Energetic, spatial, and momentum character of the electronic structure at a buried interface: The two-dimensional electron gas between two metal oxides

Nemšák, S.; Conti, G.; Gray, A. X.; Palsson, G. K.; Conlon, C.; Eiteneer, D.; Keqi, A.; Rattanachata, A.; Saw, A. Y.; Bostwick, A.; Moreschini, L.; Rotenberg, E.; Strocov, V. N.; Kobayashi, M.; Schmitt, T.; Stolte, W.; Ueda, S.; Kobayashi, K.; Gloskovskii, A.; Drube, W.; Jackson, C. A.; Moetakef, P.; Janotti, A.; Bjaalie, L.; Himmetoglu, B.; Van de Walle, C. G.; Borek, S.; Minar, J.; Braun, J.; Ebert, H.; Plucinski, L.; Kortright, J. B.; Schneider, C. M.; Balents, L.; de Groot, F. M. F.; Stemmer, S.; Fadley, C. S.

doi:10.1103/PhysRevB.93.245103

Title: Energetic, spatial, and momentum character of the electronic structure at a buried interface: The two-dimensional electron gas between two metal oxides

Publication Date:: Wed Jun 01 00:00:00 EDT 2016

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1255319

Grant/Contract Number:: DEAC02-05CH11231; AC02-05CH11231; SC0014697

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Name: Physical Review B Journal Volume: 93 Journal Issue: 24; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Nemšák, S., Conti, G., Gray, A. X., Palsson, G. K., Conlon, C., Eiteneer, D., Keqi, A., Rattanachata, A., Saw, A. Y., Bostwick, A., Moreschini, L., Rotenberg, E., Strocov, V. N., Kobayashi, M., Schmitt, T., Stolte, W., Ueda, S., Kobayashi, K., Gloskovskii, A., Drube, W., Jackson, C. A., Moetakef, P., Janotti, A., Bjaalie, L., Himmetoglu, B., Van de Walle, C. G., Borek, S., Minar, J., Braun, J., Ebert, H., Plucinski, L., Kortright, J. B., Schneider, C. M., Balents, L., de Groot, F. M. F., Stemmer, S., and Fadley, C. S. Energetic, spatial, and momentum character of the electronic structure at a buried interface: The two-dimensional electron gas between two metal oxides.  United States: N. p., 2016. 
Web.  doi:10.1103/PhysRevB.93.245103.

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                    Nemšák, S., Conti, G., Gray, A. X., Palsson, G. K., Conlon, C., Eiteneer, D., Keqi, A., Rattanachata, A., Saw, A. Y., Bostwick, A., Moreschini, L., Rotenberg, E., Strocov, V. N., Kobayashi, M., Schmitt, T., Stolte, W., Ueda, S., Kobayashi, K., Gloskovskii, A., Drube, W., Jackson, C. A., Moetakef, P., Janotti, A., Bjaalie, L., Himmetoglu, B., Van de Walle, C. G., Borek, S., Minar, J., Braun, J., Ebert, H., Plucinski, L., Kortright, J. B., Schneider, C. M., Balents, L., de Groot, F. M. F., Stemmer, S., & Fadley, C. S. Energetic, spatial, and momentum character of the electronic structure at a buried interface: The two-dimensional electron gas between two metal oxides.  United States.  https://doi.org/10.1103/PhysRevB.93.245103

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                    Nemšák, S., Conti, G., Gray, A. X., Palsson, G. K., Conlon, C., Eiteneer, D., Keqi, A., Rattanachata, A., Saw, A. Y., Bostwick, A., Moreschini, L., Rotenberg, E., Strocov, V. N., Kobayashi, M., Schmitt, T., Stolte, W., Ueda, S., Kobayashi, K., Gloskovskii, A., Drube, W., Jackson, C. A., Moetakef, P., Janotti, A., Bjaalie, L., Himmetoglu, B., Van de Walle, C. G., Borek, S., Minar, J., Braun, J., Ebert, H., Plucinski, L., Kortright, J. B., Schneider, C. M., Balents, L., de Groot, F. M. F., Stemmer, S., and Fadley, C. S. Wed .  
"Energetic, spatial, and momentum character of the electronic structure at a buried interface: The two-dimensional electron gas between two metal oxides".  United States.  https://doi.org/10.1103/PhysRevB.93.245103.

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@article{osti_1255319,

  title        = {Energetic, spatial, and momentum character of the electronic structure at a buried interface: The two-dimensional electron gas between two metal oxides},

  author       = {Nemšák, S. and Conti, G. and Gray, A. X. and Palsson, G. K. and Conlon, C. and Eiteneer, D. and Keqi, A. and Rattanachata, A. and Saw, A. Y. and Bostwick, A. and Moreschini, L. and Rotenberg, E. and Strocov, V. N. and Kobayashi, M. and Schmitt, T. and Stolte, W. and Ueda, S. and Kobayashi, K. and Gloskovskii, A. and Drube, W. and Jackson, C. A. and Moetakef, P. and Janotti, A. and Bjaalie, L. and Himmetoglu, B. and Van de Walle, C. G. and Borek, S. and Minar, J. and Braun, J. and Ebert, H. and Plucinski, L. and Kortright, J. B. and Schneider, C. M. and Balents, L. and de Groot, F. M. F. and Stemmer, S. and Fadley, C. S.},

  abstractNote = {},

  doi          = {10.1103/PhysRevB.93.245103},

  journal      = {Physical Review B},

  number       = 24,

  volume       = 93,

  place        = {United States},

  year         = {Wed Jun 01 00:00:00 EDT 2016},

  month        = {Wed Jun 01 00:00:00 EDT 2016}

}

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Title: Energetic, spatial, and momentum character of the electronic structure at a buried interface: The two-dimensional electron gas between two metal oxides

Citation Formats

Efficient hybrid density functional calculations in solids: Assessment of the Heyd–Scuseria–Ernzerhof screened Coulomb hybrid functional journal, July 2004

Projector augmented-wave method journal, December 1994

Hybrid functionals based on a screened Coulomb potential journal, May 2003

Soft-X-ray ARPES at the Swiss Light Source: From 3D Materials to Buried Interfaces and Impurities journal, March 2014

Screened hybrid density functionals applied to solids journal, April 2006

Two-Dimensional Electron Gases at Complex Oxide Interfaces journal, July 2014

Dimer Mott insulator in an oxide heterostructure journal, April 2013

Turning SrTiO 3 into a Mott insulator journal, November 2014

Calculating condensed matter properties using the KKR-Green's function method—recent developments and applications journal, August 2011

Calculation for the charge-transfer effect of La compounds in the 3 d − 1 core-hole state journal, April 1998

Unintentional F doping of SrTiO3(001) etched in HF acid-structure and electronic properties journal, February 2012

Extreme charge density SrTiO 3 /GdTiO 3 heterostructure field effect transistors journal, June 2013

Capacitance-voltage analysis of high-carrier-density SrTiO 3 /GdTiO 3 heterostructures journal, June 2012

Simulation of Electron Spectra for Surface Analysis (SESSA)for quantitative interpretation of (hard) X-ray photoelectron spectra(HAXPES) journal, October 2013

Soft-X-ray ARPES facility at the ADRESS beamline of the SLS: concepts, technical realisation and scientific applications journal, November 2013

Mineral-Aqueous Solution Interfaces and Their Impact on the Environment journal, October 2012

Band offsets in complex-oxide thin films and heterostructures of SrTiO 3 /LaNiO 3 and SrTiO 3 /GdTiO 3 by soft and hard X-ray photoelectron spectroscopy journal, April 2013

Hybrid functionals applied to perovskites journal, May 2014

Suppression of Ionic Liquid Gate-Induced Metallization of SrTiO 3 (001) by Oxygen journal, September 2013

Momentum-resolved electronic structure at a buried interface from soft X-ray standing-wave angle-resolved photoemission journal, October 2013

Modulation of over 10 14 cm −2 electrons in SrTiO 3 /GdTiO 3 heterostructures journal, May 2014

In-gap electronic structure of LaAlO 3 -SrTiO 3 heterointerfaces investigated by soft x-ray spectroscopy journal, December 2011

Symmetry Lowering in Extreme-Electron-Density Perovskite Quantum Wells journal, June 2013

Growth and properties of GdTiO3 films prepared by hybrid molecular beam epitaxy journal, September 2012

Toward an artificial Mott insulator: Correlations in confined high-density electron liquids in SrTiO 3 journal, November 2012

Two-dimensional electron gas with universal subbands at the surface of SrTiO3 journal, January 2011

Quasi-Electric Fields and band Offsets: Teaching Electrons new Tricks journal, February 2002

Correlation between metal-insulator transitions and structural distortions in high-electron-density SrTiO 3 quantum wells journal, February 2014

Creation and control of a two-dimensional electron liquid at the bare SrTiO3 surface journal, January 2011

Magnetic effects at the interface between non-magnetic oxides journal, June 2007

Looking Deeper: Angle-Resolved Photoemission with Soft and Hard X-rays journal, September 2012

Exploring the XPS limit in soft and hard x-ray angle-resolved photoemission using a temperature-dependent one-step theory journal, November 2013

Photoelectron study of SrTiO 3 : An inspection of core-level binding energies with the use of a point-ion model and self-consistent atomic-structure calculations journal, November 1990

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set journal, July 1996

Dominant role of oxygen vacancies in electrical properties of unannealed LaAlO 3 /SrTiO 3 interfaces journal, February 2014

Functional oxide interfaces journal, December 2013

Competition between screening channels in core-level x-ray photoemission as a probe of changes in the ground-state properties of transition-metal compounds journal, August 2006

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set journal, October 1996

X-Ray Interactions: Photoabsorption, Scattering, Transmission, and Reflection at E = 50-30,000 eV, Z = 1-92 journal, July 1993

Aqueous solution/metal interfaces investigated in operando by photoelectron spectroscopy journal, January 2015

Making use of x-ray optical effects in photoelectron-, Auger electron-, and x-ray emission spectroscopies: Total reflection, standing-wave excitation, and resonant effects journal, February 2013

Concentration and chemical-state profiles at heterogeneous interfaces with sub-nm accuracy from standing-wave ambient-pressure photoemission journal, November 2014

Interface properties of magnetic tunnel junction La 0.7 Sr 0.3 MnO 3 / SrTiO 3 superlattices studied by standing-wave excited photoemission spectroscopy journal, November 2010

Electrochemical Aspects of Ionic Liquids book, March 2011

Transport in ferromagnetic GdTiO3/SrTiO3 heterostructures journal, March 2011

Two-beam dynamical diffraction solution of the phase problem: A determination with x-ray standing-wave fields journal, November 1985

Oxide interfaces for novel electronic applications journal, February 2014

Band Alignment, Built-In Potential, and the Absence of Conductivity at the LaCrO 3 / SrTiO 3 ( 001 ) Heterojunction journal, November 2011

Polaronic satellites in x-ray-absorption spectra journal, June 1990

A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface journal, January 2004

Direct k -Space Mapping of the Electronic Structure in an Oxide-Oxide Interface journal, June 2013

Unfolding of electronic structure through induced representations of space groups: Application to Fe-based superconductors journal, November 2014

Superconducting Interfaces Between Insulating Oxides journal, August 2007

Carrier-Controlled Ferromagnetism in SrTiO 3 journal, June 2012

Electrostatic carrier doping of GdTiO 3 /SrTiO 3 interfaces journal, December 2011

Observation by resonant angle-resolved photoemission of a critical thickness for 2-dimensional electron gas formation in SrTiO3 embedded in GdTiO3 journal, December 2015

Direct imaging of the coexistence of ferromagnetism and superconductivity at the LaAlO3/SrTiO3 interface journal, September 2011

Fermi Surface of Three-Dimensional La 1 − x Sr x MnO 3 Explored by Soft-X-Ray ARPES: Rhombohedral Lattice Distortion and its Effect on Magnetoresistance journal, June 2015

High-density Two-Dimensional Small Polaron Gas in a Delta-Doped Mott Insulator journal, November 2013

Efficient hybrid density functional calculations in solids: Assessment of the Heyd–Scuseria–Ernzerhof screened Coulomb hybrid functional
journal, July 2004

Projector augmented-wave method
journal, December 1994

Hybrid functionals based on a screened Coulomb potential
journal, May 2003

Soft-X-ray ARPES at the Swiss Light Source: From 3D Materials to Buried Interfaces and Impurities
journal, March 2014

Screened hybrid density functionals applied to solids
journal, April 2006

Two-Dimensional Electron Gases at Complex Oxide Interfaces
journal, July 2014

Dimer Mott insulator in an oxide heterostructure
journal, April 2013

Turning ${SrTiO}_{3}$ into a Mott insulator
journal, November 2014

Calculating condensed matter properties using the KKR-Green's function method—recent developments and applications
journal, August 2011

Calculation for the charge-transfer effect of La compounds in the ${3 d}^{- 1}$ core-hole state
journal, April 1998

Unintentional F doping of SrTiO3(001) etched in HF acid-structure and electronic properties
journal, February 2012

Extreme charge density SrTiO ₃ /GdTiO ₃ heterostructure field effect transistors
journal, June 2013

Capacitance-voltage analysis of high-carrier-density SrTiO ₃ /GdTiO ₃ heterostructures
journal, June 2012

Simulation of Electron Spectra for Surface Analysis (SESSA)for quantitative interpretation of (hard) X-ray photoelectron spectra(HAXPES)
journal, October 2013

Soft-X-ray ARPES facility at the ADRESS beamline of the SLS: concepts, technical realisation and scientific applications
journal, November 2013

Mineral-Aqueous Solution Interfaces and Their Impact on the Environment
journal, October 2012

Band offsets in complex-oxide thin films and heterostructures of SrTiO ₃ /LaNiO ₃ and SrTiO ₃ /GdTiO ₃ by soft and hard X-ray photoelectron spectroscopy
journal, April 2013

Hybrid functionals applied to perovskites
journal, May 2014

Suppression of Ionic Liquid Gate-Induced Metallization of SrTiO ₃ (001) by Oxygen
journal, September 2013

Momentum-resolved electronic structure at a buried interface from soft X-ray standing-wave angle-resolved photoemission
journal, October 2013

Modulation of over 10 ¹⁴ cm ⁻² electrons in SrTiO ₃ /GdTiO ₃ heterostructures
journal, May 2014

In-gap electronic structure of LaAlO $_{3}$ -SrTiO $_{3}$ heterointerfaces investigated by soft x-ray spectroscopy
journal, December 2011

Symmetry Lowering in Extreme-Electron-Density Perovskite Quantum Wells
journal, June 2013

Growth and properties of GdTiO3 films prepared by hybrid molecular beam epitaxy
journal, September 2012

Toward an artificial Mott insulator: Correlations in confined high-density electron liquids in SrTiO $_{3}$
journal, November 2012

Two-dimensional electron gas with universal subbands at the surface of SrTiO₃
journal, January 2011

Quasi-Electric Fields and band Offsets: Teaching Electrons new Tricks
journal, February 2002

Correlation between metal-insulator transitions and structural distortions in high-electron-density SrTiO $_{3}$ quantum wells
journal, February 2014

Creation and control of a two-dimensional electron liquid at the bare SrTiO3 surface
journal, January 2011

Magnetic effects at the interface between non-magnetic oxides
journal, June 2007

Looking Deeper: Angle-Resolved Photoemission with Soft and Hard X-rays
journal, September 2012

Exploring the XPS limit in soft and hard x-ray angle-resolved photoemission using a temperature-dependent one-step theory
journal, November 2013

Photoelectron study of ${SrTiO}_{3}$ : An inspection of core-level binding energies with the use of a point-ion model and self-consistent atomic-structure calculations
journal, November 1990

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
journal, July 1996

Dominant role of oxygen vacancies in electrical properties of unannealed LaAlO ₃ /SrTiO ₃ interfaces
journal, February 2014

Functional oxide interfaces
journal, December 2013

Competition between screening channels in core-level x-ray photoemission as a probe of changes in the ground-state properties of transition-metal compounds
journal, August 2006

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996

X-Ray Interactions: Photoabsorption, Scattering, Transmission, and Reflection at E = 50-30,000 eV, Z = 1-92
journal, July 1993

Aqueous solution/metal interfaces investigated in operando by photoelectron spectroscopy
journal, January 2015

Making use of x-ray optical effects in photoelectron-, Auger electron-, and x-ray emission spectroscopies: Total reflection, standing-wave excitation, and resonant effects
journal, February 2013

Concentration and chemical-state profiles at heterogeneous interfaces with sub-nm accuracy from standing-wave ambient-pressure photoemission
journal, November 2014

Interface properties of magnetic tunnel junction ${La}_{0.7} {Sr}_{0.3} {MnO}_{3} / {SrTiO}_{3}$ superlattices studied by standing-wave excited photoemission spectroscopy
journal, November 2010

Electrochemical Aspects of Ionic Liquids
book, March 2011

Transport in ferromagnetic GdTiO3/SrTiO3 heterostructures
journal, March 2011

Two-beam dynamical diffraction solution of the phase problem: A determination with x-ray standing-wave fields
journal, November 1985

Oxide interfaces for novel electronic applications
journal, February 2014

Band Alignment, Built-In Potential, and the Absence of Conductivity at the ${LaCrO}_{3} / {SrTiO}_{3} (001)$ Heterojunction
journal, November 2011

Polaronic satellites in x-ray-absorption spectra
journal, June 1990

A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface
journal, January 2004

Direct $k$ -Space Mapping of the Electronic Structure in an Oxide-Oxide Interface
journal, June 2013

Unfolding of electronic structure through induced representations of space groups: Application to Fe-based superconductors
journal, November 2014

Superconducting Interfaces Between Insulating Oxides
journal, August 2007

Carrier-Controlled Ferromagnetism in ${SrTiO}_{3}$
journal, June 2012

Electrostatic carrier doping of GdTiO ₃ /SrTiO ₃ interfaces
journal, December 2011

Observation by resonant angle-resolved photoemission of a critical thickness for 2-dimensional electron gas formation in SrTiO3 embedded in GdTiO3
journal, December 2015

Direct imaging of the coexistence of ferromagnetism and superconductivity at the LaAlO₃/SrTiO₃ interface
journal, September 2011

Fermi Surface of Three-Dimensional ${La}_{1 - x} {Sr}_{x} {MnO}_{3}$ Explored by Soft-X-Ray ARPES: Rhombohedral Lattice Distortion and its Effect on Magnetoresistance
journal, June 2015

High-density Two-Dimensional Small Polaron Gas in a Delta-Doped Mott Insulator
journal, November 2013