Measurement and Modeling of U(IV) Adsorption to Metal Oxide Minerals

Wang, Zimeng; Ulrich, Kai-Uwe; Pan, Chao; Giammar, Daniel E.

doi:10.1021/acs.estlett.5b00156

Title: Measurement and Modeling of U(IV) Adsorption to Metal Oxide Minerals

Authors:

Wang, Zimeng ^[1]; Ulrich, Kai-Uwe ^[2]; Pan, Chao ^[3]; Giammar, Daniel E. ^[3]

Department of Civil and Environmental Engineering, Stanford University, Stanford, California 94305, United States
BGD Soil and Groundwater Laboratory, 01219 Dresden, Germany
Department of Energy, Environmental and Chemical Engineering, Washington University in St. Louis, St. Louis, Missouri 63130, United States

Publication Date:: Thu Jul 09 00:00:00 EDT 2015

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1245506

Grant/Contract Number:: FG02-06ER64227

Resource Type:: Published Article

Journal Name:: Environmental Science & Technology Letters (Online)

Additional Journal Information:: Journal Name: Environmental Science & Technology Letters (Online) Journal Volume: 2 Journal Issue: 8; Journal ID: ISSN 2328-8930

Publisher:: American Chemical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Wang, Zimeng, Ulrich, Kai-Uwe, Pan, Chao, and Giammar, Daniel E. Measurement and Modeling of U(IV) Adsorption to Metal Oxide Minerals.  United States: N. p., 2015. 
Web.  doi:10.1021/acs.estlett.5b00156.

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                    Wang, Zimeng, Ulrich, Kai-Uwe, Pan, Chao, & Giammar, Daniel E. Measurement and Modeling of U(IV) Adsorption to Metal Oxide Minerals.  United States.  https://doi.org/10.1021/acs.estlett.5b00156

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                    Wang, Zimeng, Ulrich, Kai-Uwe, Pan, Chao, and Giammar, Daniel E. Thu .  
"Measurement and Modeling of U(IV) Adsorption to Metal Oxide Minerals".  United States.  https://doi.org/10.1021/acs.estlett.5b00156.

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@article{osti_1245506,

  title        = {Measurement and Modeling of U(IV) Adsorption to Metal Oxide Minerals},

  author       = {Wang, Zimeng and Ulrich, Kai-Uwe and Pan, Chao and Giammar, Daniel E.},

  abstractNote = {},

  doi          = {10.1021/acs.estlett.5b00156},

  journal      = {Environmental Science & Technology Letters (Online)},

  number       = 8,

  volume       = 2,

  place        = {United States},

  year         = {Thu Jul 09 00:00:00 EDT 2015},

  month        = {Thu Jul 09 00:00:00 EDT 2015}

}

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Influence of Magnetite Stoichiometry on U ^VI Reduction
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Title: Measurement and Modeling of U(IV) Adsorption to Metal Oxide Minerals

Citation Formats

Bioremediation of uranium-contaminated groundwater: a systems approach to subsurface biogeochemistry journal, June 2013

Biogenic Uraninite Nanoparticles and Their Importance for Uranium Remediation journal, December 2008

Influence of Dynamical Conditions on the Reduction of U VI at the Magnetite−Solution Interface journal, January 2010

Additive Surface Complexation Modeling of Uranium(VI) Adsorption onto Quartz-Sand Dominated Sediments journal, May 2014

Adsorption of Ions Dilute Aqueous Solutions on Glass and Plastic Surfaces. journal, June 1965

Adsorption of Uranium(VI) to Manganese Oxides: X-ray Absorption Spectroscopy and Surface Complexation Modeling journal, December 2012

Dissolution of synthetic brannerite in acidic and alkaline fluids journal, September 2003

Kinetics of Uranium(VI) Reduction by Hydrogen Sulfide in Anoxic Aqueous Systems journal, August 2006

Sorption of Th(IV) on MX-80 bentonite: effect of pH and modeling journal, September 2010

U(VI) Reduction to Mononuclear U(IV) by Desulfitobacterium Species journal, June 2010

Stable U(IV) Complexes Form at High-Affinity Mineral Surface Sites journal, January 2014

Products of abiotic U(VI) reduction by biogenic magnetite and vivianite journal, May 2011

Experimental Investigation and Modeling of Uranium (VI) Transport Under Variable Chemical Conditions journal, December 1996

Adsorption of Uranium(VI) and Zirconium(IV) from Acid Solutions on Silica Gel journal, October 1992

Reduction of U(VI) to U(IV) on the surface of magnetite journal, December 2005

Uraninite oxidation and dissolution induced by manganese oxide: A redox reaction between two insoluble minerals journal, January 2013

Microbial reduction of uranium journal, April 1991

Uranium solution-mineral equilibria at low temperatures with applications to sedimentary ore deposits journal, June 1978

Upscaling Sorption/Desorption Processes in Reactive Transport Models To Describe Metal/Radionuclide Transport: A Critical Review journal, November 2010

Comparison of Arsenic(V) and Arsenic(III) Sorption onto Iron Oxide Minerals: Implications for Arsenic Mobility journal, September 2003

Surface reactions kinetics between nanocrystalline magnetite and uranyl journal, May 2003

Standard states for the activities of mineral surface sites and species journal, January 2003

Eu(III) adsorption on rutile: Batch experiments and modeling journal, September 2010

Uranium(VI) Reduction by Iron(II) Monosulfide Mackinawite journal, February 2012

Uranium Transformations in Static Microcosms journal, January 2010

Heterogeneous reduction of U6+ by structural Fe2+ from theory and experiment journal, November 2011

Solution and Microbial Controls on the Formation of Reduced U(IV) Species journal, October 2011

U(VI) Sorption and Reduction by Fe(II) Sorbed on Montmorillonite journal, May 2010

Mass Action Expressions for Bidentate Adsorption in Surface Complexation Modeling: Theory and Practice journal, April 2013

UraniumVI Adsorption on Model Minerals: Controlling Factors and Surface Complexation Modeling book, January 1998

Identification of Simultaneous U(VI) Sorption Complexes and U(IV) Nanoprecipitates on the Magnetite (111) Surface journal, March 2012

Reaction of U VI with Titanium-Substituted Magnetite: Influence of Ti on U IV Speciation journal, April 2013

Uranium speciation and stability after reductive immobilization in aquifer sediments journal, November 2011

Non-uraninite Products of Microbial U(VI) Reduction journal, December 2010

Nano-FeS Inhibits UO 2 Reoxidation under Varied Oxic Conditions journal, December 2013

Biogeochemical Controls on the Product of Microbial U(VI) Reduction journal, October 2013

The product of microbial uranium reduction includes multiple species with U(IV)–phosphate coordination journal, April 2014

Relative Reactivity of Biogenic and Chemogenic Uraninite and Biogenic Noncrystalline U(IV) journal, August 2013

Uranium (VI) sorption on colloidal magnetite under anoxic environment: experimental study and surface complexation modelling journal, July 2003

Quantitative Separation of Monomeric U(IV) from UO 2 in Products of U(VI) Reduction journal, May 2012

Study of the solubility of amorphous and crystalline uranium dioxide by combined spectroscopic methods journal, January 2007

Abiotic reduction of uranium by Fe(II) in soil journal, August 2012

Influence of Magnetite Stoichiometry on U VI Reduction journal, December 2011

Adsorption characteristics of silver, lead, cadmium, zinc, and nickel on borosilicate glass, polyethylene, and polypropylene container surfaces journal, November 1973

Uranium redox transition pathways in acetate-amended sediments journal, March 2013

Abiotic Reductive Immobilization of U(VI) by Biogenic Mackinawite journal, February 2013

Characterization of uraninite nanoparticles produced by Shewanella oneidensis MR-1 journal, October 2008

Bioremediation of uranium-contaminated groundwater: a systems approach to subsurface biogeochemistry
journal, June 2013

Biogenic Uraninite Nanoparticles and Their Importance for Uranium Remediation
journal, December 2008

Influence of Dynamical Conditions on the Reduction of U ^VI at the Magnetite−Solution Interface
journal, January 2010

Additive Surface Complexation Modeling of Uranium(VI) Adsorption onto Quartz-Sand Dominated Sediments
journal, May 2014

Adsorption of Ions Dilute Aqueous Solutions on Glass and Plastic Surfaces.
journal, June 1965

Adsorption of Uranium(VI) to Manganese Oxides: X-ray Absorption Spectroscopy and Surface Complexation Modeling
journal, December 2012

Dissolution of synthetic brannerite in acidic and alkaline fluids
journal, September 2003

Kinetics of Uranium(VI) Reduction by Hydrogen Sulfide in Anoxic Aqueous Systems
journal, August 2006

Sorption of Th(IV) on MX-80 bentonite: effect of pH and modeling
journal, September 2010

U(VI) Reduction to Mononuclear U(IV) by Desulfitobacterium Species
journal, June 2010

Stable U(IV) Complexes Form at High-Affinity Mineral Surface Sites
journal, January 2014

Products of abiotic U(VI) reduction by biogenic magnetite and vivianite
journal, May 2011

Experimental Investigation and Modeling of Uranium (VI) Transport Under Variable Chemical Conditions
journal, December 1996

Adsorption of Uranium(VI) and Zirconium(IV) from Acid Solutions on Silica Gel
journal, October 1992

Reduction of U(VI) to U(IV) on the surface of magnetite
journal, December 2005

Uraninite oxidation and dissolution induced by manganese oxide: A redox reaction between two insoluble minerals
journal, January 2013

Microbial reduction of uranium
journal, April 1991

Uranium solution-mineral equilibria at low temperatures with applications to sedimentary ore deposits
journal, June 1978

Upscaling Sorption/Desorption Processes in Reactive Transport Models To Describe Metal/Radionuclide Transport: A Critical Review
journal, November 2010

Comparison of Arsenic(V) and Arsenic(III) Sorption onto Iron Oxide Minerals: Implications for Arsenic Mobility
journal, September 2003

Surface reactions kinetics between nanocrystalline magnetite and uranyl
journal, May 2003

Standard states for the activities of mineral surface sites and species
journal, January 2003

Eu(III) adsorption on rutile: Batch experiments and modeling
journal, September 2010

Uranium(VI) Reduction by Iron(II) Monosulfide Mackinawite
journal, February 2012

Uranium Transformations in Static Microcosms
journal, January 2010

Heterogeneous reduction of U6+ by structural Fe2+ from theory and experiment
journal, November 2011

Solution and Microbial Controls on the Formation of Reduced U(IV) Species
journal, October 2011

U(VI) Sorption and Reduction by Fe(II) Sorbed on Montmorillonite
journal, May 2010

Mass Action Expressions for Bidentate Adsorption in Surface Complexation Modeling: Theory and Practice
journal, April 2013

Uranium^VI Adsorption on Model Minerals: Controlling Factors and Surface Complexation Modeling
book, January 1998

Identification of Simultaneous U(VI) Sorption Complexes and U(IV) Nanoprecipitates on the Magnetite (111) Surface
journal, March 2012

Reaction of U ^VI with Titanium-Substituted Magnetite: Influence of Ti on U ^IV Speciation
journal, April 2013

Uranium speciation and stability after reductive immobilization in aquifer sediments
journal, November 2011

Non-uraninite Products of Microbial U(VI) Reduction
journal, December 2010

Nano-FeS Inhibits UO ₂ Reoxidation under Varied Oxic Conditions
journal, December 2013

Biogeochemical Controls on the Product of Microbial U(VI) Reduction
journal, October 2013

The product of microbial uranium reduction includes multiple species with U(IV)–phosphate coordination
journal, April 2014

Relative Reactivity of Biogenic and Chemogenic Uraninite and Biogenic Noncrystalline U(IV)
journal, August 2013

Uranium (VI) sorption on colloidal magnetite under anoxic environment: experimental study and surface complexation modelling
journal, July 2003

Quantitative Separation of Monomeric U(IV) from UO ₂ in Products of U(VI) Reduction
journal, May 2012

Study of the solubility of amorphous and crystalline uranium dioxide by combined spectroscopic methods
journal, January 2007

Abiotic reduction of uranium by Fe(II) in soil
journal, August 2012

Influence of Magnetite Stoichiometry on U ^VI Reduction
journal, December 2011

Adsorption characteristics of silver, lead, cadmium, zinc, and nickel on borosilicate glass, polyethylene, and polypropylene container surfaces
journal, November 1973

Uranium redox transition pathways in acetate-amended sediments
journal, March 2013

Abiotic Reductive Immobilization of U(VI) by Biogenic Mackinawite
journal, February 2013

Characterization of uraninite nanoparticles produced by Shewanella oneidensis MR-1
journal, October 2008