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Title: Stacked waveguide reactors with gradient embedded scatterers for high-capacity water cleaning

Abstract

We present a compact water-cleaning reactor with stacked layers of waveguides containing gradient patterns of optical scatterers that enable uniform light distribution and augmented water-cleaning rates. Previous photocatalytic reactors using immersion, external, or distributive lamps suffer from poor light distribution that impedes scalability. Here, we use an external UV-source to direct photons into stacked waveguide reactors where we scatter the photons uniformly over the length of the waveguide to thin films of TiO2-catalysts. In conclusion, we also show 4.5 times improvement in activity over uniform scatterer designs, demonstrate a degradation of 67% of the organic dye, and characterize the degradation rate constant.

Authors:
 [1];  [2];  [3]
  1. Cornell Univ., Ithaca, NY (United States). Applied and Engineering Physics
  2. Cornell Univ., Ithaca, NY (United States). Electrical and Computer Engineering
  3. Cornell Univ., Ithaca, NY (United States). Sibley School of Mechanical and Aerospace Engineering
Publication Date:
Research Org.:
Cornell Univ., Ithaca, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1240845
Grant/Contract Number:  
SC0003935
Resource Type:
Accepted Manuscript
Journal Name:
Optics Express
Additional Journal Information:
Journal Volume: 23; Journal Issue: 24; Journal ID: ISSN 1094-4087
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
42 ENGINEERING

Citation Formats

Ahsan, Syed Saad, Gumus, Abdurrahman, and Erickson, David. Stacked waveguide reactors with gradient embedded scatterers for high-capacity water cleaning. United States: N. p., 2015. Web. doi:10.1364/OE.23.0A1664.
Ahsan, Syed Saad, Gumus, Abdurrahman, & Erickson, David. Stacked waveguide reactors with gradient embedded scatterers for high-capacity water cleaning. United States. doi:10.1364/OE.23.0A1664.
Ahsan, Syed Saad, Gumus, Abdurrahman, and Erickson, David. Wed . "Stacked waveguide reactors with gradient embedded scatterers for high-capacity water cleaning". United States. doi:10.1364/OE.23.0A1664. https://www.osti.gov/servlets/purl/1240845.
@article{osti_1240845,
title = {Stacked waveguide reactors with gradient embedded scatterers for high-capacity water cleaning},
author = {Ahsan, Syed Saad and Gumus, Abdurrahman and Erickson, David},
abstractNote = {We present a compact water-cleaning reactor with stacked layers of waveguides containing gradient patterns of optical scatterers that enable uniform light distribution and augmented water-cleaning rates. Previous photocatalytic reactors using immersion, external, or distributive lamps suffer from poor light distribution that impedes scalability. Here, we use an external UV-source to direct photons into stacked waveguide reactors where we scatter the photons uniformly over the length of the waveguide to thin films of TiO2-catalysts. In conclusion, we also show 4.5 times improvement in activity over uniform scatterer designs, demonstrate a degradation of 67% of the organic dye, and characterize the degradation rate constant.},
doi = {10.1364/OE.23.0A1664},
journal = {Optics Express},
number = 24,
volume = 23,
place = {United States},
year = {2015},
month = {11}
}

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