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Title: Dynamic compression of dense oxide (Gd 3Ga 5O 12) from 0.4 to 2.6 TPa: Universal Hugoniot of fluid metals

Materials at high pressures and temperatures are of great current interest for warm dense matter physics, planetary sciences, and inertial fusion energy research. Shock-compression equation-of-state data and optical reflectivities of the fluid dense oxide, Gd 3Ga 5O 12 (GGG), were measured at extremely high pressures up to 2.6 TPa (26 Mbar) generated by high-power laser irradiation and magnetically-driven hypervelocity impacts. Above 0.75 TPa, the GGG Hugoniot data approach/reach a universal linear line of fluid metals, and the optical reflectivity most likely reaches a constant value indicating that GGG undergoes a crossover from fluid semiconductor to poor metal with minimum metallic conductivity (MMC). These results suggest that most fluid compounds, e.g., strong planetary oxides, reach a common state on the universal Hugoniot of fluid metals (UHFM) with MMC at sufficiently extreme pressures and temperatures. Lastly, the systematic behaviors of warm dense fluid would be useful benchmarks for developing theoretical equation-of-state and transport models in the warm dense matter regime in determining computational predictions.
 [1] ;  [2] ;  [3] ;  [4] ;  [5] ;  [4] ;  [6] ;  [7] ;  [1] ;  [1] ;  [1] ;  [1]
  1. Osaka Univ., Osaka (Japan)
  2. Harvard Univ., Cambridge, MA (United States)
  3. Kumamoto Univ., Kumamoto (Japan)
  4. Uppsala Univ., Uppsala (Sweden)
  5. Uppsala Univ., Uppsala (Sweden); KTH Royal Institute of Technology, Stockholm (Sweden)
  6. Ehime Univ., Ehime (Japan)
  7. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Washington State Univ., Pullman, WA (United States)
Publication Date:
Grant/Contract Number:
Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 6; Journal ID: ISSN 2045-2322
Nature Publishing Group
Research Org:
Sandia National Lab. (SNL-CA), Livermore, CA (United States); Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org:
Country of Publication:
United States
giant planets; laser-produced plasmas; phase transitions and critical phenomena
OSTI Identifier: