Flexible MXene/Carbon Nanotube Composite Paper with High Volumetric Capacitance
Abstract
Electrochemical capacitors attract attention because of their high power densities and long cycle lives. Moreover, with increasing demand for portable and wearable electronics, recent research has focused primarily on improving the energy density per unit of volume of electrochemical capacitors. But, the volumetric capacitances of carbon-based electrodes is limited at around 60 F cm -3 for commercial devices, and at best in the range of 300 F cm -3 for low-density porous carbons (<0.5–1 g cm -3 ). Although extremely high capacitances of 1000–1500 F cm -3 can be achieved for hydrated ruthenium oxide, RuO 2 , its high cost limits its wide-spread applications.
- Authors:
-
- Drexel Univ., Philadelphia, PA (United States)
- Drexel Univ., Philadelphia, PA (United States); Dalian Univ. of Technology (China)
- Drexel Univ., Philadelphia, PA (United States); East China Univ. of Science and Technology, Shanghai (China)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1265885
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 27; Journal Issue: 2; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Zhao, Meng-Qiang, Ren, Chang E., Ling, Zheng, Lukatskaya, Maria R., Zhang, Chuanfang, Van Aken, Katherine L., Barsoum, Michel W., and Gogotsi, Yury. Flexible MXene/Carbon Nanotube Composite Paper with High Volumetric Capacitance. United States: N. p., 2014.
Web. doi:10.1002/adma.201404140.
Zhao, Meng-Qiang, Ren, Chang E., Ling, Zheng, Lukatskaya, Maria R., Zhang, Chuanfang, Van Aken, Katherine L., Barsoum, Michel W., & Gogotsi, Yury. Flexible MXene/Carbon Nanotube Composite Paper with High Volumetric Capacitance. United States. https://doi.org/10.1002/adma.201404140
Zhao, Meng-Qiang, Ren, Chang E., Ling, Zheng, Lukatskaya, Maria R., Zhang, Chuanfang, Van Aken, Katherine L., Barsoum, Michel W., and Gogotsi, Yury. Tue .
"Flexible MXene/Carbon Nanotube Composite Paper with High Volumetric Capacitance". United States. https://doi.org/10.1002/adma.201404140. https://www.osti.gov/servlets/purl/1265885.
@article{osti_1265885,
title = {Flexible MXene/Carbon Nanotube Composite Paper with High Volumetric Capacitance},
author = {Zhao, Meng-Qiang and Ren, Chang E. and Ling, Zheng and Lukatskaya, Maria R. and Zhang, Chuanfang and Van Aken, Katherine L. and Barsoum, Michel W. and Gogotsi, Yury},
abstractNote = {Electrochemical capacitors attract attention because of their high power densities and long cycle lives. Moreover, with increasing demand for portable and wearable electronics, recent research has focused primarily on improving the energy density per unit of volume of electrochemical capacitors. But, the volumetric capacitances of carbon-based electrodes is limited at around 60 F cm -3 for commercial devices, and at best in the range of 300 F cm -3 for low-density porous carbons (<0.5–1 g cm -3 ). Although extremely high capacitances of 1000–1500 F cm -3 can be achieved for hydrated ruthenium oxide, RuO 2 , its high cost limits its wide-spread applications.},
doi = {10.1002/adma.201404140},
journal = {Advanced Materials},
number = 2,
volume = 27,
place = {United States},
year = {Tue Nov 18 00:00:00 EST 2014},
month = {Tue Nov 18 00:00:00 EST 2014}
}
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Carbon-intercalated Ti 3 C 2 T x MXene for high-performance electrochemical energy storage
journal, January 2018
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- Journal of Materials Chemistry A, Vol. 6, Issue 46
Integrating MXene nanosheets with cobalt-tipped carbon nanotubes for an efficient oxygen reduction reaction
journal, January 2019
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- Journal of Materials Chemistry A, Vol. 7, Issue 3
Interface engineering in the BNNS@Ti 3 C 2 intercalation structure for enhanced electrocatalytic hydrogen evolution
journal, January 2019
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Synthesis of (V 2/3 Sc 1/3 ) 2 AlC i-MAX phase and V 2−x C MXene scrolls
journal, January 2019
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- Nanoscale, Vol. 11, Issue 31
A facile method for synthesizing CuS decorated Ti 3 C 2 MXene with enhanced performance for asymmetric supercapacitors
journal, January 2019
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- Journal of Materials Chemistry A, Vol. 7, Issue 15
Pursuit of a high-capacity and long-life Mg-storage cathode by tailoring sandwich-structured MXene@carbon nanosphere composites
journal, January 2019
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- Journal of Materials Chemistry A, Vol. 7, Issue 28
Few-layered Ti 3 C 2 T x MXenes coupled with Fe 2 O 3 nanorod arrays grown on carbon cloth as anodes for flexible asymmetric supercapacitors
journal, January 2019
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Synthesis and Li-ion electrode properties of layered MAB phases Ni n+1 ZnB n ( n = 1, 2)
journal, January 2020
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Superionic liquids in conducting nanoslits: A variety of phase transitions and ensuing charging behavior
journal, November 2019
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Surface-agnostic highly stretchable and bendable conductive MXene multilayers
journal, March 2018
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High-Voltage Symmetric Supercapacitor Based on 2D Titanium Carbide (MXene, Ti 2 CT x )/Carbon Nanosphere Composites in a Neutral Aqueous Electrolyte
journal, January 2018
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A Highly Flexible Supercapacitor Based on MnO2/RGO Nanosheets and Bacterial Cellulose-Filled Gel Electrolyte
journal, October 2017
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- Materials, Vol. 10, Issue 11
Synthesis and Characterization of 2D Molybdenum Carbide (MXene)
journal, February 2016
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Layer-by-Layer Assembly of Cross-Functional Semi-transparent MXene-Carbon Nanotubes Composite Films for Next-Generation Electromagnetic Interference Shielding
journal, September 2018
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Engineering 3D Ion Transport Channels for Flexible MXene Films with Superior Capacitive Performance
journal, February 2019
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Chemically Crosslinked Hydrogel Film Leads to Integrated Flexible Supercapacitors with Superior Performance
journal, October 2015
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A Metal-Free Supercapacitor Electrode Material with a Record High Volumetric Capacitance over 800 F cm −3
journal, November 2015
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Ultrathin MXene-Micropattern-Based Field-Effect Transistor for Probing Neural Activity
journal, February 2016
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Photoluminescent Ti 3 C 2 MXene Quantum Dots for Multicolor Cellular Imaging
journal, February 2017
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Battery-Supercapacitor Hybrid Devices: Recent Progress and Future Prospects
journal, February 2017
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Ultrastrong and Highly Conductive MXene‐Based Films for High‐Performance Electromagnetic Interference Shielding
journal, November 2019
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Flexible All-Solid-State Supercapacitors with High Volumetric Capacitances Boosted by Solution Processable MXene and Electrochemically Exfoliated Graphene
journal, November 2016
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2D Metal Carbides and Nitrides (MXenes) as High-Performance Electrode Materials for Lithium-Based Batteries
journal, September 2018
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Antimonene Engineered Highly Deformable Freestanding Electrode with Extraordinarily Improved Energy Storage Performance
journal, October 2019
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Ultrathin Titanate Nanosheets/Graphene Films Derived from Confined Transformation for Excellent Na/K Ion Storage
journal, June 2018
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2D Titanium Carbide/Reduced Graphene Oxide Heterostructures for Supercapacitor Applications
journal, April 2018
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Porous Two-Dimensional Transition Metal Carbide (MXene) Flakes for High-Performance Li-Ion Storage
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Two-Step Oxidation of Mxene in the Synthesis of Layer-Stacked Anatase Titania with Enhanced Lithium-Storage Performance
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Fabrication of Cobaltosic Oxide Nanoparticle‐Doped 3 D MXene/Graphene Hybrid Porous Aerogels for All‐Solid‐State Supercapacitors
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Synthesis of Grain-like MoS 2 for High-Performance Sodium-Ion Batteries
journal, June 2018
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Recent Progress of MXene-Based Nanomaterials in Flexible Energy Storage and Electronic Devices
journal, December 2018
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Facile Solution Processing of Stable MXene Dispersions towards Conductive Composite Fibers
journal, July 2019
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MXene‐Based Nonlinear Optical Information Converter for All‐Optical Modulator and Switcher
journal, October 2018
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Ultrafast Fabrication of TiO 2 -Inlaid Multilayered Carbon for Supercapacitor
journal, October 2018
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Production of Two-Dimensional Nanomaterials via Liquid-Based Direct Exfoliation
journal, December 2015
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High-Performance Biscrolled MXene/Carbon Nanotube Yarn Supercapacitors
journal, August 2018
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Room‐Temperature Liquid Metal Confined in MXene Paper as a Flexible, Freestanding, and Binder‐Free Anode for Next‐Generation Lithium‐Ion Batteries
journal, October 2019
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Recent advances in MXene: Preparation, properties, and applications
journal, June 2015
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2D metal carbides and nitrides (MXenes) for energy storage
journal, January 2017
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Hierarchical porous carbons with layer-by-layer motif architectures from confined soft-template self-assembly in layered materials
journal, June 2017
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In situ atomistic insight into the growth mechanisms of single layer 2D transition metal carbides
journal, June 2018
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One-step Solution Processing of Ag, Au and Pd@MXene Hybrids for SERS
journal, August 2016
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H 2 O 2 assisted room temperature oxidation of Ti 2 C MXene for Li-ion battery anodes
journal, January 2016
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Recent progress in layered transition metal carbides and/or nitrides (MXenes) and their composites: synthesis and applications
journal, January 2017
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Highly conductive and flexible molybdenum oxide nanopaper for high volumetric supercapacitor electrode
journal, January 2017
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Titanium carbide sheet based high performance wire type solid state supercapacitors
journal, January 2017
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Latest advances in supercapacitors: from new electrode materials to novel device designs
journal, January 2017
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Sb 2 O 3 /MXene(Ti 3 C 2 T x ) hybrid anode materials with enhanced performance for sodium-ion batteries
journal, January 2017
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Freestanding CoSeO 3 ·H 2 O nanoribbon/carbon nanotube composite paper for 2.4 V high-voltage, flexible, solid-state supercapacitors
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A comparative study on the oxidation of two-dimensional Ti 3 C 2 MXene structures in different environments
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Thick and freestanding MXene/PANI pseudocapacitive electrodes with ultrahigh specific capacitance
journal, January 2018
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A flexible VOCs sensor based on a 3D Mxene framework with a high sensing performance
journal, January 2018
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Mo 2 B, an MBene member with high electrical and thermal conductivities, and satisfactory performances in lithium ion batteries
journal, January 2020
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A high-performance trace level acetone sensor using an indispensable V 4 C 3 T x MXene
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Fabrication of novel MXene (Ti 3 C 2 )/polyacrylamide nanocomposite hydrogels with enhanced mechanical and drug release properties
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Solution-processed single-wall carbon nanotube transistor arrays for wearable display backplanes
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Effects of biaxial strain and functional groups on SiC/ti 3 C 2 heterostructure: a first principle calculation
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Composites of TiO 2 Nanoparticles Deposited on Ti 3 C 2 MXene Nanosheets with Enhanced Electrochemical Performance
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Stretchable Supercapacitor with Adjustable Volumetric Capacitance Based on 3D Interdigital Electrodes
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Flexible MXene/Graphene Films for Ultrafast Supercapacitors with Outstanding Volumetric Capacitance
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Highly Conductive Transition Metal Carbide/Carbonitride(MXene)@polystyrene Nanocomposites Fabricated by Electrostatic Assembly for Highly Efficient Electromagnetic Interference Shielding
journal, October 2017
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High-Performance Ultrathin Flexible Solid-State Supercapacitors Based on Solution Processable Mo 1.33 C MXene and PEDOT:PSS
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Flexible Ti 3 C 2 T x @Al electrodes with Ultrahigh Areal Capacitance: In Situ Regulation of Interlayer Conductivity and Spacing
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Infiltrated Porous Polymer Sheets as Free-Standing Flexible Lithium-Sulfur Battery Electrodes
journal, May 2016
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Interwoven MXene Nanosheet/Carbon-Nanotube Composites as Li-S Cathode Hosts
journal, November 2016
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Electronic and Optical Properties of 2D Transition Metal Carbides and Nitrides (MXenes)
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Highly Stretchable and Self‐Healable MXene/Polyvinyl Alcohol Hydrogel Electrode for Wearable Capacitive Electronic Skin
journal, May 2019
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Functional MXene Materials: Progress of Their Applications
journal, August 2018
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Hierarchical Cobalt Borate/MXenes Hybrid with Extraordinary Electrocatalytic Performance in Oxygen Evolution Reaction
journal, October 2018
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A Flexible Si@C Electrode with Excellent Stability Employing an MXene as a Multifunctional Binder for Lithium‐Ion Batteries
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Niobium carbide/reduced graphene oxide hybrid porous aerogel as high capacity and long‐life anode material for Li‐ion batteries
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Self‐Standing Hybrid Film of SnO 2 Nanotubes and MXene as A High‐Performance Anode Material for Thin Film Lithium‐Ion Batteries
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Chemically Integrated Inorganic-Graphene Two-Dimensional Hybrid Materials for Flexible Energy Storage Devices
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Recent Advances in Layered Ti 3 C 2 T x MXene for Electrochemical Energy Storage
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Facile synthesis of MXene/MnO2 composite with high specific capacitance
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Highly conductive dodecaborate/MXene composites for high performance supercapacitors
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Vibrational properties of Ti 3 C 2 and Ti 3 C 2 T 2 (T = O, F, OH) monosheets by first-principles calculations: a comparative study
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Self-assembled Ti 3 C 2 T x MXene film with high gravimetric capacitance
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3D assembly of Ti 3 C 2 -MXene directed by water/oil interfaces
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In situ synthesis of CNTs@Ti 3 C 2 hybrid structures by microwave irradiation for high-performance anodes in lithium ion batteries
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Effect of glycine functionalization of 2D titanium carbide (MXene) on charge storage
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MXene-supported Co 3 O 4 quantum dots for superior lithium storage and oxygen evolution activities
journal, January 2019
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Flexible Ti 3 C 2 T x /PEDOT:PSS films with outstanding volumetric capacitance for asymmetric supercapacitors
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Sulfur nanodots as MoS 2 antiblocking agent for stable sodium ion battery anodes
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MXene and MXene-based composites: synthesis, properties and environment-related applications
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Improving the performance of a titanium carbide MXene in supercapacitors by partial oxidation treatment
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A general way to fabricate transition metal dichalcogenide/oxide-sandwiched MXene nanosheets as flexible film anodes for high-performance lithium storage
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Multivalent metal ion hybrid capacitors: a review with a focus on zinc-ion hybrid capacitors
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A wearable, self-adhesive, long-lastingly moist and healable epidermal sensor assembled from conductive MXene nanocomposites
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Peaked dielectric responses in Ti 3 C 2 MXene nanosheets enabled composites with efficient microwave absorption
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A perspective on two-dimensional materials for planar micro-supercapacitors
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Pseudocapacitive materials for electrochemical capacitors: from rational synthesis to capacitance optimization
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Fabrication of Flexible, Lightweight, Magnetic Mushroom Gills and Coral-Like MXene–Carbon Nanotube Nanocomposites for EMI Shielding Application
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Hierarchical Ni-Co Hydroxide Petals on Mechanically Robust Graphene Petal Foam for High-Energy Asymmetric Supercapacitors
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Waterproof, Ultrahigh Areal-Capacitance, Wearable Supercapacitor Fabrics
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Transparent, Flexible, and Conductive 2D Titanium Carbide (MXene) Films with High Volumetric Capacitance
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Facile Synthesis of Crumpled Nitrogen-Doped MXene Nanosheets as a New Sulfur Host for Lithium-Sulfur Batteries
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MXene Aerogel Scaffolds for High‐Rate Lithium Metal Anodes
journal, October 2018
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An Ultrafast Conducting Polymer@MXene Positive Electrode with High Volumetric Capacitance for Advanced Asymmetric Supercapacitors
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Ultrathin and Flexible CNTs/MXene/Cellulose Nanofibrils Composite Paper for Electromagnetic Interference Shielding
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Rational control of the interlayer space inside two-dimensional titanium carbides for highly efficient uranium removal and imprisonment
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2D molybdenum and vanadium nitrides synthesized by ammoniation of 2D transition metal carbides (MXenes)
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“All-in-Gel” design for supercapacitors towards solid-state energy devices with thermal and mechanical compliance
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Nitrogen and Sulfur Co-Doped 2D Titanium Carbides for Enhanced Electrochemical Performance
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Measurement and Analysis of Thermal Conductivity of Ti3C2Tx MXene Films
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Recent advances in flexible supercapacitors based on carbon nanotubes and graphene
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Bio-inspired high-performance solid-state supercapacitors with the electrolyte, separator, binder and electrodes entirely from kelp
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Two-dimensional MXene-reinforced robust surface superhydrophobicity with self-cleaning and photothermal-actuating binary effects
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2D Ti3C2Tx (MXene)-reinforced polyvinyl alcohol (PVA) nanofibers with enhanced mechanical and electrical properties
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Amine-Assisted Delamination of Nb 2 C MXene for Li-Ion Energy Storage Devices
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Bifunctional Hybrid Ni/Ni 2 P Nanoparticles Encapsulated by Graphitic Carbon Supported with N, S Modified 3D Carbon Framework for Highly Efficient Overall Water Splitting
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Emergent Pseudocapacitance of 2D Nanomaterials
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2 D MXene‐based Energy Storage Materials: Interfacial Structure Design and Functionalization
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Flexible 3D Porous MXene Foam for High‐Performance Lithium‐Ion Batteries
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Charge transfer induced polymerization of EDOT confined between 2D titanium carbide layers
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Conjugated systems of porphyrin–carbon nanoallotropes: a review
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Out-of-plane ion transport makes nitrogenated holey graphite a promising high-rate anode for both Li and Na ion batteries
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Carbon–metal compound composite electrodes for capacitive deionization: synthesis, development and applications
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Materials Design and System Construction for Conventional and New-Concept Supercapacitors
journal, February 2017
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Battery-Supercapacitor Hybrid Devices: Recent Progress and Future Prospects
journal, February 2017
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Paper-Based Electrodes for Flexible Energy Storage Devices
journal, May 2017
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Modified MXene/Holey Graphene Films for Advanced Supercapacitor Electrodes with Superior Energy Storage
journal, August 2018
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Kirigami Patterning of MXene/Bacterial Cellulose Composite Paper for All‐Solid‐State Stretchable Micro‐Supercapacitor Arrays
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Facile Solution Processing of Stable MXene Dispersions towards Conductive Composite Fibers
journal, July 2019
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Beyond Graphene Anode Materials for Emerging Metal Ion Batteries and Supercapacitors
journal, October 2018
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- Nano-Micro Letters, Vol. 10, Issue 4
Multidimensional materials and device architectures for future hybrid energy storage
journal, September 2016
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- Nature Communications, Vol. 7, Issue 1
A highly flexible and sensitive piezoresistive sensor based on MXene with greatly changed interlayer distances
journal, October 2017
- Ma, Yanan; Liu, Nishuang; Li, Luying
- Nature Communications, Vol. 8, Issue 1
One-step Solution Processing of Ag, Au and Pd@MXene Hybrids for SERS
journal, August 2016
- Satheeshkumar, Elumalai; Makaryan, Taron; Melikyan, Armen
- Scientific Reports, Vol. 6, Issue 1
Surface-agnostic highly stretchable and bendable conductive MXene multilayers
journal, March 2018
- An, Hyosung; Habib, Touseef; Shah, Smit
- Science Advances, Vol. 4, Issue 3
Preparation of Ti3C2Tx/NiZn Ferrite Hybrids with Improved Electromagnetic Properties
journal, February 2020
- Zhou, Xiaobing; Li, Youbing; Huang, Qing
- Materials, Vol. 13, Issue 4
Deformation and Failure of MXene Nanosheets
journal, March 2020
- Zeleniakiene, Daiva; Monastyreckis, Gediminas; Aniskevich, Andrey
- Materials, Vol. 13, Issue 5
Fabrication of Flexible, Lightweight, Magnetic Mushroom Gills and Coral-Like MXene–Carbon Nanotube Nanocomposites for EMI Shielding Application
journal, April 2019
- Raagulan, Kanthasamy; Braveenth, Ramanaskanda; Ro Lee, Lee
- Nanomaterials, Vol. 9, Issue 4