Reprint of “Mass-selected supported cluster catalysts: Size effects on CO oxidation activity, electronic structure, and thermal stability of Pd /alumina (n≤ 30) model catalysts”

Kane, Matthew D.; Roberts, F. Sloan; Anderson, Scott L.

doi:10.1016/j.ijms.2014.07.044

Title: Reprint of “Mass-selected supported cluster catalysts: Size effects on CO oxidation activity, electronic structure, and thermal stability of Pd /alumina (n≤ 30) model catalysts”

Authors:: Kane, Matthew D.; Roberts, F. Sloan; Anderson, Scott L.

Publication Date:: Sun Feb 01 00:00:00 EST 2015

Sponsoring Org.:: USDOE

OSTI Identifier:: 1253411

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: International Journal of Mass Spectrometry

Additional Journal Information:: Journal Name: International Journal of Mass Spectrometry Journal Volume: 377 Journal Issue: C; Journal ID: ISSN 1387-3806

Publisher:: Elsevier

Country of Publication:: Netherlands

Language:: English

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                    Kane, Matthew D., Roberts, F. Sloan, and Anderson, Scott L. Reprint of “Mass-selected supported cluster catalysts: Size effects on CO oxidation activity, electronic structure, and thermal stability of Pd /alumina (n≤ 30) model catalysts”.  Netherlands: N. p., 2015. 
Web.  doi:10.1016/j.ijms.2014.07.044.

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                    Kane, Matthew D., Roberts, F. Sloan, & Anderson, Scott L. Reprint of “Mass-selected supported cluster catalysts: Size effects on CO oxidation activity, electronic structure, and thermal stability of Pd /alumina (n≤ 30) model catalysts”.  Netherlands.  https://doi.org/10.1016/j.ijms.2014.07.044

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                    Kane, Matthew D., Roberts, F. Sloan, and Anderson, Scott L. Sun .  
"Reprint of “Mass-selected supported cluster catalysts: Size effects on CO oxidation activity, electronic structure, and thermal stability of Pd /alumina (n≤ 30) model catalysts”".  Netherlands.  https://doi.org/10.1016/j.ijms.2014.07.044.

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@article{osti_1253411,

  title        = {Reprint of “Mass-selected supported cluster catalysts: Size effects on CO oxidation activity, electronic structure, and thermal stability of Pd /alumina (n≤ 30) model catalysts”},

  author       = {Kane, Matthew D. and Roberts, F. Sloan and Anderson, Scott L.},

  abstractNote = {},

  doi          = {10.1016/j.ijms.2014.07.044},

  journal      = {International Journal of Mass Spectrometry},

  number       = C,

  volume       = 377,

  place        = {Netherlands},

  year         = {Sun Feb 01 00:00:00 EST 2015},

  month        = {Sun Feb 01 00:00:00 EST 2015}

}

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Title: Reprint of “Mass-selected supported cluster catalysts: Size effects on CO oxidation activity, electronic structure, and thermal stability of Pd /alumina (n≤ 30) model catalysts”

Citation Formats

Photolysis of chemisorbed dioxygen on Pd(111): Dependence on photon energy journal, December 1989

The Growth and Properties of Pd and Pt on Al 2 O 3 /NiAl(110) journal, November 1995

Atomic subshell photoionization cross sections and asymmetry parameters: 1 ⩽ Z ⩽ 103 journal, January 1985

Size-Dependent Subnanometer Pd Cluster (Pd 4 , Pd 6 , and Pd 17 ) Water Oxidation Electrocatalysis journal, June 2013

Catalytic CO Oxidation by Free Au2-: Experiment and Theory journal, August 2003

Reaction kinetics on supported model catalysts: Molecular beam/ in situ time-resolved infrared reflection absorption spectroscopy study of the CO oxidation on alumina supported Pd particles journal, July 2001

Electrochemically induced nanocluster migration journal, December 2010

Structural Modification of Platinum Model Systems under High Pressure CO Annealing journal, July 2012

Size-selected clusters as heterogeneous model catalysts under applied reaction conditions journal, January 2010

Oxidative Dehydrogenation of Cyclohexane on Cobalt Oxide (Co 3 O 4 ) Nanoparticles: The Effect of Particle Size on Activity and Selectivity journal, September 2012

Cleavage of the C–O–C bond on size-selected subnanometer cobalt catalysts and on ALD-cobalt coated nanoporous membranes journal, February 2011

Overcoming the Strong Metal−Support Interaction State: CO Oxidation on TiO 2 (110)-Supported Pt Nanoclusters journal, February 2011

Size-dependent selectivity and activity of silver nanoclusters in the partial oxidation of propylene to propylene oxide and acrolein: A joint experimental and theoretical study journal, February 2011

Phase-contrast imaging in aberration-corrected scanning transmission electron microscopy journal, June 2013

Enhanced oxygen binding through surface mediated ionic bonds journal, June 2012

Formic acid adsorption and decomposition on TiO 2 (1 1 0) and on Pd/TiO 2 (1 1 0) model catalysts journal, June 2002

CO adsorption on palladium model catalysts: XPS Pd–Al2O3 interaction study journal, November 2000

Sintering, oxidation, and chemical properties of size-selected nickel clusters on TiO2(110) journal, September 2002

Exceptional oxidation activity with size-controlled supported gold clusters of low atomicity journal, August 2013

Synthesis and catalytic properties of large ligand stabilized palladium clusters journal, May 1996

CO Oxidation on Supported Single Pt Atoms: Experimental and ab Initio Density Functional Studies of CO Interaction with Pt Atom on θ-Al 2 O 3 (010) Surface journal, August 2013

Correlation between Fischer-Tropsch catalytic activity and composition of catalysts journal, November 2011

Model catalysts of supported Au nanoparticles and mass-selected clusters journal, January 2010

Epitaxial growth of ultrathin Al2O3 films on Ta(110) journal, June 1994

Strong Effects of Cluster Size and Air Exposure on Oxygen Reduction and Carbon Oxidation Electrocatalysis by Size-Selected Pt n ( n ≤ 11) on Glassy Carbon Electrodes journal, February 2013

Size-dependent XPS spectra of small supported Au-clusters journal, February 2013

Water on Rutile TiO 2 (110) and Au/TiO 2 (110): Effects on Au Mobility and the Isotope Exchange Reaction journal, May 2008

Interactions between oxygen and carbon monoxide on a Pd(111) surface journal, September 1978

CO 2 as a Probe for Monitoring the Surface Defects on TiO 2 (110)Temperature-Programmed Desorption journal, October 2003

Electronic structure of metal clusters journal, March 1989

Stable Subnanometer Cobalt Oxide Clusters on Ultrananocrystalline Diamond and Alumina Supports: Oxidation State and the Origin of Sintering Resistance journal, November 2012

Size-Selected Monodisperse Nanoclusters on Supported Graphene: Bonding, Isomerism, and Mobility journal, October 2012

Oxidation and Reduction of Mass-Selected Au Clusters on SiO2/Si journal, September 2006

Gold/Titania Interfaces and Their Role in Carbon Monoxide Oxidation journal, January 1999

Model oxide-supported metal catalysts: energetics, particle thicknesses, chemisorption and catalytic properties journal, January 2000

The reactivity of gold and platinum metals in their cluster phase journal, December 1999

Linear and Nonlinear Laser Spectroscopy of Surface Adsorbates with Sub-Monolayer Sensitivity journal, April 2012

Size-effects in the acetylene cyclotrimerization on supported size-selected Pdn clusters (1≤n≤30) journal, May 2000

Surface residence times and reaction mechanism in the catalytic oxidation of CO on Pd(111) journal, February 1978

Adsorption of CO on Pd/Al 2 O 3 /Ta(110) model catalysts journal, May 1996

CO oxidation on Pd(110): a high-resolution XPS and molecular beam study journal, September 1999

Effect of ultraviolet and x-ray radiation on the work function of TiO2 surfaces journal, May 2010

Size Dependence of the Adsorption Energy of CO on Metal Nanoparticles: A DFT Search for the Minimum Value journal, January 2012

Cluster size dependence of Pt core-level shifts for mass-selected Pt clusters on TiO2(110) surfaces journal, September 2010

Chemical properties of size-selected Au clusters treated under ambient conditions journal, May 2008

The Structure of Catalytically Active Gold on Titania journal, October 2004

Oxygen adsorption on well-defined gold particles on TiO2(110) journal, July 1999

Assignment of the d-orbitals involved in the chemisorption bond of CO on Re(0001) journal, January 1979

Activation of oxygen on palladium nanocluster journal, December 2011

CO adsorption on a Pd/TiO2() model catalyst journal, January 2002

Growth of ultrathin crystalline Al 2 O 3 films on Ru(0001) and Re(0001) surfaces journal, July 1996

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Cluster size effects on sintering, CO adsorption, and implantation in Ir/SiO2 journal, September 2009

Oxidation of deposited Aun (n=2–13) on SiO2/Si: Influence of the NaOH(aq) treatment journal, May 2009

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Metal Atoms and Particles on Oxide Supports: Probing Structure and Charge by Infrared Spectroscopy journal, September 2001

The CO+NO Reaction over Pd: A Combined Study Using Single-Crystal, Planar-Model-Supported, and High-Surface-Area Pd/Al2O3Catalysts journal, April 1997

Oxidation State and Symmetry of Magnesia-Supported Pd 13 O x Nanocatalysts Influence Activation Barriers of CO Oxidation journal, April 2012

Highly active surfaces for CO oxidation on Rh, Pd, and Pt journal, December 2007

Supported Pdn (n=1?20) cluster reactivity : CO chemisorption journal, March 1993

Observation of induced dipoles between small palladium clusters and α-(0001) Al 2 O 3 journal, June 1995

Identification of Active Gold Nanoclusters on Iron Oxide Supports for CO Oxidation journal, September 2008

Size-selected Metal Clusters: New Models for Catalysis with Atomic Precision journal, March 2011

Size-dependent oxidation of Pdn (n⩽13) on alumina/NiAl(110): Correlation with Pd core level binding energies journal, September 2009

Subnanometre platinum clusters as highly active and selective catalysts for the oxidative dehydrogenation of propane journal, February 2009

Alumina support and Pdn cluster size effects on activity of Pdn for catalytic oxidation of CO journal, January 2013

Thermal desorption of gases journal, July 1962

A molecular beam investigation of the catalytic oxidation of CO on Pd (111) journal, January 1978

Nanoclusters deposited on surfaces journal, October 2001

CO Adsorption on Monometallic and Bimetallic Au−Pd Nanoparticles Supported on Oxide Thin Films journal, July 2010

Electronic Structure Controls Reactivity of Size-Selected Pd Clusters Adsorbed on TiO2 Surfaces journal, November 2009

Oxidation and reduction of size-selected subnanometer Pd clusters on Al 2 O 3 surface journal, June 2013

The mechanism of the catalytic action of platinum in the reactions 2Co + O2= 2Co2 and 2H2+ O2= 2H2O journal, January 1922

Dual pulsed-beam controlled mole fraction studies of the catalytic oxidation of CO on supported Pd nanocatalysts journal, April 2008

Femtosecond-laser photoemission and photodesorption from magnesia supported gold clusters journal, May 2010

Determination of interface dipole and band bending at the Ag/tris (8-hydroxyquinolinato) gallium organic Schottky contact by ultraviolet photoemission spectroscopy journal, April 2000

Combined temperature-programmed reaction and in situ x-ray scattering studies of size-selected silver clusters under realistic reaction conditions in the epoxidation of propene journal, September 2009

Size-Selected Subnanometer Cluster Catalysts on Semiconductor Nanocrystal Films for Atomic Scale Insight into Photocatalysis journal, October 2012

Photolysis of chemisorbed dioxygen on Pd(111): Dependence on photon energy
journal, December 1989

The Growth and Properties of Pd and Pt on Al ₂ O ₃ /NiAl(110)
journal, November 1995

Atomic subshell photoionization cross sections and asymmetry parameters: 1 ⩽ Z ⩽ 103
journal, January 1985

Size-Dependent Subnanometer Pd Cluster (Pd ₄ , Pd ₆ , and Pd ₁₇ ) Water Oxidation Electrocatalysis
journal, June 2013

Catalytic CO Oxidation by Free Au₂^-: Experiment and Theory
journal, August 2003

Reaction kinetics on supported model catalysts: Molecular beam/ in situ time-resolved infrared reflection absorption spectroscopy study of the CO oxidation on alumina supported Pd particles
journal, July 2001

Electrochemically induced nanocluster migration
journal, December 2010

Structural Modification of Platinum Model Systems under High Pressure CO Annealing
journal, July 2012

Size-selected clusters as heterogeneous model catalysts under applied reaction conditions
journal, January 2010

Oxidative Dehydrogenation of Cyclohexane on Cobalt Oxide (Co ₃ O ₄ ) Nanoparticles: The Effect of Particle Size on Activity and Selectivity
journal, September 2012

Cleavage of the C–O–C bond on size-selected subnanometer cobalt catalysts and on ALD-cobalt coated nanoporous membranes
journal, February 2011

Overcoming the Strong Metal−Support Interaction State: CO Oxidation on TiO ₂ (110)-Supported Pt Nanoclusters
journal, February 2011

Size-dependent selectivity and activity of silver nanoclusters in the partial oxidation of propylene to propylene oxide and acrolein: A joint experimental and theoretical study
journal, February 2011

Phase-contrast imaging in aberration-corrected scanning transmission electron microscopy
journal, June 2013

Enhanced oxygen binding through surface mediated ionic bonds
journal, June 2012

Formic acid adsorption and decomposition on TiO 2 (1 1 0) and on Pd/TiO 2 (1 1 0) model catalysts
journal, June 2002

CO adsorption on palladium model catalysts: XPS Pd–Al2O3 interaction study
journal, November 2000

Sintering, oxidation, and chemical properties of size-selected nickel clusters on TiO2(110)
journal, September 2002

Exceptional oxidation activity with size-controlled supported gold clusters of low atomicity
journal, August 2013

Synthesis and catalytic properties of large ligand stabilized palladium clusters
journal, May 1996

CO Oxidation on Supported Single Pt Atoms: Experimental and ab Initio Density Functional Studies of CO Interaction with Pt Atom on θ-Al ₂ O ₃ (010) Surface
journal, August 2013

Correlation between Fischer-Tropsch catalytic activity and composition of catalysts
journal, November 2011

Model catalysts of supported Au nanoparticles and mass-selected clusters
journal, January 2010

Epitaxial growth of ultrathin Al2O3 films on Ta(110)
journal, June 1994

Strong Effects of Cluster Size and Air Exposure on Oxygen Reduction and Carbon Oxidation Electrocatalysis by Size-Selected Pt _n ( n ≤ 11) on Glassy Carbon Electrodes
journal, February 2013

Size-dependent XPS spectra of small supported Au-clusters
journal, February 2013

Water on Rutile TiO ₂ (110) and Au/TiO ₂ (110): Effects on Au Mobility and the Isotope Exchange Reaction
journal, May 2008

Interactions between oxygen and carbon monoxide on a Pd(111) surface
journal, September 1978

CO ₂ as a Probe for Monitoring the Surface Defects on TiO ₂ (110)Temperature-Programmed Desorption
journal, October 2003

Electronic structure of metal clusters
journal, March 1989

Stable Subnanometer Cobalt Oxide Clusters on Ultrananocrystalline Diamond and Alumina Supports: Oxidation State and the Origin of Sintering Resistance
journal, November 2012

Size-Selected Monodisperse Nanoclusters on Supported Graphene: Bonding, Isomerism, and Mobility
journal, October 2012

Oxidation and Reduction of Mass-Selected Au Clusters on SiO2/Si
journal, September 2006

Gold/Titania Interfaces and Their Role in Carbon Monoxide Oxidation
journal, January 1999

Model oxide-supported metal catalysts: energetics, particle thicknesses, chemisorption and catalytic properties
journal, January 2000

The reactivity of gold and platinum metals in their cluster phase
journal, December 1999

Linear and Nonlinear Laser Spectroscopy of Surface Adsorbates with Sub-Monolayer Sensitivity
journal, April 2012

Size-effects in the acetylene cyclotrimerization on supported size-selected Pdn clusters (1≤n≤30)
journal, May 2000

Surface residence times and reaction mechanism in the catalytic oxidation of CO on Pd(111)
journal, February 1978

Adsorption of CO on Pd/Al ₂ O ₃ /Ta(110) model catalysts
journal, May 1996

CO oxidation on Pd(110): a high-resolution XPS and molecular beam study
journal, September 1999

Effect of ultraviolet and x-ray radiation on the work function of TiO2 surfaces
journal, May 2010

Size Dependence of the Adsorption Energy of CO on Metal Nanoparticles: A DFT Search for the Minimum Value
journal, January 2012

Cluster size dependence of Pt core-level shifts for mass-selected Pt clusters on TiO2(110) surfaces
journal, September 2010

Chemical properties of size-selected Au clusters treated under ambient conditions
journal, May 2008

The Structure of Catalytically Active Gold on Titania
journal, October 2004

Oxygen adsorption on well-defined gold particles on TiO2(110)
journal, July 1999

Assignment of the d-orbitals involved in the chemisorption bond of CO on Re(0001)
journal, January 1979

Activation of oxygen on palladium nanocluster
journal, December 2011

CO adsorption on a Pd/TiO2() model catalyst
journal, January 2002

Growth of ultrathin crystalline Al ₂ O ₃ films on Ru(0001) and Re(0001) surfaces
journal, July 1996

Oxidative Decomposition of Methanol on Subnanometer Palladium Clusters: The Effect of Catalyst Size and Support Composition
journal, May 2010

Cluster size effects on sintering, CO adsorption, and implantation in Ir/SiO2
journal, September 2009

Oxidation of deposited Aun (n=2–13) on SiO2/Si: Influence of the NaOH(aq) treatment
journal, May 2009

Size Dependent Reaction Kinetics on Supported Model Catalysts: A Molecular Beam/IRAS Study of the CO Oxidation on Alumina-Supported Pd Particles
journal, May 2001

Metal Atoms and Particles on Oxide Supports: Probing Structure and Charge by Infrared Spectroscopy
journal, September 2001

The CO+NO Reaction over Pd: A Combined Study Using Single-Crystal, Planar-Model-Supported, and High-Surface-Area Pd/Al2O3Catalysts
journal, April 1997

Oxidation State and Symmetry of Magnesia-Supported Pd ₁₃ O _x Nanocatalysts Influence Activation Barriers of CO Oxidation
journal, April 2012

Highly active surfaces for CO oxidation on Rh, Pd, and Pt
journal, December 2007

Supported Pdn (n=1?20) cluster reactivity : CO chemisorption
journal, March 1993

Observation of induced dipoles between small palladium clusters and α-(0001) ${Al}_{2}$ $O_{3}$
journal, June 1995

Identification of Active Gold Nanoclusters on Iron Oxide Supports for CO Oxidation
journal, September 2008

Size-selected Metal Clusters: New Models for Catalysis with Atomic Precision
journal, March 2011

Size-dependent oxidation of Pdn (n⩽13) on alumina/NiAl(110): Correlation with Pd core level binding energies
journal, September 2009

Subnanometre platinum clusters as highly active and selective catalysts for the oxidative dehydrogenation of propane
journal, February 2009

Alumina support and Pdn cluster size effects on activity of Pdn for catalytic oxidation of CO
journal, January 2013

Thermal desorption of gases
journal, July 1962

A molecular beam investigation of the catalytic oxidation of CO on Pd (111)
journal, January 1978

Nanoclusters deposited on surfaces
journal, October 2001

CO Adsorption on Monometallic and Bimetallic Au−Pd Nanoparticles Supported on Oxide Thin Films
journal, July 2010

Electronic Structure Controls Reactivity of Size-Selected Pd Clusters Adsorbed on TiO2 Surfaces
journal, November 2009

Oxidation and reduction of size-selected subnanometer Pd clusters on Al ₂ O ₃ surface
journal, June 2013

The mechanism of the catalytic action of platinum in the reactions 2Co + O2= 2Co2 and 2H2+ O2= 2H2O
journal, January 1922

Dual pulsed-beam controlled mole fraction studies of the catalytic oxidation of CO on supported Pd nanocatalysts
journal, April 2008

Femtosecond-laser photoemission and photodesorption from magnesia supported gold clusters
journal, May 2010

Determination of interface dipole and band bending at the Ag/tris (8-hydroxyquinolinato) gallium organic Schottky contact by ultraviolet photoemission spectroscopy
journal, April 2000

Combined temperature-programmed reaction and in situ x-ray scattering studies of size-selected silver clusters under realistic reaction conditions in the epoxidation of propene
journal, September 2009

Size-Selected Subnanometer Cluster Catalysts on Semiconductor Nanocrystal Films for Atomic Scale Insight into Photocatalysis
journal, October 2012

Understanding the Behavior of TiO ₂ (110)-Supported Pd ₇ Cluster: A Density Functional Study
journal, November 2012

Structure sensitivity of CO oxidation over model Au/TiO₂ ₂ catalysts
journal, January 1998