Enhanced -Ray Emission from Neutron Unbound States Populated in Decay
Abstract
Total absorption spectroscopy was used to investigate the β -decay intensity to states above the neutron separation energy followed by γ -ray emission in 87,88Br and 94Rb. Accurate results were obtained thanks to the careful control of systematic errors. An unexpectedly large γ intensity was observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The γ branching as a function of excitation energy was compared to Hauser-Feshbach model calculations. For 87Br and 88Br the branching reaches 57% and 20% respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich 94Rb the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled introducing an enhancement of one order-of-magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proved to bemore »
- Authors:
-
more »
- Univ. of Valencia (Spain). Institute of Corpuscular Physics
- Univ. of Surrey, Guildford (United Kingdom). Dept. of Physics
- Univ. de Nantes, Nantes (France)
- Univ. of Jyvaskyla (Finland). Dept. of Physics
- Univ. of Helsinki (Finland). Helsinki Institute of Physics
- Petersburg Nuclear Physics Institute, Gatchina (Russia)
- Universitat Politecnica de Catalunya, Barcelona (Spain)
- Centre for Energy, Environment and Technology (CIEMAT), Madrid (Spain)
- Argonne National Lab. (ANL), Argonne, IL (United States). Nuclear Engineering Division
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1240585
- Alternate Identifier(s):
- OSTI ID: 1209177
- Report Number(s):
- BNL-108020-2015-JA
Journal ID: ISSN 0031-9007; PRLTAO; R&D Project: EST-003-NEFA; KB0301041
- Grant/Contract Number:
- SC00112704; AC02-06CH11357; FPA2008-06419; FPA2010-17142; FPA2011-24553
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Letters
- Additional Journal Information:
- Journal Volume: 115; Journal Issue: 6; Journal ID: ISSN 0031-9007
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 73 NUCLEAR PHYSICS AND RADIATION PHYSICS
Citation Formats
Tain, J. L., Valencia, E., Algora, A., Agramunt, J., Rubio, B., Rice, S., Gelletly, W., Regan, P., Zakari-Issoufou, A. -A., Fallot, M., Porta, A., Rissanen, J., Eronen, T., Äystö, J., Batist, L., Bowry, M., Bui, V. M., Caballero-Folch, R., Cano-Ott, D., Elomaa, V. -V., Estevez, E., Farrelly, G. F., Garcia, A. R., Gomez-Hornillos, B., Gorlychev, V., Hakala, J., Jordan, M. D., Jokinen, A., Kolhinen, V. S., Kondev, F. G., Martínez, T., Mendoza, E., Moore, I., Penttilä, H., Podolyák, Zs., Reponen, M., Sonnenschein, V., and Sonzogni, A. A. Enhanced γ -Ray Emission from Neutron Unbound States Populated in β Decay. United States: N. p., 2015.
Web. doi:10.1103/PhysRevLett.115.062502.
Tain, J. L., Valencia, E., Algora, A., Agramunt, J., Rubio, B., Rice, S., Gelletly, W., Regan, P., Zakari-Issoufou, A. -A., Fallot, M., Porta, A., Rissanen, J., Eronen, T., Äystö, J., Batist, L., Bowry, M., Bui, V. M., Caballero-Folch, R., Cano-Ott, D., Elomaa, V. -V., Estevez, E., Farrelly, G. F., Garcia, A. R., Gomez-Hornillos, B., Gorlychev, V., Hakala, J., Jordan, M. D., Jokinen, A., Kolhinen, V. S., Kondev, F. G., Martínez, T., Mendoza, E., Moore, I., Penttilä, H., Podolyák, Zs., Reponen, M., Sonnenschein, V., & Sonzogni, A. A. Enhanced γ -Ray Emission from Neutron Unbound States Populated in β Decay. United States. https://doi.org/10.1103/PhysRevLett.115.062502
Tain, J. L., Valencia, E., Algora, A., Agramunt, J., Rubio, B., Rice, S., Gelletly, W., Regan, P., Zakari-Issoufou, A. -A., Fallot, M., Porta, A., Rissanen, J., Eronen, T., Äystö, J., Batist, L., Bowry, M., Bui, V. M., Caballero-Folch, R., Cano-Ott, D., Elomaa, V. -V., Estevez, E., Farrelly, G. F., Garcia, A. R., Gomez-Hornillos, B., Gorlychev, V., Hakala, J., Jordan, M. D., Jokinen, A., Kolhinen, V. S., Kondev, F. G., Martínez, T., Mendoza, E., Moore, I., Penttilä, H., Podolyák, Zs., Reponen, M., Sonnenschein, V., and Sonzogni, A. A. Sat .
"Enhanced γ -Ray Emission from Neutron Unbound States Populated in β Decay". United States. https://doi.org/10.1103/PhysRevLett.115.062502. https://www.osti.gov/servlets/purl/1240585.
@article{osti_1240585,
title = {Enhanced γ -Ray Emission from Neutron Unbound States Populated in β Decay},
author = {Tain, J. L. and Valencia, E. and Algora, A. and Agramunt, J. and Rubio, B. and Rice, S. and Gelletly, W. and Regan, P. and Zakari-Issoufou, A. -A. and Fallot, M. and Porta, A. and Rissanen, J. and Eronen, T. and Äystö, J. and Batist, L. and Bowry, M. and Bui, V. M. and Caballero-Folch, R. and Cano-Ott, D. and Elomaa, V. -V. and Estevez, E. and Farrelly, G. F. and Garcia, A. R. and Gomez-Hornillos, B. and Gorlychev, V. and Hakala, J. and Jordan, M. D. and Jokinen, A. and Kolhinen, V. S. and Kondev, F. G. and Martínez, T. and Mendoza, E. and Moore, I. and Penttilä, H. and Podolyák, Zs. and Reponen, M. and Sonnenschein, V. and Sonzogni, A. A.},
abstractNote = {Total absorption spectroscopy was used to investigate the β -decay intensity to states above the neutron separation energy followed by γ -ray emission in 87,88Br and 94Rb. Accurate results were obtained thanks to the careful control of systematic errors. An unexpectedly large γ intensity was observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The γ branching as a function of excitation energy was compared to Hauser-Feshbach model calculations. For 87Br and 88Br the branching reaches 57% and 20% respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich 94Rb the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled introducing an enhancement of one order-of-magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proved to be correct, leads to a similar increase in the (n, γ) cross section that would have an impact on r process abundance calculations.},
doi = {10.1103/PhysRevLett.115.062502},
journal = {Physical Review Letters},
number = 6,
volume = 115,
place = {United States},
year = {Sat Aug 01 00:00:00 EDT 2015},
month = {Sat Aug 01 00:00:00 EDT 2015}
}
Web of Science
Works referenced in this record:
Gamma-ray emission in competition with neutron emission in the beta decay of 87Br
journal, January 1972
- Slaughter, D. R.; Nuh, F. M.; Shihab-Eldin, A. A.
- Physics Letters B, Vol. 38, Issue 1
Gamma-ray competition with neutron emission in the decay of 137I
journal, January 1975
- Nuh, F. M.; Slaughter, D. R.; Prussin, S. G.
- Physics Letters B, Vol. 53, Issue 5
Gamma-ray decay schemes for , , and
journal, March 1977
- Bischof, C. J.; Talbert, W. L.
- Physical Review C, Vol. 15, Issue 3
Investigation of beta strength functions by neutron and gamma-ray spectroscopy
journal, April 1979
- Kratz, K. -L.; Rudolph, W.; Ohm, H.
- Nuclear Physics A, Vol. 317, Issue 2-3
Decay of mass-separated to and systematics of isotones
journal, September 1982
- Yamamoto, H.; Wohn, F. K.; Sistemich, K.
- Physical Review C, Vol. 26, Issue 3
The beta-decay of95Rb and97Rb
journal, March 1983
- Kratz, K. -L.; Ohm, H.; Schr�der, A.
- Zeitschrift f�r Physik A Atoms and Nuclei, Vol. 312, Issue 1-2
decay of the ground state of studied with MeV and MeV purified radioactive beams
journal, November 2009
- Ilyushkin, S. V.; Winger, J. A.; Gross, C. J.
- Physical Review C, Vol. 80, Issue 5
-decay studies of the transitional nucleus and the structure of
journal, January 2011
- Ilyushkin, S. V.; Winger, J. A.; Rykaczewski, K. P.
- Physical Review C, Vol. 83, Issue 1
The essential decay of pandemonium: A demonstration of errors in complex beta-decay schemes
journal, November 1977
- Hardy, J. C.; Carraz, L. C.; Jonson, B.
- Physics Letters B, Vol. 71, Issue 2
Radiative neutron captures by neutron-rich nuclei and the r-process nucleosynthesis
journal, September 1998
- Goriely, S.
- Physics Letters B, Vol. 436, Issue 1-2
Changes in r -process abundances at late times
journal, August 2001
- Surman, R.; Engel, J.
- Physical Review C, Vol. 64, Issue 3
Dynamical -process studies within the neutrino-driven wind scenario and its sensitivity to the nuclear physics input
journal, April 2011
- Arcones, A.; Martínez-Pinedo, G.
- Physical Review C, Vol. 83, Issue 4
Astrophysical Reaction Rates From Statistical Model Calculations
journal, May 2000
- Rauscher, Thomas; Thielemann, Friedrich-Karl
- Atomic Data and Nuclear Data Tables, Vol. 75, Issue 1-2
The GT resonance revealed in β+-decay using new experimental techniques
journal, July 1999
- Algora, A.; Cano-Ott, D.; Rubio, B.
- Nuclear Physics A, Vol. 654, Issue 1
decay of : Evidence for the Gamow-Teller resonance near
journal, July 1999
- Hu, Z.; Batist, L.; Agramunt, J.
- Physical Review C, Vol. 60, Issue 2
High-energy γ-rays in 87Kr following the decay of 87Br
journal, November 1975
- Tovedal, H.; Fogelberg, B.
- Nuclear Physics A, Vol. 252, Issue 2
Delayed neutrons and high-energy γ-rays from decay of 87Br
journal, December 1977
- Nuh, F. M.; Slaughter, D. R.; Prussin, S. G.
- Nuclear Physics A, Vol. 293, Issue 3
Overlapping decay and resonance neutron spectroscopy of levels in
journal, August 1983
- Raman, S.; Fogelberg, B.; Harvey, J. A.
- Physical Review C, Vol. 28, Issue 2
Nuclear Data Sheets for A = 87
journal, March 2002
- Helmer, R. G.
- Nuclear Data Sheets, Vol. 95, Issue 3
Nuclear Data Sheets for A = 88
journal, January 2014
- McCutchan, E. A.; Sonzogni, A. A.
- Nuclear Data Sheets, Vol. 115
Nuclear Data Sheets for A = 94
journal, September 2006
- Abriola, D.; Sonzogni, A. A.
- Nuclear Data Sheets, Vol. 107, Issue 9
Development and applications of the IGISOL technique
journal, October 2001
- Äystö, Juha
- Nuclear Physics A, Vol. 693, Issue 1-2
JYFLTRAP: a cylindrical Penning trap for isobaric beam purification at IGISOL
journal, August 2004
- Kolhinen, V. S.; Kopecky, S.; Eronen, T.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 528, Issue 3
JYFLTRAP: a Penning trap for precision mass spectroscopy and isobaric purification
journal, April 2012
- Eronen, T.; Kolhinen, V. S.; Elomaa, V. -V.
- The European Physical Journal A, Vol. 48, Issue 4
Geant4—a simulation toolkit
journal, July 2003
- Agostinelli, S.; Allison, J.; Amako, K.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 506, Issue 3
ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data
journal, December 2011
- Chadwick, M. B.; Herman, M.; Obložinský, P.
- Nuclear Data Sheets, Vol. 112, Issue 12
The sensitivity of LaBr3:Ce scintillation detectors to low energy neutrons: Measurement and Monte Carlo simulation
journal, February 2015
- Tain, J. L.; Agramunt, J.; Algora, A.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 774
Pulse pileup correction of large NaI(Tl) total absorption spectra using the true pulse shape
journal, July 1999
- Cano-Ott, D.; Tain, J. L.; Gadea, A.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 430, Issue 2-3
New Beta-delayed Neutron Measurements in the Light-mass Fission Group
journal, June 2014
- Agramunt, J.; García, A. R.; Algora, A.
- Nuclear Data Sheets, Vol. 120
The influence of the unknown de-excitation pattern in the analysis of -decay total absorption spectra
journal, February 2007
- Tain, J. L.; Cano-Ott, D.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 571, Issue 3
Algorithms for the analysis of -decay total absorption spectra
journal, February 2007
- Tain, J. L.; Cano-Ott, D.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 571, Issue 3
Improved microscopic nuclear level densities within the Hartree-Fock-Bogoliubov plus combinatorial method
journal, December 2008
- Goriely, S.; Hilaire, S.; Koning, A. J.
- Physical Review C, Vol. 78, Issue 6
RIPL – Reference Input Parameter Library for Calculation of Nuclear Reactions and Nuclear Data Evaluations
journal, December 2009
- Capote, R.; Herman, M.; Obložinský, P.
- Nuclear Data Sheets, Vol. 110, Issue 12
Reactor Decay Heat in : Solving the Discrepancy in the 4–3000-s Cooling Period
journal, November 2010
- Algora, A.; Jordan, D.; Taín, J. L.
- Physical Review Letters, Vol. 105, Issue 20
New Antineutrino Energy Spectra Predictions from the Summation of Beta Decay Branches of the Fission Products
journal, November 2012
- Fallot, M.; Cormon, S.; Estienne, M.
- Physical Review Letters, Vol. 109, Issue 20
Local and global nucleon optical models from 1 keV to 200 MeV
journal, January 2003
- Koning, A. J.; Delaroche, J. P.
- Nuclear Physics A, Vol. 713, Issue 3-4
Works referencing / citing this record:
Total Absorption Spectroscopy
journal, April 2018
- Algora, A.; Rubio, B.; Tain, J. L.
- Nuclear Physics News, Vol. 28, Issue 2