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Title: Passive gamma analysis of the boiling-water-reactor assemblies

This research focused on the analysis of a set of stationary passive gamma measurements taken on the spent nuclear fuel assemblies from a boiling water reactor (BWR) using pulse height analysis data acquisition. The measurements were performed on 25 different BWR assemblies in 2014 at Sweden’s Central Interim Storage Facility for Spent Nuclear Fuel (Clab). This study was performed as part of the Next Generation of Safeguards Initiative–Spent Fuel project to research the application of nondestructive assay (NDA) to spent fuel assemblies. The NGSI–SF team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay (NDA) measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins, (3) estimate the plutonium mass, (4) estimate the decay heat, and (5) determine the reactivity of spent fuel assemblies. The final objective of this project is to quantify the capability of several integrated NDA instruments to meet the aforementioned goals using the combined signatures of neutrons, gamma rays, and heat. This report presents a selection of the measured data and summarizes an analysis of the results. Specifically, trends in themore » count rates measured for spectral lines from the following isotopes were analyzed as a function of the declared burnup and cooling time: 137Cs, 154Eu, 134Cs, and to a lesser extent, 106Ru and 144Ce. From these measured count rates, predictive algorithms were developed to enable the estimation of the burnup and cooling time. Furthermore, these algorithms were benchmarked on a set of assemblies not included in the standard assemblies set used by this research team.« less
Authors:
 [1] ;  [1] ;  [2] ;  [3] ;  [2] ;  [4] ;  [5] ;  [6] ;  [1] ;  [1] ;
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  3. Uppsala Univ. (Sweden)
  4. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  5. European Atomic Energy Community (EURATOM) (Luxemburg)
  6. Swedish Nuclear Fuel and Waste Management Company, Stockholm (Sweden)
Publication Date:
Report Number(s):
LA-UR-16-23293
Journal ID: ISSN 0168-9002
Grant/Contract Number:
AC52-06NA25396; AC05-00OR22725
Type:
Accepted Manuscript
Journal Name:
Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment
Additional Journal Information:
Journal Volume: 830; Journal Issue: C; Journal ID: ISSN 0168-9002
Publisher:
Elsevier
Research Org:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org:
USDOE National Nuclear Security Administration (NNSA)
Country of Publication:
United States
Language:
English
Subject:
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL PROTECTION; Spent fuel, Passive gamma, Initial enrichment, Burnup, Boiling-Water-Reactor, BWR Cooling time; passive gamma; initial enrichment; burnup; cooling time; spent fuel NDA; BWR
OSTI Identifier:
1261559
Alternate Identifier(s):
OSTI ID: 1260577