Effective spin-12 scalar chiral order on kagome lattices in Nd3Sb3Mg2O14

Scheie, A.; Sanders, M.; Krizan, J.; Qiu, Y.; Cava, R. J.; Broholm, C.

doi:10.1103/PhysRevB.93.180407

Title: Effective spin- $\frac{1}{2}$ scalar chiral order on kagome lattices in ${Nd}_{3} {Sb}_{3} {Mg}_{2} O_{14}$

Abstract

We introduce Nd₃Sb₃Mg₂O₁₄ with ideal kagome lattices of neodymium ions in ABC stacking. Thermodynamic measurements show a Curie-Weiss temperature of Θ_CW = – 0.12 K, a Nd³⁺ spin- $\frac{1}{2}$ Kramers doublet ground state, and a second-order phase transition at T_N = 0.56 (2) K. Neutron scattering reveals noncoplanar scalar chiral k = 0 magnetic order with a correlation length exceeding 400 Å = 55a and an ordered moment of 1.79 (5) μ_B. Furthermore, this order includes a canted ferromagnetic component perpendicular to the kagome planes favored by Dzyaloshinskii-Moriya interactions.

Authors:

Scheie, A. ^[1]; Sanders, M. ^[2]; Krizan, J. ^[2]; Qiu, Y. ^[3]; Cava, R. J. ^[2]; Broholm, C. ^[4]

Johns Hopkins Univ., Baltimore, MD (United States)
Princeton Univ., NJ (United States)
National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
Johns Hopkins Univ., Baltimore, MD (United States); National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)

Publication Date:: Fri May 20 00:00:00 EDT 2016

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

OSTI Identifier:: 1322355

Alternate Identifier(s):: OSTI ID: 1254057

Grant/Contract Number:: AC02-06CH11357; FG02-08ER46544; DMR-1508249

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 93; Journal Issue: 18; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: ENGLISH

Subject:: 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; antiferromagnetism; composition; Dzyaloshinskii-Moriya interaction; ferromagnetism; frustrated magnetism; magnetic interactions; magnetic order; magnetic phase transitions; magnetic susceptibility; condensed matter & materials physics

Citation Formats


                    Scheie, A., Sanders, M., Krizan, J., Qiu, Y., Cava, R. J., and Broholm, C. Effective spin-12 scalar chiral order on kagome lattices in Nd3Sb3Mg2O14.  United States: N. p., 2016. 
Web.  doi:10.1103/PhysRevB.93.180407.

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                    Scheie, A., Sanders, M., Krizan, J., Qiu, Y., Cava, R. J., & Broholm, C. Effective spin-12 scalar chiral order on kagome lattices in Nd3Sb3Mg2O14.  United States.  https://doi.org/10.1103/PhysRevB.93.180407

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                    Scheie, A., Sanders, M., Krizan, J., Qiu, Y., Cava, R. J., and Broholm, C. Fri .  
"Effective spin-12 scalar chiral order on kagome lattices in Nd3Sb3Mg2O14".  United States.  https://doi.org/10.1103/PhysRevB.93.180407.  https://www.osti.gov/servlets/purl/1322355.

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@article{osti_1322355,

  title        = {Effective spin-12 scalar chiral order on kagome lattices in Nd3Sb3Mg2O14},

  author       = {Scheie, A. and Sanders, M. and Krizan, J. and Qiu, Y. and Cava, R. J. and Broholm, C.},

  abstractNote = {We introduce Nd3Sb3Mg2O14 with ideal kagome lattices of neodymium ions in ABC stacking. Thermodynamic measurements show a Curie-Weiss temperature of ΘCW = – 0.12 K, a Nd3+ spin-12 Kramers doublet ground state, and a second-order phase transition at TN = 0.56 (2) K. Neutron scattering reveals noncoplanar scalar chiral k = 0 magnetic order with a correlation length exceeding 400 Å = 55a and an ordered moment of 1.79 (5) μB. Furthermore, this order includes a canted ferromagnetic component perpendicular to the kagome planes favored by Dzyaloshinskii-Moriya interactions.},

  doi          = {10.1103/PhysRevB.93.180407},

  journal      = {Physical Review B},

  number       = 18,

  volume       = 93,

  place        = {United States},

  year         = {Fri May 20 00:00:00 EDT 2016},

  month        = {Fri May 20 00:00:00 EDT 2016}

}

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Title: Effective spin- 1 2 scalar chiral order on kagome lattices in Nd 3 Sb 3 Mg 2 O 14

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Spin folding in the two-dimensional Heisenberg kagomé antiferromagnet journal, June 1993

MACS—a new high intensity cold neutron spectrometer at NIST journal, January 2008

Strong frustration and dilution-enhanced order in a quasi-2D spin glass journal, April 1990

Thermal Hall Effect of Spin Excitations in a Kagome Magnet journal, September 2015

Global phase diagram of competing ordered and quantum spin-liquid phases on the kagome lattice journal, February 2015

Spin anisotropy and quantum Hall effect in the kagomé lattice: Chiral spin state based on a ferromagnet journal, September 2000

Structural and magnetic investigations of single-crystalline neodymium zirconate pyrochlore Nd 2 Zr 2 O 7 journal, May 2015

Hyperfine Interactions in Rare‐Earth Metals journal, April 1963

Geometric Magnetic Frustration in Ba 2 Sn 2 Ga 3 ZnCr 7 O 22 : A Two-Dimensional Spinel Based Kagomé Lattice journal, January 2001

Dzyaloshinskii-Moriya interaction and spin reorientation transition in the frustrated kagome lattice antiferromagnet journal, June 2011

A new protocol for the determination of magnetic structures using simulated annealing and representational analysis (SARAh) journal, March 2000

Magnetic structure and spin waves in the Kagomé jarosite compound K Fe 3 ( S O 4 ) 2 ( O H ) 6 journal, June 2006

A Structurally Perfect S = 1 / 2 Kagomé Antiferromagnet journal, October 2005

Magnetic frustration in lead pyrochlores journal, March 2015

Structural and magnetic properties of new rare-earth – antimony pyrochlore-type oxides Ln2BSbO7 (B = Sc, Ga, In) journal, April 2010

Synthesis and structure of new pyrochlore-type oxides Ln2ScNbO7 (Ln=Pr, Nd, Eu, Gd, Dy) journal, August 2008

RE 3 Sb 3 Zn 2 O 14 (RE = La, Pr, Nd, Sm, Eu, Gd): a new family of pyrochlore derivatives with rare earth ions on a 2D Kagome lattice journal, January 2016

Low-Temperature Magnetic Properties of Pyrochlore Stannates journal, June 2002

Statistics of Kagome Lattice journal, June 1951

Syntheses and properties of a family of new compounds RE3Sb3Co2O14 (RE=La, Pr, Nd, Sm–Ho) with an ordered pyrochlore structure journal, September 2014

Magnetic Ground States of the Rare-Earth Tripod Kagome Lattice Mg 2 RE 3 Sb 3 O 14 ( RE = Gd , Dy , Er ) journal, April 2016

Less than 50% sublattice polarization in an insulating S = 3 2 kagomé antiferromagnet at T ≈ 0 journal, October 1997

Three-sublattice order in triangular- and Kagomé-lattice spin-half antiferromagnets journal, March 1992

Magnetic structure of the kagomé lattice antiferromagnet potassium jarosite KFe 3 ( OH ) 6 ( S O 4 ) 2 journal, May 2000

Symmetry breaking due to Dzyaloshinsky-Moriya interactions in the kagomé lattice journal, July 2002

Spin Dynamics of the Spin- 1 / 2 Kagome Lattice Antiferromagnet ZnCu 3 ( OH ) 6 Cl 2 journal, March 2007

Hidden Magnetic Frustration by Quantum Relaxation in Anisotropic Nd Langasite journal, June 2008

Kagome lattice antiferromagnets and Dzyaloshinsky-Moriya interactions journal, November 2007

On the Spin Arrangement in “Kagome” Lattice of Antiferromagnetic KFe 3 (OH) 6 (SO 4 ) 2 journal, April 1971

Statistics of Kagomé Lattice journal, September 1951

A Structurally Perfect S = 1/2 Kagome Antiferromagnet. journal, December 2005

Geometric Magnetic Frustration in Ba2Sn2Ga3ZnCr7O22: A Two-Dimensional Spinel Based Kagomé Lattice text, January 2001

Kagome lattice antiferromagnets and Dzyaloshinsky-Moriya interactions text, January 2007

Hidden magnetic frustration by quantum relaxation in anisotropic Nd-langasite text, January 2008

Vesignieite BaCu3V2O8(OH)2 as a Candidate Spin-1/2 Kagome Antiferromagnet text, January 2009

Dzyaloshinskii-Moriya interaction and spin re-orientation transition in the frustrated kagome lattice antiferromagnet text, January 2011

Magnetic Frustration in Lead Pyrochlores text, January 2015

Symmetry breaking due to Dzyaloshinsky-Moriya interactions in the kagome lattice text, January 2002

Synthesis, crystal structure, and magnetic properties of novel 2D kagome materials RE 3 Sb 3 Mg 2 O 14 (RE = La, Pr, Sm, Eu, Tb, Ho): Comparison to RE 3 Sb 3 Zn 2 O 14 family : Properties of novel 2D kagome materials RE journal, August 2016

Emergent order in the kagome Ising magnet Dy3Mg2Sb3O14 journal, December 2016

Magnetic states of coupled spin tubes with frustrated geometry in CsCrF4 journal, April 2019

Magnetic properties of lithium-containing rare earth garnets Li 3 RE 3 Te 2 O 12 (RE = Y, Pr, Nd, Sm-Lu) journal, September 2018

Magnonic analogs of topological Dirac semimetals journal, September 2017

Majorana spin liquids, topology, and superconductivity in ladders journal, November 2017

Engineering quantum spin liquids and many-body Majorana states with a driven superconducting box circuit journal, July 2018

Supercooling and fragile glassiness in a dipolar kagome Ising magnet journal, October 2018

Emergent order in the kagome Ising magnet Dy$_3$Mg$_2$Sb$_3$O$_{14}$ text, January 2016

Supercooling and fragile glassiness in a dipolar kagome Ising magnet text, January 2018

Magnonic Analogs of Topological Dirac Semimetals text, January 2016

Majorana Spin Liquids, Topology and Superconductivity in Ladders text, January 2017

Engineering Quantum Spin Liquids and Many-Body Majorana States with a Driven Superconducting Box Circuit text, January 2018

Supercooling and fragile glassiness in a dipolar kagome Ising magnet text, January 2018

Ground-state phase diagram of the Kitaev-Heisenberg model on a kagome lattice text, January 2018

Title: Effective spin- $\frac{1}{2}$ scalar chiral order on kagome lattices in ${Nd}_{3} {Sb}_{3} {Mg}_{2} O_{14}$

Crystal structure of Mn2Ln3Sb3O14 (Ln=La, Pr and Nd): A new ordered rhombohedral pyrochlore
journal, May 2014

Spin-1/2 Kagomé -Like Lattice in Volborthite Cu ₃ V ₂ O ₇ (OH) ₂ ·2H ₂ O
journal, November 2001

Magnetic frustration on a Kagomé lattice in R ₃ Ga ₅ SiO ₁₄ langasites with R = Nd, Pr
journal, May 2006

Magnetic pyrochlore oxides
journal, January 2010

Models for ordering in the jarosites Kagomé systems
journal, June 2003

A kagome map of spin liquids from XXZ to Dzyaloshinskii–Moriya ferromagnet
journal, January 2016

Vesignieite BaCu ₃ V ₂ O ₈ (OH) ₂ as a Candidate Spin-1/2 Kagome Antiferromagnet
journal, March 2009

Schwinger-boson approach to the kagome antiferromagnet with Dzyaloshinskii-Moriya interactions: Phase diagram and dynamical structure factors
journal, February 2010

Topological excitations and the dynamic structure factor of spin liquids on the kagome lattice
journal, March 2014

Magnetic ordering and spin dynamics in potassium jarosite: A Heisenberg kagomé lattice antiferromagnet
journal, June 2003

Spin-Liquid Ground State of the S = 1/2 Kagome Heisenberg Antiferromagnet
journal, April 2011

Recent advances in magnetic structure determination by neutron powder diffraction
journal, October 1993

Magnetic frustration and lattice dimensionality in SrCr8Ga4O19
journal, January 1988

Quantum criticality of the kagome antiferromagnet with Dzyaloshinskii-Moriya interactions
journal, April 2010

Order from disorder in a kagomé antiferromagnet
journal, August 1992

Spin folding in the two-dimensional Heisenberg kagomé antiferromagnet
journal, June 1993

MACS—a new high intensity cold neutron spectrometer at NIST
journal, January 2008

Strong frustration and dilution-enhanced order in a quasi-2D spin glass
journal, April 1990

Thermal Hall Effect of Spin Excitations in a Kagome Magnet
journal, September 2015

Global phase diagram of competing ordered and quantum spin-liquid phases on the kagome lattice
journal, February 2015

Spin anisotropy and quantum Hall effect in the kagomé lattice: Chiral spin state based on a ferromagnet
journal, September 2000

Structural and magnetic investigations of single-crystalline neodymium zirconate pyrochlore ${Nd}_{2} {Zr}_{2} O_{7}$
journal, May 2015

Hyperfine Interactions in Rare‐Earth Metals
journal, April 1963

Geometric Magnetic Frustration in ${Ba}_{2} {Sn}_{2} {Ga}_{3} {ZnCr}_{7} O_{22}$ : A Two-Dimensional Spinel Based Kagomé Lattice
journal, January 2001

Dzyaloshinskii-Moriya interaction and spin reorientation transition in the frustrated kagome lattice antiferromagnet
journal, June 2011

A new protocol for the determination of magnetic structures using simulated annealing and representational analysis (SARAh)
journal, March 2000

Magnetic structure and spin waves in the Kagomé jarosite compound $K {Fe}_{3} {(S O_{4})}_{2} {(O H)}_{6}$
journal, June 2006

A Structurally Perfect S = ¹ / ₂ Kagomé Antiferromagnet
journal, October 2005

Magnetic frustration in lead pyrochlores
journal, March 2015

Structural and magnetic properties of new rare-earth – antimony pyrochlore-type oxides Ln2BSbO7 (B = Sc, Ga, In)
journal, April 2010

Synthesis and structure of new pyrochlore-type oxides Ln2ScNbO7 (Ln=Pr, Nd, Eu, Gd, Dy)
journal, August 2008

RE ₃ Sb ₃ Zn ₂ O ₁₄ (RE = La, Pr, Nd, Sm, Eu, Gd): a new family of pyrochlore derivatives with rare earth ions on a 2D Kagome lattice
journal, January 2016

Low-Temperature Magnetic Properties of Pyrochlore Stannates
journal, June 2002

Statistics of Kagome Lattice
journal, June 1951

Syntheses and properties of a family of new compounds RE3Sb3Co2O14 (RE=La, Pr, Nd, Sm–Ho) with an ordered pyrochlore structure
journal, September 2014

Magnetic Ground States of the Rare-Earth Tripod Kagome Lattice ${Mg}_{2} {RE}_{3} {Sb}_{3} O_{14}$ ( $RE = Gd, Dy, Er$ )
journal, April 2016

Less than 50% sublattice polarization in an insulating $S =$ $\frac{3}{2}$ kagomé antiferromagnet at $T \approx 0$
journal, October 1997

Three-sublattice order in triangular- and Kagomé-lattice spin-half antiferromagnets
journal, March 1992

Magnetic structure of the kagomé lattice antiferromagnet potassium jarosite ${KFe}_{3} {(OH)}_{6} {(S O}_{4})_{2}$
journal, May 2000

Symmetry breaking due to Dzyaloshinsky-Moriya interactions in the kagomé lattice
journal, July 2002

Spin Dynamics of the Spin- $1 / 2$ Kagome Lattice Antiferromagnet ${ZnCu}_{3} (OH)_{6} {Cl}_{2}$
journal, March 2007

Hidden Magnetic Frustration by Quantum Relaxation in Anisotropic Nd Langasite
journal, June 2008

Kagome lattice antiferromagnets and Dzyaloshinsky-Moriya interactions
journal, November 2007

On the Spin Arrangement in “Kagome” Lattice of Antiferromagnetic KFe ₃ (OH) ₆ (SO ₄ ) ₂
journal, April 1971

Statistics of Kagomé Lattice
journal, September 1951

A Structurally Perfect S = 1/2 Kagome Antiferromagnet.
journal, December 2005

Geometric Magnetic Frustration in Ba2Sn2Ga3ZnCr7O22: A Two-Dimensional Spinel Based Kagomé Lattice
text, January 2001

Kagome lattice antiferromagnets and Dzyaloshinsky-Moriya interactions
text, January 2007

Hidden magnetic frustration by quantum relaxation in anisotropic Nd-langasite
text, January 2008

Vesignieite BaCu3V2O8(OH)2 as a Candidate Spin-1/2 Kagome Antiferromagnet
text, January 2009

Dzyaloshinskii-Moriya interaction and spin re-orientation transition in the frustrated kagome lattice antiferromagnet
text, January 2011

Magnetic Frustration in Lead Pyrochlores
text, January 2015

Symmetry breaking due to Dzyaloshinsky-Moriya interactions in the kagome lattice
text, January 2002

Synthesis, crystal structure, and magnetic properties of novel 2D kagome materials RE ₃ Sb ₃ Mg ₂ O ₁₄ (RE = La, Pr, Sm, Eu, Tb, Ho): Comparison to RE ₃ Sb ₃ Zn ₂ O ₁₄ family : Properties of novel 2D kagome materials RE
journal, August 2016

Emergent order in the kagome Ising magnet Dy3Mg2Sb3O14
journal, December 2016

Magnetic states of coupled spin tubes with frustrated geometry in CsCrF4
journal, April 2019

Magnetic properties of lithium-containing rare earth garnets Li ₃ RE ₃ Te ₂ O ₁₂ (RE = Y, Pr, Nd, Sm-Lu)
journal, September 2018

Magnonic analogs of topological Dirac semimetals
journal, September 2017

Majorana spin liquids, topology, and superconductivity in ladders
journal, November 2017

Engineering quantum spin liquids and many-body Majorana states with a driven superconducting box circuit
journal, July 2018

Supercooling and fragile glassiness in a dipolar kagome Ising magnet
journal, October 2018

Emergent order in the kagome Ising magnet Dy$_3$Mg$_2$Sb$_3$O$_{14}$
text, January 2016

Supercooling and fragile glassiness in a dipolar kagome Ising magnet
text, January 2018

Magnonic Analogs of Topological Dirac Semimetals
text, January 2016

Majorana Spin Liquids, Topology and Superconductivity in Ladders
text, January 2017

Engineering Quantum Spin Liquids and Many-Body Majorana States with a Driven Superconducting Box Circuit
text, January 2018

Supercooling and fragile glassiness in a dipolar kagome Ising magnet
text, January 2018

Ground-state phase diagram of the Kitaev-Heisenberg model on a kagome lattice
text, January 2018