Magnetic Precursor of the Pressure-Induced Superconductivity in Fe-Ladder Compounds
Abstract
We studied the pressure effects on the antiferromagentic orders in iron-based ladder compounds CsFe$$_2$$Se$$_3$$ and BaFe$$_2$$S$$_3$$ using single crytal neutron diffraction technique. With identical crystal structure and similar magnetic structures, the two compounds exhibit highly contrasting magnetic behaviors under moderate external pressures. In CsFe$$_2$$Se$$_3$$ the ladders are brought much closer to each other by pressure, but the stripe-type of magnetic order shows no observable change. Furthermore, the stripe order in BaFe$$_2$$S$$_3$$, undergoes a quantum phase transition where an abrupt increase of $$N\acute{e}el$$ temperature by more than 50$$\%$$ occurs at about 1 GPa, accompanied by a jump in ordered moment. Finally, with its spin structure unchanged, BaFe$$_2$$S$$_3$$ enters an enhanced magnetic phase that bears the characteristics of an orbital selective Mott phase, which is the true herald for superconductivity emerging at higher pressures.
- Authors:
-
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division
- Univ. of Tokyo (Japan). Inst. for Solid State Physics (ISSP)
- Univ. of Tokyo (Japan). Inst. for Solid State Physics
- Tohoku Univ., Sendai (Japan). Dept. of Physics
- Tohoku Univ., Sendai (Japan). Dept. of Physics; Univ. of Tokyo (Japan). Inst. for Solid State Physics
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). High Flux Isotope Reactor (HFIR)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1327614
- Alternate Identifier(s):
- OSTI ID: 1267549
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Letters
- Additional Journal Information:
- Journal Volume: 117; Journal Issue: 4; Journal ID: ISSN 0031-9007
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Chi, Songxue, Uwatoko, Yoshiya, Cao, Huibo, Hirata, Yasuyuki, Hashizume, Kazuki, Aoyama, Takuya, and Ohgushi, Kenya. Magnetic Precursor of the Pressure-Induced Superconductivity in Fe-Ladder Compounds. United States: N. p., 2016.
Web. doi:10.1103/PhysRevLett.117.047003.
Chi, Songxue, Uwatoko, Yoshiya, Cao, Huibo, Hirata, Yasuyuki, Hashizume, Kazuki, Aoyama, Takuya, & Ohgushi, Kenya. Magnetic Precursor of the Pressure-Induced Superconductivity in Fe-Ladder Compounds. United States. https://doi.org/10.1103/PhysRevLett.117.047003
Chi, Songxue, Uwatoko, Yoshiya, Cao, Huibo, Hirata, Yasuyuki, Hashizume, Kazuki, Aoyama, Takuya, and Ohgushi, Kenya. Thu .
"Magnetic Precursor of the Pressure-Induced Superconductivity in Fe-Ladder Compounds". United States. https://doi.org/10.1103/PhysRevLett.117.047003. https://www.osti.gov/servlets/purl/1327614.
@article{osti_1327614,
title = {Magnetic Precursor of the Pressure-Induced Superconductivity in Fe-Ladder Compounds},
author = {Chi, Songxue and Uwatoko, Yoshiya and Cao, Huibo and Hirata, Yasuyuki and Hashizume, Kazuki and Aoyama, Takuya and Ohgushi, Kenya},
abstractNote = {We studied the pressure effects on the antiferromagentic orders in iron-based ladder compounds CsFe$_2$Se$_3$ and BaFe$_2$S$_3$ using single crytal neutron diffraction technique. With identical crystal structure and similar magnetic structures, the two compounds exhibit highly contrasting magnetic behaviors under moderate external pressures. In CsFe$_2$Se$_3$ the ladders are brought much closer to each other by pressure, but the stripe-type of magnetic order shows no observable change. Furthermore, the stripe order in BaFe$_2$S$_3$, undergoes a quantum phase transition where an abrupt increase of $N\acute{e}el$ temperature by more than 50$\%$ occurs at about 1 GPa, accompanied by a jump in ordered moment. Finally, with its spin structure unchanged, BaFe$_2$S$_3$ enters an enhanced magnetic phase that bears the characteristics of an orbital selective Mott phase, which is the true herald for superconductivity emerging at higher pressures.},
doi = {10.1103/PhysRevLett.117.047003},
journal = {Physical Review Letters},
number = 4,
volume = 117,
place = {United States},
year = {Thu Jul 21 00:00:00 EDT 2016},
month = {Thu Jul 21 00:00:00 EDT 2016}
}
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Works referencing / citing this record:
Iron-Based Chalcogenide Spin Ladder BaFe2X3 (X = Se,S)
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