Effect of interfacial structures on spin dependent tunneling in epitaxial L10-FePt/MgO/FePt perpendicular magnetic tunnel junctions
Abstract
In this study, epitaxial FePt(001)/MgO/FePt magnetic tunnel junctions with L10-FePt electrodes showing perpendicular magnetic anisotropy were fabricated by molecular beam epitaxial growth. Tunnel magnetoresistance ratios of 21% and 53% were obtained at 300 K and 10 K, respectively. Our previous work, based on transmission electron microscopy, confirmed a semi-coherent interfacial structure with atomic steps (Kohn et al., APL 102, 062403 (2013)). Here, we show by x-ray photoemission spectroscopy and first-principles calculation that the bottom FePt/MgO interface is either Pt-terminated for regular growth or when an Fe layer is inserted at the interface, it is chemically bonded to O. Finally, both these structures have a dominant role in spin dependent tunneling across the MgO barrier resulting in a decrease of the tunneling magnetoresistance ratio compared with previous predictions.
- Authors:
-
- Chinese Academy of Sciences (CAS), Beijing (China). State Key Lab. of Magnetism. Beijing National Lab. for Condensed Matter Physics. Inst. of Physics
- Univ. of Oxford (United Kingdom). Clarendon Lab. Dept. of Physics
- Ben-Gurion Univ. of the Negev, Beer-Sheva (Israel). Dept. of Materials Engineering. Ilse Katz Inst. for Nanoscale Science and Technology
- Univ. of Florida, Gainesville, FL (United States). Dept. of Physics. Quantum Theory Project; Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences. Computer Science and Mathematics Division
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE
- Contributing Org.:
- Chinese Academy of Sciences (CAS), Beijing (China); Ben-Gurion Univ. of the Negev, Beer-Sheva (Israel)
- OSTI Identifier:
- 1265531
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Applied Physics
- Additional Journal Information:
- Journal Volume: 117; Journal Issue: 8; Journal ID: ISSN 0021-8979
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; interface structure; magnetic tunnel junctions; tunneling; epitaxy; electrodes
Citation Formats
Yang, G., Li, D. L., Wang, S. G., Ma, Q. L., Liang, S. H., Wei, H. X., Han, X. F., Hesjedal, T., Ward, R. C. C., Kohn, A., Elkayam, A., Tal, N., and Zhang, X. -G. Effect of interfacial structures on spin dependent tunneling in epitaxial L10-FePt/MgO/FePt perpendicular magnetic tunnel junctions. United States: N. p., 2015.
Web. doi:10.1063/1.4913265.
Yang, G., Li, D. L., Wang, S. G., Ma, Q. L., Liang, S. H., Wei, H. X., Han, X. F., Hesjedal, T., Ward, R. C. C., Kohn, A., Elkayam, A., Tal, N., & Zhang, X. -G. Effect of interfacial structures on spin dependent tunneling in epitaxial L10-FePt/MgO/FePt perpendicular magnetic tunnel junctions. United States. https://doi.org/10.1063/1.4913265
Yang, G., Li, D. L., Wang, S. G., Ma, Q. L., Liang, S. H., Wei, H. X., Han, X. F., Hesjedal, T., Ward, R. C. C., Kohn, A., Elkayam, A., Tal, N., and Zhang, X. -G. Tue .
"Effect of interfacial structures on spin dependent tunneling in epitaxial L10-FePt/MgO/FePt perpendicular magnetic tunnel junctions". United States. https://doi.org/10.1063/1.4913265. https://www.osti.gov/servlets/purl/1265531.
@article{osti_1265531,
title = {Effect of interfacial structures on spin dependent tunneling in epitaxial L10-FePt/MgO/FePt perpendicular magnetic tunnel junctions},
author = {Yang, G. and Li, D. L. and Wang, S. G. and Ma, Q. L. and Liang, S. H. and Wei, H. X. and Han, X. F. and Hesjedal, T. and Ward, R. C. C. and Kohn, A. and Elkayam, A. and Tal, N. and Zhang, X. -G.},
abstractNote = {In this study, epitaxial FePt(001)/MgO/FePt magnetic tunnel junctions with L10-FePt electrodes showing perpendicular magnetic anisotropy were fabricated by molecular beam epitaxial growth. Tunnel magnetoresistance ratios of 21% and 53% were obtained at 300 K and 10 K, respectively. Our previous work, based on transmission electron microscopy, confirmed a semi-coherent interfacial structure with atomic steps (Kohn et al., APL 102, 062403 (2013)). Here, we show by x-ray photoemission spectroscopy and first-principles calculation that the bottom FePt/MgO interface is either Pt-terminated for regular growth or when an Fe layer is inserted at the interface, it is chemically bonded to O. Finally, both these structures have a dominant role in spin dependent tunneling across the MgO barrier resulting in a decrease of the tunneling magnetoresistance ratio compared with previous predictions.},
doi = {10.1063/1.4913265},
journal = {Journal of Applied Physics},
number = 8,
volume = 117,
place = {United States},
year = {Tue Feb 24 00:00:00 EST 2015},
month = {Tue Feb 24 00:00:00 EST 2015}
}
Web of Science
Works referenced in this record:
Current-induced magnetization reversal in nanopillars with perpendicular anisotropy
journal, February 2006
- Mangin, S.; Ravelosona, D.; Katine, J. A.
- Nature Materials, Vol. 5, Issue 3
Inelastic electron tunneling spectrum from surface magnon and magnetic impurity scatterings in magnetic tunnel junctions
journal, October 2010
- Wei, H. -X.; Qin, Q. -H.; Ma, Q. -L.
- Physical Review B, Vol. 82, Issue 13
Spin-transfer-induced precessional magnetization reversal
journal, May 2004
- Kent, A. D.; Özyilmaz, B.; del Barco, E.
- Applied Physics Letters, Vol. 84, Issue 19
A perpendicular-anisotropy CoFeB–MgO magnetic tunnel junction
journal, July 2010
- Ikeda, S.; Miura, K.; Yamamoto, H.
- Nature Materials, Vol. 9, Issue 9
Special points for Brillouin-zone integrations
journal, June 1976
- Monkhorst, Hendrik J.; Pack, James D.
- Physical Review B, Vol. 13, Issue 12, p. 5188-5192
QUANTUM ESPRESSO: a modular and open-source software project for quantum simulations of materials
journal, September 2009
- Giannozzi, Paolo; Baroni, Stefano; Bonini, Nicola
- Journal of Physics: Condensed Matter, Vol. 21, Issue 39, Article No. 395502
Tunnel Magnetoresistance Over 100% in MgO-Based Magnetic Tunnel Junction Films With Perpendicular Magnetic L1$_{0}$-FePt Electrodes
journal, November 2008
- Yoshikawa, M.; Kitagawa, E.; Nagase, T.
- IEEE Transactions on Magnetics, Vol. 44, Issue 11
Analytical investigation of spin-transfer dynamics using a perpendicular-to-plane polarizer
journal, January 2005
- Lee, K. J.; Redon, O.; Dieny, B.
- Applied Physics Letters, Vol. 86, Issue 2
Evidence for magnon excitation contribution to the magnetoresistance behavior during thermal annealing in CoFeB/MgO/CoFeB magnetic tunnel junctions
journal, June 2011
- Ma, Q. L.; Wang, S. G.; Wei, H. X.
- Physical Review B, Vol. 83, Issue 22
Evidence for FeO formation at the Fe/MgO interface in epitaxial TMR structure by X-ray photoelectron spectroscopy
journal, March 2007
- Wang, S. G.; Han, G.; Yu, G. H.
- Journal of Magnetism and Magnetic Materials, Vol. 310, Issue 2
Surface energy anisotropy of FePt nanoparticles
journal, April 2005
- Hong, Suklyun; Yoo, M. H.
- Journal of Applied Physics, Vol. 97, Issue 8
Chemical structure of the interface between MgO films and Fe(001)
journal, January 2003
- Oh, H.; Lee, S. B.; Seo, Jikeun
- Applied Physics Letters, Vol. 82, Issue 3
Temperature dependence of giant tunnel magnetoresistance in epitaxial Fe/MgO/Fe magnetic tunnel junctions
journal, November 2008
- Wang, S. G.; Ward, R. C. C.; Du, G. X.
- Physical Review B, Vol. 78, Issue 18
Surface energies of stoichiometric FePt and CoPt alloys and their implications for nanoparticle morphologies
journal, December 2009
- Dannenberg, Antje; Gruner, Markus E.; Hucht, Alfred
- Physical Review B, Vol. 80, Issue 24
FePdB layer for perpendicular magnetic tunnel junctions
journal, November 2010
- Choi, Gyung-Min; Min, Byoung-Chul; Shin, Kyung-Ho
- Applied Physics Letters, Vol. 97, Issue 20
Magnetotransport and magnetic properties of molecular-beam epitaxy L10 FePt thin films
journal, May 2000
- Yu, J.; Ruediger, U.; Kent, A. D.
- Journal of Applied Physics, Vol. 87, Issue 9
Abrupt Transition from Ferromagnetic to Antiferromagnetic of Interfacial Exchange in Perpendicularly Magnetized -MnGa/FeCo Tuned by Fermi Level Position
journal, April 2014
- Ma, Q. L.; Mizukami, S.; Kubota, T.
- Physical Review Letters, Vol. 112, Issue 15
Interface Characterization of Epitaxial Fe/MgO/Fe Magnetic Tunnel Junctions
journal, February 2012
- Wang, S. G.; Ward, R. C. C.; Hesjedal, T.
- Journal of Nanoscience and Nanotechnology, Vol. 12, Issue 2
Geometrical and Compositional Structure at Metal-Oxide Interfaces: MgO on Fe(001)
journal, July 2001
- Meyerheim, H. L.; Popescu, R.; Kirschner, J.
- Physical Review Letters, Vol. 87, Issue 7
Soft self-consistent pseudopotentials in a generalized eigenvalue formalism
journal, April 1990
- Vanderbilt, David
- Physical Review B, Vol. 41, Issue 11, p. 7892-7895
Chemical-order-dependent magnetic anisotropy and exchange stiffness constant of FePt (001) epitaxial films
journal, July 2002
- Okamoto, S.; Kikuchi, N.; Kitakami, O.
- Physical Review B, Vol. 66, Issue 2
Interface reaction of NiO/NiFe and its influence on magnetic properties
journal, March 2001
- Yu, G. H.; Chai, C. L.; Zhu, F. W.
- Applied Physics Letters, Vol. 78, Issue 12
Tunneling magnetoresistance of magnetic tunnel junctions using perpendicular magnetization L10-CoPt electrodes
journal, April 2008
- Kim, Gukcheon; Sakuraba, Yuya; Oogane, Mikihiko
- Applied Physics Letters, Vol. 92, Issue 17
Structure of epitaxial L1 0 -FePt/MgO perpendicular magnetic tunnel junctions
journal, February 2013
- Kohn, Amit; Tal, Nadav; Elkayam, Ayala
- Applied Physics Letters, Vol. 102, Issue 6
Temperature dependence of resistance in epitaxial Fe/MgO/Fe magnetic tunnel junctions
journal, August 2009
- Ma, Q. L.; Wang, S. G.; Zhang, J.
- Applied Physics Letters, Vol. 95, Issue 5
Magnetic tunnel junctions with L10-ordered FePt alloy electrodes
journal, June 2004
- Moriyama, T.; Mitani, S.; Seki, T.
- Journal of Applied Physics, Vol. 95, Issue 11
Spin-dependent tunneling spectroscopy for interface characterization of epitaxial Fe/MgO/Fe magnetic tunnel junctions
journal, February 2010
- Du, G. X.; Wang, S. G.; Ma, Q. L.
- Physical Review B, Vol. 81, Issue 6
Theoretical Studies on Spin-Dependent Conductance in FePt/MgO/FePt(001) Magnetic Tunnel Junctions
journal, November 2008
- Taniguchi, Y.; Miura, Y.; Abe, K.
- IEEE Transactions on Magnetics, Vol. 44, Issue 11
Correlation hole of the spin-polarized electron gas, with exact small-wave-vector and high-density scaling
journal, December 1991
- Wang, Yue; Perdew, John P.
- Physical Review B, Vol. 44, Issue 24
Magnetoresistance effect in L 1 0 -MnGa/MgO/CoFeB perpendicular magnetic tunnel junctions with Co interlayer
journal, July 2012
- Ma, Q. L.; Kubota, T.; Mizukami, S.
- Applied Physics Letters, Vol. 101, Issue 3
Magnetic coupling between high magnetization perpendicular electrodes in an epitaxial magnetic tunnel junction
journal, November 2007
- de Person, P.; Warin, P.; Jamet, M.
- Physical Review B, Vol. 76, Issue 18
Enhanced interface perpendicular magnetic anisotropy in Ta|CoFeB|MgO using nitrogen doped Ta underlayers
journal, June 2013
- Sinha, Jaivardhan; Hayashi, Masamitsu; Kellock, Andrew J.
- Applied Physics Letters, Vol. 102, Issue 24
Works referencing / citing this record:
Influence of HfO 2 interlayers on magnetocrystalline anisotropy in Fe |MgO |Fe magnetic tunnel junction: First-principles investigation
journal, June 2019
- Chen, W. Z.; Zhang, J.; Yang, B. S.
- Journal of Applied Physics, Vol. 125, Issue 23
Tunnel magnetoresistance in ultrathin L1 0 MnGa/MgO perpendicular magnetic tunnel junctions
journal, May 2018
- Suzuki, K. Z.; Miura, Y.; Ranjbar, R.
- Journal of Physics D: Applied Physics, Vol. 51, Issue 23
[Co/Ni] multilayers with robust post-annealing performance for spintronics device applications
journal, October 2018
- Gupta, S.; Sbiaa, R.; Al Bahri, M.
- Journal of Physics D: Applied Physics, Vol. 51, Issue 46