray free-electron laser
journal, December 2011


On the interpretation of molecular valence Auger spectra
journal, August 1981

  • Ågren, Hans
  • The Journal of Chemical Physics, Vol. 75, Issue 3
  • DOI: 10.1063/1.442176

Chirped Seeded Free-Electron Lasers: Self-Standing Light Sources for Two-Color Pump-Probe Experiments
journal, February 2013


Electron Rearrangement Dynamics in Dissociating I 2 n + Molecules Accessed by Extreme Ultraviolet Pump-Probe Experiments
journal, August 2014


Auger-electron ion coincidence studies of soft-x-ray induced fragmentation of N 2
journal, January 1987


Kinetic energies of fragment ions from N 2 absorbing soft X-rays by a photoion-photoion coincidence technique
journal, December 1987


K-shell photoionization of CO and N 2 : is there a link between the photoelectron angular distribution and the molecular decay dynamics?
journal, September 2001

  • Weber, Th; Jagutzki, O.; Hattass, M.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 34, Issue 18
  • DOI: 10.1088/0953-4075/34/18/305

The influence of the σ resonance on the Auger decay of core-ionized molecular nitrogen
journal, April 2008


Molecular Dissociative Ionization and Wave-Packet Dynamics Studied Using Two-Color XUV and IR Pump-Probe Spectroscopy
journal, September 2009


Evidence for interatomic Coulombic decay in Xe K -shell-vacancy decay of XeF 2
journal, September 2012


Ultrafast dynamics in acetylene clocked in a femtosecond XUV stopwatch
journal, August 2013

  • Jiang, Y. H.; Senftleben, A.; Kurka, M.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 46, Issue 16
  • DOI: 10.1088/0953-4075/46/16/164027

Indications of radiation damage in ferredoxin microcrystals using high-intensity X-FEL beams
journal, February 2015

  • Nass, Karol; Foucar, Lutz; Barends, Thomas R. M.
  • Journal of Synchrotron Radiation, Vol. 22, Issue 2
  • DOI: 10.1107/S1600577515002349

Experimental Demonstration of Femtosecond Two-Color X-Ray Free-Electron Lasers
journal, March 2013


Observing the Creation of Electronic Feshbach Resonances in Soft X-ray-Induced O2 Dissociation
journal, November 2008


The Atomic, Molecular and Optical Science instrument at the Linac Coherent Light Source
journal, April 2015

  • Ferguson, Ken R.; Bucher, Maximilian; Bozek, John D.
  • Journal of Synchrotron Radiation, Vol. 22, Issue 3
  • DOI: 10.1107/S1600577515004646

Tracking nuclear wave-packet dynamics in molecular oxygen ions with few-cycle infrared laser pulses
journal, July 2010


Imaging molecular isomerization using molecular-frame photoelectron angular distributions
journal, September 2012

  • Rescigno, T. N.; Douguet, Nicolas; Orel, A. E.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 45, Issue 19
  • DOI: 10.1088/0953-4075/45/19/194001

Recoil-ion and electron momentum spectroscopy: reaction-microscopes
journal, August 2003


Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules
journal, January 2013


High-intensity double-pulse X-ray free-electron laser
journal, March 2015

  • Marinelli, A.; Ratner, D.; Lutman, A. A.
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms7369

Extreme-ultraviolet pump–probe studies of one-femtosecond-scale electron dynamics
journal, July 2011

  • Tzallas, P.; Skantzakis, E.; Nikolopoulos, L. A. A.
  • Nature Physics, Vol. 7, Issue 10
  • DOI: 10.1038/nphys2033

Selecting core-hole localization or delocalization in CS2 by photofragmentation dynamics
journal, January 2015

  • Guillemin, R.; Decleva, P.; Stener, M.
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms7166