In-situ luminescence monitoring of ion-induced damage evolution in SiO2 and Al2O3

Crespillo, Miguel L.; Graham, Joseph T.; Zhang, Yanwen; Weber, William J.

doi:10.1016/j.jlumin.2015.12.016

Title: In-situ luminescence monitoring of ion-induced damage evolution in SiO₂ and Al₂O₃

Abstract

Real-time, in-situ ionoluminescence measurements provide information of evolution of emission bands with ion fluence, and thereby establish a correlation between point defect kinetics and phase stability. Using fast light ions (2 MeV H and 3.5 He MeV) and medium mass-high energy ions (8 MeV O, E=0.5 MeV/amu), scintillation materials of a-SiO₂, crystalline quartz, and Al₂O₃ are comparatively investigated at room temperature with the aim of obtaining a further insight on the structural defects induced by ion irradiation and understand the role of electronic energy loss on the damage processes. For more energetic heavy ions, the electronic energy deposition pattern offers higher rates of excitation deeper into the material and allows to evaluate the competing mechanisms between the radiative and non-radiative de-excitation processes. Irradiations with 8 MeV O ions have been selected corresponding to the electronic stopping regime, where the electronic stopping power is dominant, and above the critical amorphization threshold for quartz. Lastly, the usefulness of IBIL and its specific capabilities as a sensitive tool to investigate the material characterization and evaluation of radiation effects are demonstrated.

Authors:

Crespillo, Miguel L. ^[1]; Graham, Joseph T. ^[1]; Zhang, Yanwen ^[2]; Weber, William J. ^[2]

Univ. of Tennessee, Knoxville, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Publication Date:: Thu Dec 17 00:00:00 EST 2015

Research Org.:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC)

OSTI Identifier:: 1265945

Alternate Identifier(s):: OSTI ID: 1396535

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Journal of Luminescence

Additional Journal Information:: Journal Volume: 172; Journal ID: ISSN 0022-2313

Publisher:: Elsevier

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; luminescence; radiation damage; silica; alumina; quartz; ion beam induced luminescence; ion-solid interaction; irradiation effects

Citation Formats


                    Crespillo, Miguel L., Graham, Joseph T., Zhang, Yanwen, and Weber, William J. In-situ luminescence monitoring of ion-induced damage evolution in SiO2 and Al2O3.  United States: N. p., 2015. 
Web.  doi:10.1016/j.jlumin.2015.12.016.

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                    Crespillo, Miguel L., Graham, Joseph T., Zhang, Yanwen, & Weber, William J. In-situ luminescence monitoring of ion-induced damage evolution in SiO2 and Al2O3.  United States.  https://doi.org/10.1016/j.jlumin.2015.12.016

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                    Crespillo, Miguel L., Graham, Joseph T., Zhang, Yanwen, and Weber, William J. Thu .  
"In-situ luminescence monitoring of ion-induced damage evolution in SiO2 and Al2O3".  United States.  https://doi.org/10.1016/j.jlumin.2015.12.016.  https://www.osti.gov/servlets/purl/1265945.

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@article{osti_1265945,

  title        = {In-situ luminescence monitoring of ion-induced damage evolution in SiO2 and Al2O3},

  author       = {Crespillo, Miguel L. and Graham, Joseph T. and Zhang, Yanwen and Weber, William J.},

  abstractNote = {Real-time, in-situ ionoluminescence measurements provide information of evolution of emission bands with ion fluence, and thereby establish a correlation between point defect kinetics and phase stability. Using fast light ions (2 MeV H and 3.5 He MeV) and medium mass-high energy ions (8 MeV O, E=0.5 MeV/amu), scintillation materials of a-SiO2, crystalline quartz, and Al2O3 are comparatively investigated at room temperature with the aim of obtaining a further insight on the structural defects induced by ion irradiation and understand the role of electronic energy loss on the damage processes. For more energetic heavy ions, the electronic energy deposition pattern offers higher rates of excitation deeper into the material and allows to evaluate the competing mechanisms between the radiative and non-radiative de-excitation processes. Irradiations with 8 MeV O ions have been selected corresponding to the electronic stopping regime, where the electronic stopping power is dominant, and above the critical amorphization threshold for quartz. Lastly, the usefulness of IBIL and its specific capabilities as a sensitive tool to investigate the material characterization and evaluation of radiation effects are demonstrated.},

  doi          = {10.1016/j.jlumin.2015.12.016},

  journal      = {Journal of Luminescence},

  number       = ,

  volume       = 172,

  place        = {United States},

  year         = {Thu Dec 17 00:00:00 EST 2015},

  month        = {Thu Dec 17 00:00:00 EST 2015}

}

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Title: In-situ luminescence monitoring of ion-induced damage evolution in SiO2 and Al2O3

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Citation Formats

Information obtainable from ion beam luminescence journal, August 2007

Variations on the use of ion beam luminescence journal, September 2012

The response of several luminescent materials to keV and MeV ions journal, April 2005

Luminescence characteristics and defect formation in silica glasses under H and He ion irradiation journal, August 2007

Luminescence in SiO2 induced by MeV energy proton irradiation journal, August 2004

Silica luminescence induced by fast light ions journal, April 2007

Ionoluminescence induced by swift heavy ions in silica and quartz: A comparative analysis journal, September 2012

Ionoluminescence as Sensor of Structural Disorder in Crystalline SiO$_{2}$: Determination of Amorphization Threshold by Swift Heavy Ions journal, December 2011

Ion beam excited luminescence of sapphire journal, February 1990

The characterisation of high-grade synthetic quartz, corundum and spinel using ionoluminescence (IL) journal, July 1997

Radioluminescence monitoring of radiation induced surface electrical degradation in aluminas journal, November 2013

Ion bombardment induced surface electrical degradation monitoring by means of luminescence in aluminas journal, October 2013

In situ luminescence qualification of radiation damage in aluminas: F-aggregation and Al colloids journal, October 2014

Ion beam induced luminescence analysis of painting pigments journal, January 2007

Ion beam induced luminescence of materials journal, May 2002

An Ideal System for Analysis and Interpretation of Ion Beam Induced Luminescence journal, January 2015

Radiation induced optical absorption and radioluminescence in electron irradiated SiO2 journal, October 1998

Fused Silica Final Optics for Inertial Fusion Energy: Radiation Studies and System-Level Analysis journal, June 2003

γ and fission‐reactor radiation effects on the visible‐range transparency of aluminum‐jacketed, all‐silica optical fibers journal, August 1996

Induced optical absorption in gamma, neutron and ultraviolet irradiated fused quartz and silica journal, May 1997

Color center formation in silica glass induced by high energy Fe and Xe ions journal, January 2010

Defects in oxide glasses journal, January 2005

Creation of Quasistable Lattice Defects by Electronic Excitation in Si O 2 journal, August 1983

Optical studies of self-trapped excitons in SiO 2 journal, September 1988

Swift heavy ion irradiation of InP: Thermal spike modeling of track formation journal, May 2006

Optical waveguides obtained by swift-ion irradiation on silica (a-SiO2) journal, October 2010

Thick optical waveguides in lithium niobate induced by swift heavy ions (~10 MeV/amu) at ultralow fluences journal, January 2009

Effect of defect accumulation on ion-beam damage morphology by electronic excitation in lithium niobate: A MonteCarlo approach journal, July 2010

Amorphization kinetics under swift heavy ion irradiation: A cumulative overlapping-track approach journal, February 2011

New ion beam materials laboratory for materials modification and irradiation effects research journal, November 2014

Track formation in SiO 2 quartz and the thermal-spike mechanism journal, May 1994

Ion tracks in quartz and vitreous silica journal, August 2004

SRIM – The stopping and range of ions in matter (2010) journal, June 2010

Defect production in ceramics journal, November 1997

Ionoluminescence of zircon: rare earth emissions and radiation damage journal, September 2004

Damage process and luminescent characteristics in silica glasses under ion irradiation journal, April 2009

Model of ion-induced luminescence based on energy deposition by secondary electrons journal, June 1994

The problem of dating quartz 1: Spectroscopic ionoluminescence of dose dependence journal, January 2011

Generation and excitation of point defects in silica by synchrotron radiation above the absorption edge journal, January 2010

Cathodoluminescence microcharacterization of point defects in α-quartz journal, August 2009

Excitons in crystalline and amorphous SiO2: formation, relaxation and conversion to Frenkel pairs journal, November 1994

Self-Trapped Excitons in Silicon Dioxide: Mechanism and Properties journal, October 2005

Excitons in SiO2: a review journal, October 1992

Characterization of exciton self-trapping in amorphous silica journal, July 2006

Vacuum ultraviolet excitation of the 2.7eV emission band in neutron irradiated silica journal, July 2009

A review of electron spin spectroscopy and its application to the study of paramagnetic defects in crystalline quartz journal, March 1984

An ab initio study of self-trapped excitons in α-quartz journal, April 2003

Optical properties of the F + center in crystalline Al 2 O 3 journal, December 1978

Radiation effects in pure and doped Al2O3 crystals journal, May 1998

Photoluminescence and thermoluminescence of titanium ions in sapphire crystals journal, October 2001

Chemistry, textures and physical properties of quartz — geological interpretation and technical application journal, August 2009

Optically active oxygen-deficiency-related centers in amorphous silicon dioxide journal, October 1998

Kinetics of color center formation in silica irradiated with swift heavy ions: Thresholding and formation efficiency journal, October 2012

Mechanical response to swift ion irradiation-induced nano-tracks in silica journal, June 2015

Tunneling states in neutron-irradiated quartz: Measurements of the ultrasonic attenuation and velocity change journal, September 1990

Ionic and electronic processes in quartz:Mechanisms of thermoluminescence and optically stimulated luminescence journal, November 2002

Electronic damage in quartz (c-SiO2) by MeV ion irradiations: Potentiality for optical waveguiding applications journal, February 2012

The radial distribution of dose around the path of a heavy ion in liquid water journal, January 1986

Hole mobility and transport in thin SiO 2 films journal, April 1975

Kinetics of amorphization induced by swift heavy ions in α-quartz journal, November 2012

Generation of amorphous surface layers in LiNbO3 by ion-beam irradiation: thresholding and boundary propagation journal, November 2005

Luminescence of sapphire and ruby induced by He and Ar ion irradiation journal, July 1996

Swift-uranium-ion-induced damage in sapphire journal, May 1995

The blue emission at 2.8 eV in strontium titanate: evidence for a radiative transition of self-trapped excitons from unbound states journal, April 2019

Structural and Optical Properties of α -Quartz Cluster with Oxygen-Deficiency Centers journal, January 2018

Title: In-situ luminescence monitoring of ion-induced damage evolution in SiO₂ and Al₂O₃

Information obtainable from ion beam luminescence
journal, August 2007

Variations on the use of ion beam luminescence
journal, September 2012

The response of several luminescent materials to keV and MeV ions
journal, April 2005

Luminescence characteristics and defect formation in silica glasses under H and He ion irradiation
journal, August 2007

Luminescence in SiO2 induced by MeV energy proton irradiation
journal, August 2004

Silica luminescence induced by fast light ions
journal, April 2007

Ionoluminescence induced by swift heavy ions in silica and quartz: A comparative analysis
journal, September 2012

Ionoluminescence as Sensor of Structural Disorder in Crystalline SiO$_{2}$: Determination of Amorphization Threshold by Swift Heavy Ions
journal, December 2011

Ion beam excited luminescence of sapphire
journal, February 1990

The characterisation of high-grade synthetic quartz, corundum and spinel using ionoluminescence (IL)
journal, July 1997

Radioluminescence monitoring of radiation induced surface electrical degradation in aluminas
journal, November 2013

Ion bombardment induced surface electrical degradation monitoring by means of luminescence in aluminas
journal, October 2013

In situ luminescence qualification of radiation damage in aluminas: F-aggregation and Al colloids
journal, October 2014

Ion beam induced luminescence analysis of painting pigments
journal, January 2007

Ion beam induced luminescence of materials
journal, May 2002

An Ideal System for Analysis and Interpretation of Ion Beam Induced Luminescence
journal, January 2015

Radiation induced optical absorption and radioluminescence in electron irradiated SiO2
journal, October 1998

Fused Silica Final Optics for Inertial Fusion Energy: Radiation Studies and System-Level Analysis
journal, June 2003

γ and fission‐reactor radiation effects on the visible‐range transparency of aluminum‐jacketed, all‐silica optical fibers
journal, August 1996

Induced optical absorption in gamma, neutron and ultraviolet irradiated fused quartz and silica
journal, May 1997

Color center formation in silica glass induced by high energy Fe and Xe ions
journal, January 2010

Defects in oxide glasses
journal, January 2005

Creation of Quasistable Lattice Defects by Electronic Excitation in Si $O_{2}$
journal, August 1983

Optical studies of self-trapped excitons in SiO ₂
journal, September 1988

Swift heavy ion irradiation of InP: Thermal spike modeling of track formation
journal, May 2006

Optical waveguides obtained by swift-ion irradiation on silica (a-SiO2)
journal, October 2010

Thick optical waveguides in lithium niobate induced by swift heavy ions (~10 MeV/amu) at ultralow fluences
journal, January 2009

Effect of defect accumulation on ion-beam damage morphology by electronic excitation in lithium niobate: A MonteCarlo approach
journal, July 2010

Amorphization kinetics under swift heavy ion irradiation: A cumulative overlapping-track approach
journal, February 2011

New ion beam materials laboratory for materials modification and irradiation effects research
journal, November 2014

Track formation in ${SiO}_{2}$ quartz and the thermal-spike mechanism
journal, May 1994

Ion tracks in quartz and vitreous silica
journal, August 2004

SRIM – The stopping and range of ions in matter (2010)
journal, June 2010

Defect production in ceramics
journal, November 1997

Ionoluminescence of zircon: rare earth emissions and radiation damage
journal, September 2004

Damage process and luminescent characteristics in silica glasses under ion irradiation
journal, April 2009

Model of ion-induced luminescence based on energy deposition by secondary electrons
journal, June 1994

The problem of dating quartz 1: Spectroscopic ionoluminescence of dose dependence
journal, January 2011

Generation and excitation of point defects in silica by synchrotron radiation above the absorption edge
journal, January 2010

Cathodoluminescence microcharacterization of point defects in α-quartz
journal, August 2009

Excitons in crystalline and amorphous SiO2: formation, relaxation and conversion to Frenkel pairs
journal, November 1994

Self-Trapped Excitons in Silicon Dioxide: Mechanism and Properties
journal, October 2005

Excitons in SiO2: a review
journal, October 1992

Characterization of exciton self-trapping in amorphous silica
journal, July 2006

Vacuum ultraviolet excitation of the 2.7eV emission band in neutron irradiated silica
journal, July 2009

A review of electron spin spectroscopy and its application to the study of paramagnetic defects in crystalline quartz
journal, March 1984

An ab initio study of self-trapped excitons in α-quartz
journal, April 2003

Optical properties of the $F^{+}$ center in crystalline ${Al}_{2}$ $O_{3}$
journal, December 1978

Radiation effects in pure and doped Al2O3 crystals
journal, May 1998

Photoluminescence and thermoluminescence of titanium ions in sapphire crystals
journal, October 2001

Chemistry, textures and physical properties of quartz — geological interpretation and technical application
journal, August 2009

Optically active oxygen-deficiency-related centers in amorphous silicon dioxide
journal, October 1998

Kinetics of color center formation in silica irradiated with swift heavy ions: Thresholding and formation efficiency
journal, October 2012

Mechanical response to swift ion irradiation-induced nano-tracks in silica
journal, June 2015

Tunneling states in neutron-irradiated quartz: Measurements of the ultrasonic attenuation and velocity change
journal, September 1990

Ionic and electronic processes in quartz:Mechanisms of thermoluminescence and optically stimulated luminescence
journal, November 2002

Electronic damage in quartz (c-SiO2) by MeV ion irradiations: Potentiality for optical waveguiding applications
journal, February 2012

The radial distribution of dose around the path of a heavy ion in liquid water
journal, January 1986

Hole mobility and transport in thin SiO ₂ films
journal, April 1975

Kinetics of amorphization induced by swift heavy ions in α-quartz
journal, November 2012

Generation of amorphous surface layers in LiNbO3 by ion-beam irradiation: thresholding and boundary propagation
journal, November 2005

Luminescence of sapphire and ruby induced by He and Ar ion irradiation
journal, July 1996

Swift-uranium-ion-induced damage in sapphire
journal, May 1995

The blue emission at 2.8 eV in strontium titanate: evidence for a radiative transition of self-trapped excitons from unbound states
journal, April 2019

Structural and Optical Properties of α -Quartz Cluster with Oxygen-Deficiency Centers
journal, January 2018