Magnetic control of valley pseudospin in monolayer WSe2
Abstract
Local energy extrema of the bands in momentum space, or valleys, can endow electrons in solids with pseudo-spin in addition to real spin1-5. In transition metal dichalcogenides this valley pseudo-spin, like real spin, is associated with a magnetic moment1,6 which underlies the valley-dependent circular dichroism6 that allows optical generation of valley polarization7-9, intervalley quantum coherence10, and the valley Hall effect11. However, magnetic manipulation of valley pseudospin via this magnetic moment12-13, analogous to what is possible with real spin, has not been shown before. Here we report observation of the valley Zeeman splitting and magnetic tuning of polarization and coherence of the excitonic valley pseudospin, by performing polarization-resolved magneto-photoluminescence on monolayer WSe2. Our measurements reveal both the atomic orbital and lattice contributions to the valley orbital magnetic moment; demonstrate the deviation of the band edges in the valleys from an exact massive Dirac fermion model; and reveal a striking difference between the magnetic responses of neutral and charged valley excitons which is explained by renormalization of the excitonic spectrum due to strong exchange interactions.
- Authors:
-
- Univ. of Washington, Seattle, WA (United States)
- Univ. of Hong Kong, Hong Kong (China)
- Univ. of Texas-Dallas, Richardson, TX (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division; Univ. of Tennessee, Knoxville, TN (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1265429
- Grant/Contract Number:
- AC05-00OR22725; SC0008145; SC0002197; HKU705513P; HKU9/CRF/13G; AoE/P-04/08
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Physics
- Additional Journal Information:
- Journal Volume: 11; Journal Issue: 2; Journal ID: ISSN 1745-2473
- Publisher:
- Nature Publishing Group (NPG)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS
Citation Formats
Aivazian, G., Gong, Zhirui, Jones, Aaron M., Chu, Rui-Lin, Yan, J., Mandrus, D. G., Zhang, Chuanwei, Cobden, David, Yao, Wang, and Xu, X. Magnetic control of valley pseudospin in monolayer WSe2. United States: N. p., 2015.
Web. doi:10.1038/nphys3201.
Aivazian, G., Gong, Zhirui, Jones, Aaron M., Chu, Rui-Lin, Yan, J., Mandrus, D. G., Zhang, Chuanwei, Cobden, David, Yao, Wang, & Xu, X. Magnetic control of valley pseudospin in monolayer WSe2. United States. https://doi.org/10.1038/nphys3201
Aivazian, G., Gong, Zhirui, Jones, Aaron M., Chu, Rui-Lin, Yan, J., Mandrus, D. G., Zhang, Chuanwei, Cobden, David, Yao, Wang, and Xu, X. Mon .
"Magnetic control of valley pseudospin in monolayer WSe2". United States. https://doi.org/10.1038/nphys3201. https://www.osti.gov/servlets/purl/1265429.
@article{osti_1265429,
title = {Magnetic control of valley pseudospin in monolayer WSe2},
author = {Aivazian, G. and Gong, Zhirui and Jones, Aaron M. and Chu, Rui-Lin and Yan, J. and Mandrus, D. G. and Zhang, Chuanwei and Cobden, David and Yao, Wang and Xu, X.},
abstractNote = {Local energy extrema of the bands in momentum space, or valleys, can endow electrons in solids with pseudo-spin in addition to real spin1-5. In transition metal dichalcogenides this valley pseudo-spin, like real spin, is associated with a magnetic moment1,6 which underlies the valley-dependent circular dichroism6 that allows optical generation of valley polarization7-9, intervalley quantum coherence10, and the valley Hall effect11. However, magnetic manipulation of valley pseudospin via this magnetic moment12-13, analogous to what is possible with real spin, has not been shown before. Here we report observation of the valley Zeeman splitting and magnetic tuning of polarization and coherence of the excitonic valley pseudospin, by performing polarization-resolved magneto-photoluminescence on monolayer WSe2. Our measurements reveal both the atomic orbital and lattice contributions to the valley orbital magnetic moment; demonstrate the deviation of the band edges in the valleys from an exact massive Dirac fermion model; and reveal a striking difference between the magnetic responses of neutral and charged valley excitons which is explained by renormalization of the excitonic spectrum due to strong exchange interactions.},
doi = {10.1038/nphys3201},
journal = {Nature Physics},
number = 2,
volume = 11,
place = {United States},
year = {Mon Jan 26 00:00:00 EST 2015},
month = {Mon Jan 26 00:00:00 EST 2015}
}
Web of Science
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