Balancing surface adsorption and diffusion of lithium-polysulfides on nonconductive oxides for lithium–sulfur battery design
Abstract
Lithium–sulfur batteries have attracted attention due to their six-fold specific energy compared with conventional lithium-ion batteries. Dissolution of lithium polysulfides, volume expansion of sulfur and uncontrollable deposition of lithium sulfide are three of the main challenges for this technology. State-of-the-art sulfur cathodes based on metal-oxide nanostructures can suppress the shuttle-effect and enable controlled lithium sulfide deposition. However, a clear mechanistic understanding and corresponding selection criteria for the oxides are still lacking. Herein, various nonconductive metal-oxide nanoparticle-decorated carbon flakes are synthesized via a facile biotemplating method. The cathodes based on magnesium oxide, cerium oxide and lanthanum oxide show enhanced cycling performance. Adsorption experiments and theoretical calculations reveal that polysulfide capture by the oxides is via monolayered chemisorption. Moreover, we show that better surface diffusion leads to higher deposition efficiency of sulfide species on electrodes. Lastly, oxide selection is proposed to balance optimization between sulfide-adsorption and diffusion on the oxides.
- Authors:
-
- Zhejiang Univ. of Technology, Hangzhou (China); Stanford Univ., Stanford, CA (United States)
- Zhejiang Univ. of Technology, Hangzhou (China)
- Stanford Univ., Stanford, CA (United States)
- Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1255528
- Grant/Contract Number:
- AC02-76SF00515
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 7; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE
Citation Formats
Tao, Xinyong, Wang, Jianguo, Liu, Chong, Wang, Haotian, Yao, Hongbin, Zheng, Guangyuan, Seh, Zhi Wei, Cai, Qiuxia, Li, Weiyang, Zhou, Guangmin, Zu, Chenxi, and Cui, Yi. Balancing surface adsorption and diffusion of lithium-polysulfides on nonconductive oxides for lithium–sulfur battery design. United States: N. p., 2016.
Web. doi:10.1038/ncomms11203.
Tao, Xinyong, Wang, Jianguo, Liu, Chong, Wang, Haotian, Yao, Hongbin, Zheng, Guangyuan, Seh, Zhi Wei, Cai, Qiuxia, Li, Weiyang, Zhou, Guangmin, Zu, Chenxi, & Cui, Yi. Balancing surface adsorption and diffusion of lithium-polysulfides on nonconductive oxides for lithium–sulfur battery design. United States. https://doi.org/10.1038/ncomms11203
Tao, Xinyong, Wang, Jianguo, Liu, Chong, Wang, Haotian, Yao, Hongbin, Zheng, Guangyuan, Seh, Zhi Wei, Cai, Qiuxia, Li, Weiyang, Zhou, Guangmin, Zu, Chenxi, and Cui, Yi. Tue .
"Balancing surface adsorption and diffusion of lithium-polysulfides on nonconductive oxides for lithium–sulfur battery design". United States. https://doi.org/10.1038/ncomms11203. https://www.osti.gov/servlets/purl/1255528.
@article{osti_1255528,
title = {Balancing surface adsorption and diffusion of lithium-polysulfides on nonconductive oxides for lithium–sulfur battery design},
author = {Tao, Xinyong and Wang, Jianguo and Liu, Chong and Wang, Haotian and Yao, Hongbin and Zheng, Guangyuan and Seh, Zhi Wei and Cai, Qiuxia and Li, Weiyang and Zhou, Guangmin and Zu, Chenxi and Cui, Yi},
abstractNote = {Lithium–sulfur batteries have attracted attention due to their six-fold specific energy compared with conventional lithium-ion batteries. Dissolution of lithium polysulfides, volume expansion of sulfur and uncontrollable deposition of lithium sulfide are three of the main challenges for this technology. State-of-the-art sulfur cathodes based on metal-oxide nanostructures can suppress the shuttle-effect and enable controlled lithium sulfide deposition. However, a clear mechanistic understanding and corresponding selection criteria for the oxides are still lacking. Herein, various nonconductive metal-oxide nanoparticle-decorated carbon flakes are synthesized via a facile biotemplating method. The cathodes based on magnesium oxide, cerium oxide and lanthanum oxide show enhanced cycling performance. Adsorption experiments and theoretical calculations reveal that polysulfide capture by the oxides is via monolayered chemisorption. Moreover, we show that better surface diffusion leads to higher deposition efficiency of sulfide species on electrodes. Lastly, oxide selection is proposed to balance optimization between sulfide-adsorption and diffusion on the oxides.},
doi = {10.1038/ncomms11203},
journal = {Nature Communications},
number = ,
volume = 7,
place = {United States},
year = {Tue Apr 05 00:00:00 EDT 2016},
month = {Tue Apr 05 00:00:00 EDT 2016}
}
Web of Science
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A Novel Strategy for the Selection of Polysulfide Adsorbents Toward High‐Performance Lithium‐Sulfur Batteries
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Enhanced Sulfur Transformation by Multifunctional FeS 2 /FeS/S Composites for High‐Volumetric Capacity Cathodes in Lithium–Sulfur Batteries
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Large-Area Preparation of Crack-Free Crystalline Microporous Conductive Membrane to Upgrade High Energy Lithium-Sulfur Batteries
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Enhanced Electrochemical Kinetics on Conductive Polar Mediators for Lithium-Sulfur Batteries
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A Supramolecular Capsule for Reversible Polysulfide Storage/Delivery in Lithium-Sulfur Batteries
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Electrocatalysis in Lithium Sulfur Batteries under Lean Electrolyte Conditions
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Core-Shell Structure and Interaction Mechanism of γ-MnO 2 Coated Sulfur for Improved Lithium-Sulfur Batteries
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Constructing Patch‐Ni‐Shelled Pt@Ni Nanoparticles within Confined Nanoreactors for Catalytic Oxidation of Insoluble Polysulfides in Li‐S Batteries
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Sulfur Hosts against the Shuttle Effect
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Synthesis of graphitic carbon nitride via direct polymerization using different precursors and its application in lithium–sulfur batteries
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One-pot synthesis of highly conductive nickel-rich phosphide/CNTs hybrid as a polar sulfur host for high-rate and long-cycle Li-S battery
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Revisiting the anchoring behavior in lithium-sulfur batteries: many-body effect on the suppression of shuttle effect
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Bio-templated fabrication of metal-free boron carbonitride tubes for visible light photocatalysis
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Rational design of yolk–shell silicon dioxide@hollow carbon spheres as advanced Li–S cathode hosts
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The adsorption effect of freestanding SiO x -decorated stabilized polyacrylonitrile interlayers in lithium–sulfur batteries
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Adsorption and diffusion of lithium polysulfides over blue phosphorene for Li–S batteries
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A long life sodium–selenium cathode by encapsulating selenium into N-doped interconnected carbon aerogels
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Accelerated polysulfide conversion on hierarchical porous vanadium–nitrogen–carbon for advanced lithium–sulfur batteries
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Constructing a 3D compact sulfur host based on carbon-nanotube threaded defective Prussian blue nanocrystals for high performance lithium–sulfur batteries
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Ni 3 S 2 anchored to N/S co-doped reduced graphene oxide with highly pleated structure as a sulfur host for lithium–sulfur batteries
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Promoting Redox Reduction of Lithium-Sulfur Battery by Tris(2-carboxyl)phosphine Shearing S-S Bond
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Lithium Bond Chemistry in Lithium-Sulfur Batteries
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Natural Okra Shells Derived Nitrogen‐Doped Porous Carbon to Regulate Polysulfides for High‐Performance Lithium–Sulfur Batteries
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Ionic conductivity promotion of polymer electrolyte with ionic liquid grafted oxides for all-solid-state lithium–sulfur batteries
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Revisiting the use of electrolyte additives in Li–S batteries: the role of porosity of sulfur host materials
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Spiderweb-Mimicking Anion-Exchanging Separators for Li-S Batteries
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Catalytic Interfaces‐Enriched Hybrid Hollow Spheres Sulfur Host for Advanced Li–S Batteries
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Simultaneous Suppression of the Dendrite Formation and Shuttle Effect in a Lithium-Sulfur Battery by Bilateral Solid Electrolyte Interface
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Hierarchical N-Rich Carbon Sponge with Excellent Cycling Performance for Lithium-Sulfur Battery at High Rates
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Honeycomb-Like Nitrogen-Doped Carbon 3D Nanoweb@Li 2 S Cathode Material for Use in Lithium Sulfur Batteries
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2 D Materials for Inhibiting the Shuttle Effect in Advanced Lithium–Sulfur Batteries
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High-performance Li–S battery cathode with catalyst-like carbon nanotube-MoP promoting polysulfide redox
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Sepiolite/CNT/S@PANI composite with stable network structure for high performance lithium sulfur batteries
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Mesoporous silica nanoplates facilitating fast Li + diffusion as effective polysulfide-trapping materials for lithium–sulfur batteries
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Catalytic Effects in Lithium-Sulfur Batteries: Promoted Sulfur Transformation and Reduced Shuttle Effect
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Boosting High‐Rate Li–S Batteries by an MOF‐Derived Catalytic Electrode with a Layer‐by‐Layer Structure
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An Aqueous Inorganic Polymer Binder for High Performance Lithium–Sulfur Batteries with Flame-Retardant Properties
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Foldable interpenetrated metal-organic frameworks/carbon nanotubes thin film for lithium–sulfur batteries
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Exceptional catalytic effects of black phosphorus quantum dots in shuttling-free lithium sulfur batteries
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Achieving three-dimensional lithium sulfide growth in lithium-sulfur batteries using high-donor-number anions
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Ether-compatible sulfurized polyacrylonitrile cathode with excellent performance enabled by fast kinetics via selenium doping
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Cathode porosity is a missing key parameter to optimize lithium-sulfur battery energy density
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High performance lithium-sulfur batteries for storing pulsed energy generated by triboelectric nanogenerators
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Sandwich-structured nanoparticles-grafted functionalized graphene based 3D nanocomposites for high-performance biosensors to detect ascorbic acid biomolecule
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A review of biomass materials for advanced lithium–sulfur batteries
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A Novel Approach to Eliminate the Effect of External Stress on Interdiffusivity Measurement
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Favorable Lithium Nucleation on Lithiophilic Framework Porphyrin for Dendrite-Free Lithium Metal Anodes
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