Origin of modulated phases and magnetic hysteresis in TmB4

Wierschem, Keola; Sunku, Sai Swaroop; Kong, Tai; Ito, Toshimitsu; Canfield, Paul C.; Panagopoulos, Christos; Sengupta, Pinaki

doi:10.1103/PhysRevB.92.214433

Title: Origin of modulated phases and magnetic hysteresis in TmB₄

Abstract

In this study, we investigate the low-temperature magnetic phases in TmB₄, a metallic quantum magnet on the geometrically frustrated Shastry-Sutherland lattice, using coordinated experimental and theoretical studies. Our results provide an explanation for the appearance of the intriguing fractional plateau in TmB₄ and accompanying magnetic hysteresis. Together with observation of the bump in the half plateau, our results support the picture that the magnetization plateau structure in TmB₄ is strongly influenced by the zero-field modulated phases. We present a phenomenological model to explain the appearance of the modulated phases and a microscopic Hamiltonian that captures the complete magnetic behavior of TmB₄.

Authors:

Wierschem, Keola ^[1]; Sunku, Sai Swaroop ^[1]; Kong, Tai ^[2]; Ito, Toshimitsu ^[3]; Canfield, Paul C. ^[2]; Panagopoulos, Christos ^[1]; Sengupta, Pinaki ^[1]

Nanyang Technological Univ. (Singapore)
Iowa State Univ., Ames, IA (United States)
National Institute of Advanced Industrial Science and Technology (AIST), Ibaraki (Japan)

Publication Date:: Wed Dec 23 00:00:00 EST 2015

Research Org.:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1239160

Alternate Identifier(s):: OSTI ID: 1233890

Report Number(s):: IS-J-8906
Journal ID: ISSN 1098-0121; PRBMDO

Grant/Contract Number:: AC02-07CH11358

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Volume: 92; Journal Issue: 21; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Wierschem, Keola, Sunku, Sai Swaroop, Kong, Tai, Ito, Toshimitsu, Canfield, Paul C., Panagopoulos, Christos, and Sengupta, Pinaki. Origin of modulated phases and magnetic hysteresis in TmB4.  United States: N. p., 2015. 
Web.  doi:10.1103/PhysRevB.92.214433.

Copy to clipboard


                    Wierschem, Keola, Sunku, Sai Swaroop, Kong, Tai, Ito, Toshimitsu, Canfield, Paul C., Panagopoulos, Christos, & Sengupta, Pinaki. Origin of modulated phases and magnetic hysteresis in TmB4.  United States.  https://doi.org/10.1103/PhysRevB.92.214433

Copy to clipboard


                    Wierschem, Keola, Sunku, Sai Swaroop, Kong, Tai, Ito, Toshimitsu, Canfield, Paul C., Panagopoulos, Christos, and Sengupta, Pinaki. Wed .  
"Origin of modulated phases and magnetic hysteresis in TmB4".  United States.  https://doi.org/10.1103/PhysRevB.92.214433.  https://www.osti.gov/servlets/purl/1239160.

Copy to clipboard


                    
@article{osti_1239160,

  title        = {Origin of modulated phases and magnetic hysteresis in TmB4},

  author       = {Wierschem, Keola and Sunku, Sai Swaroop and Kong, Tai and Ito, Toshimitsu and Canfield, Paul C. and Panagopoulos, Christos and Sengupta, Pinaki},

  abstractNote = {In this study, we investigate the low-temperature magnetic phases in TmB4, a metallic quantum magnet on the geometrically frustrated Shastry-Sutherland lattice, using coordinated experimental and theoretical studies. Our results provide an explanation for the appearance of the intriguing fractional plateau in TmB4 and accompanying magnetic hysteresis. Together with observation of the bump in the half plateau, our results support the picture that the magnetization plateau structure in TmB4 is strongly influenced by the zero-field modulated phases. We present a phenomenological model to explain the appearance of the modulated phases and a microscopic Hamiltonian that captures the complete magnetic behavior of TmB4.},

  doi          = {10.1103/PhysRevB.92.214433},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 21,

  volume       = 92,

  place        = {United States},

  year         = {Wed Dec 23 00:00:00 EST 2015},

  month        = {Wed Dec 23 00:00:00 EST 2015}

}

Copy to clipboard

Journal Article:

Free Publicly Available Full Text

Accepted Manuscript (Publisher)

Accepted Manuscript (DOE)

Publisher's Version of Record

https://doi.org/10.1103/PhysRevB.92.214433

Other availability

Search WorldCat to find libraries that may hold this journal

Citation Metrics:

Cited by: 20 works

Citation information provided by
Web of Science

Save / Share:

Export Metadata

Save to My Library

Works referenced in this record:

Spin liquids in frustrated magnets
journal, March 2010

Balents, Leon
Nature, Vol. 464, Issue 7286
DOI: 10.1038/nature08917

Introduction to Frustrated Magnetism
book, January 2011

Lacroix, Claudine; Mendels, Philippe; Mila, Frédéric
Springer Series in Solid-State Sciences
DOI: 10.1007/978-3-642-10589-0

Exact Dimer Ground State and Quantized Magnetization Plateaus in the Two-Dimensional Spin System ${SrCu}_{2} ({BO}_{3})_{2}$
journal, April 1999

Kageyama, H.; Yoshimura, K.; Stern, R.
Physical Review Letters, Vol. 82, Issue 15
DOI: 10.1103/PhysRevLett.82.3168

Magnetic Superstructure in the Two-Dimensional Quantum Antiferromagnet SrCu2(BO3)2
journal, October 2002

Kodama, K.
Science, Vol. 298, Issue 5592
DOI: 10.1126/science.1075045

Fractalization drives crystalline states in a frustrated spin system
journal, December 2008

Sebastian, S. E.; Harrison, N.; Sengupta, P.
Proceedings of the National Academy of Sciences, Vol. 105, Issue 51
DOI: 10.1073/pnas.0804320105

Incomplete Devil’s Staircase in the Magnetization Curve of ${SrCu}_{2} ({BO}_{3})_{2}$
journal, February 2013

Takigawa, M.; Horvatić, M.; Waki, T.
Physical Review Letters, Vol. 110, Issue 6
DOI: 10.1103/PhysRevLett.110.067210

Magnetic Structure and Phase Diagram of TmB ₄
journal, January 2008

Gabáni, S.; Maťaš, S.; Priputen, P.
Acta Physica Polonica A, Vol. 113, Issue 1
DOI: 10.12693/APhysPolA.113.227

Highly anisotropic magnetic phase diagram of a 2-dimensional orthogonal dimer system TmB4
journal, March 2007

Iga, F.; Shigekawa, A.; Hasegawa, Y.
Journal of Magnetism and Magnetic Materials, Vol. 310, Issue 2
DOI: 10.1016/j.jmmm.2006.10.476

Fractional Magnetization Plateaus and Magnetic Order in the Shastry-Sutherland Magnet ${TmB}_{4}$
journal, October 2008

Siemensmeyer, K.; Wulf, E.; Mikeska, H. -J.
Physical Review Letters, Vol. 101, Issue 17
DOI: 10.1103/PhysRevLett.101.177201

Complex Magnetic Structures of a Shastry–Sutherland Lattice TmB ₄ Studied by Powder Neutron Diffraction Analysis
journal, February 2009

Michimura, Shinji; Shigekawa, Akira; Iga, Fumitoshi
Journal of the Physical Society of Japan, Vol. 78, Issue 2
DOI: 10.1143/JPSJ.78.024707

Anisotropy and metamagnetism in the RNi2Ge2 (R=Y, La–Nd, Sm–Lu) series
journal, October 1999

Bud'ko, S. L.; Islam, Z.; Wiener, T. A.
Journal of Magnetism and Magnetic Materials, Vol. 205, Issue 1
DOI: 10.1016/S0304-8853(99)00486-2

Systematic study of anisotropic transport and magnetic properties of RAgSb2 (R=Y, La–Nd, Sm, Gd–Tm)
journal, October 1999

Myers, K. D.; Bud'ko, S. L.; Fisher, I. R.
Journal of Magnetism and Magnetic Materials, Vol. 205, Issue 1
DOI: 10.1016/S0304-8853(99)00472-2

Angular dependence of metamagnetic transitions in ${DyAgSb}_{2}$
journal, January 1999

Myers, K. D.; Canfield, P. C.; Kalatsky, V. A.
Physical Review B, Vol. 59, Issue 2
DOI: 10.1103/PhysRevB.59.1121

Angular dependence of metamagnetic transitions in ${HoNi}_{2}$ $B_{2}$ C
journal, January 1997

Canfield, P. C.; Bud'ko, S. L.; Cho, B. K.
Physical Review B, Vol. 55, Issue 2
DOI: 10.1103/PhysRevB.55.970

Magnetic properties of the spin- $\frac{1}{2}$ XXZ model on the Shastry-Sutherland lattice: Effect of long-range interactions
journal, November 2009

Suzuki, Takahumi; Tomita, Yusuke; Kawashima, Naoki
Physical Review B, Vol. 80, Issue 18
DOI: 10.1103/PhysRevB.80.180405

Monte Carlo Study of the Axial Next-Nearest-Neighbor Ising Model
journal, May 2010

Zhang, Kai; Charbonneau, Patrick
Physical Review Letters, Vol. 104, Issue 19
DOI: 10.1103/PhysRevLett.104.195703

Finite-temperature phase transition to the $m = \frac{1}{2}$ plateau phase in the spin- $\frac{1}{2}$ $X X Z$ model on the Shastry-Sutherland lattices
journal, December 2010

Suzuki, T.; Tomita, Y.; Kawashima, N.
Physical Review B, Vol. 82, Issue 21
DOI: 10.1103/PhysRevB.82.214404

Phases and magnetization process of an anisotropic Shastry-Sutherland model
journal, December 2008

Meng, Zi Yang; Wessel, Stefan
Physical Review B, Vol. 78, Issue 22
DOI: 10.1103/PhysRevB.78.224416

Magnetization plateau of the classical Ising model on the Shastry-Sutherland lattice: A tensor renormalization-group approach
journal, March 2009

Chang, Ming-Che; Yang, Min-Fong
Physical Review B, Vol. 79, Issue 10
DOI: 10.1103/PhysRevB.79.104411

Ground States of the Ising Model on the Shastry-Sutherland Lattice and the Origin of the Fractional Magnetization Plateaus in Rare-Earth-Metal Tetraborides
journal, October 2012

Dublenych, Yu. I.
Physical Review Letters, Vol. 109, Issue 16
DOI: 10.1103/PhysRevLett.109.167202

Dynamic magnetization process in the frustrated Shastry-Sutherland system TmB ₄
journal, May 2013

Huang, W. C.; Huo, L.; Feng, J. J.
EPL (Europhysics Letters), Vol. 102, Issue 3
DOI: 10.1209/0295-5075/102/37005

Columnar Antiferromagnetic Order and Spin Supersolid Phase on the Extended Shastry-Sutherland Lattice
journal, May 2013

Wierschem, Keola; Sengupta, Pinaki
Physical Review Letters, Vol. 110, Issue 20
DOI: 10.1103/PhysRevLett.110.207207

Rare-earth–boron bonding and 4f state trends in $R B_{4}$ tetraborides
journal, January 2008

Yin, Z. P.; Pickett, W. E.
Physical Review B, Vol. 77, Issue 3
DOI: 10.1103/PhysRevB.77.035135

Works referencing / citing this record:

Rotating magnetocaloric effect and unusual magnetic features in metallic strongly anisotropic geometrically frustrated TmB4
journal, July 2018

Orendáč, Matúš; Gabáni, Slavomír; Gažo, Emil
Scientific Reports, Vol. 8, Issue 1
DOI: 10.1038/s41598-018-29399-2

Similar Records in DOE PAGES and OSTI.GOV collections:

Hysteretic magnetoresistance and unconventional anomalous Hall effect in the frustrated magnet TmB₄

Journal Article Sunku, Sai Swaroop ; Kong, Tai ; Ito, Toshimitsu ; ... - Physical Review B

We study TmB₄, a frustrated magnet on the Archimedean Shastry-Sutherland lattice, through magnetization and transport experiments. The lack of anisotropy in resistivity shows that TmB4 is an electronically three-dimensional system. The magnetoresistance (MR) is hysteretic at low temperature even though a corresponding hysteresis in magnetization is absent. The Hall resistivity shows unconventional anomalous Hall effect (AHE) and is linear above saturation despite a large MR. In conclusion, we propose that complex structures at magnetic domain walls may be responsible for the hysteretic MR and may also lead to the AHE.
Cited by 22
https://doi.org/10.1103/PhysRevB.93.174408

Full Text Available
Degeneracy of the 1/8 Plateau and Antiferromagnetic Phases in the Shastry-Sutherland Magnet TmB₄

Journal Article Trinh, Jennifer ; Mitra, Sreemanta ; Panagopoulos, Christos ; ... - Physical Review Letters

The 1/8 fractional plateau phase (1/8 FPP) in Shastry-Sutherland lattice (SSL) spin systems has been viewed an exemplar of emergence on an Archimedean lattice. Here we explore this phase in the Ising magnet TmB₄ using high-resolution specific heat (C) and magnetization (M) in the field-temperature plane. We show that the 1/8 FPP is smoothly connected to the antiferromagnetic phase on ramping the field from H = 0. Furthermore, the 1/8 FPP is not a distinct thermodynamic ground state of TmB₄. The implication of these results for Heisenberg spins on the SSL is discussed.
Cited by 16
https://doi.org/10.1103/physrevlett.121.167203

Full Text Available
Simulating the Shastry-Sutherland Ising Model Using Quantum Annealing

Journal Article Kairys, Paul ; King, Andrew D. ; Ozfidan, Isil ; ... - PRX Quantum

A core concept in condensed matter physics is geometric frustration that leads to emergent spin phases in magnetic materials. These distinct phases, which depart from the conventional ferromagnet or the antiferromagnet, require unique computational techniques to decipher. In this study, we use the canonical Ising Shastry-Sutherland lattice to demonstrate new techniques for solving frustrated Hamiltonians using a quantum annealer of programmable superconducting qubits. This Hamiltonian can be tuned to produce a variety of intriguing ground states ranging from short- and long-range orders and fractional order parameters. We show that a large-scale finite-field quantum annealing experiment is possible on 468 logicalmore »« less
https://doi.org/10.1103/prxquantum.1.020320
Discovery of quantum phases in the Shastry-Sutherland compound SrCu₂(BO₃)₂ under extreme conditions of field and pressure

Journal Article Shi, Zhenzhong ; Dissanayake, Sachith ; Corboz, Philippe ; ... - Nature Communications

The 2-dimensional layered oxide material SrCu₂(BO₃)₂, long studied as a realization of the Shastry-Sutherland spin topology, exhibits a range of intriguing physics as a function of both hydrostatic pressure and magnetic field, with a still debated intermediate plaquette phase appearing at approximately 20 kbar and a possible deconfined critical point at higher pressure. Here, we employ a tunnel diode oscillator (TDO) technique to probe the behavior in the combined extreme conditions of high pressure, high magnetic field, and low temperature. We reveal an extensive phase space consisting of multiple magnetic analogs of the elusive supersolid phase and a magnetization plateau.more »« less
https://doi.org/10.1038/s41467-022-30036-w

Full Text Available
Magnetization Plateaus of SrCu{sub 2}(BO{sub 3}){sub 2} from a Chern-Simons Theory

Journal Article Misguich, G ; Jolicoeur, Th ; Girvin, S M - Physical Review Letters

The antiferromagnetic Heisenberg model on the frustrated Shastry-Sutherland lattice is studied by a mapping onto spinless fermions carrying one quantum of statistical flux. Using a mean-field approximation these fermions populate the bands of a generalized Hofstadter problem. Their filling leads to the magnetization curve. For SrCu{sub 2}(BO{sub 3}){sub 2} we reproduce plateaus at 1/3 and 1/4 of the saturation moment and predict a new one at 1/2 . Gaussian fluctuations of the gauge field are shown to be massive at these plateau values.
https://doi.org/10.1103/PhysRevLett.87.097203

Similar Records

Title: Origin of modulated phases and magnetic hysteresis in TmB4

Abstract

Citation Formats

Spin liquids in frustrated magnets journal, March 2010

Introduction to Frustrated Magnetism book, January 2011

Exact Dimer Ground State and Quantized Magnetization Plateaus in the Two-Dimensional Spin System SrCu 2 ( BO 3 ) 2 journal, April 1999

Magnetic Superstructure in the Two-Dimensional Quantum Antiferromagnet SrCu2(BO3)2 journal, October 2002

Fractalization drives crystalline states in a frustrated spin system journal, December 2008

Incomplete Devil’s Staircase in the Magnetization Curve of SrCu 2 ( BO 3 ) 2 journal, February 2013

Magnetic Structure and Phase Diagram of TmB 4 journal, January 2008

Highly anisotropic magnetic phase diagram of a 2-dimensional orthogonal dimer system TmB4 journal, March 2007

Fractional Magnetization Plateaus and Magnetic Order in the Shastry-Sutherland Magnet TmB 4 journal, October 2008

Complex Magnetic Structures of a Shastry–Sutherland Lattice TmB 4 Studied by Powder Neutron Diffraction Analysis journal, February 2009

Anisotropy and metamagnetism in the RNi2Ge2 (R=Y, La–Nd, Sm–Lu) series journal, October 1999

Systematic study of anisotropic transport and magnetic properties of RAgSb2 (R=Y, La–Nd, Sm, Gd–Tm) journal, October 1999

Angular dependence of metamagnetic transitions in DyAgSb 2 journal, January 1999

Angular dependence of metamagnetic transitions in HoNi 2 B 2 C journal, January 1997

Magnetic properties of the spin- 1 2 XXZ model on the Shastry-Sutherland lattice: Effect of long-range interactions journal, November 2009

Monte Carlo Study of the Axial Next-Nearest-Neighbor Ising Model journal, May 2010

Finite-temperature phase transition to the m = 1 2 plateau phase in the spin- 1 2 X X Z model on the Shastry-Sutherland lattices journal, December 2010

Phases and magnetization process of an anisotropic Shastry-Sutherland model journal, December 2008

Magnetization plateau of the classical Ising model on the Shastry-Sutherland lattice: A tensor renormalization-group approach journal, March 2009

Ground States of the Ising Model on the Shastry-Sutherland Lattice and the Origin of the Fractional Magnetization Plateaus in Rare-Earth-Metal Tetraborides journal, October 2012

Dynamic magnetization process in the frustrated Shastry-Sutherland system TmB 4 journal, May 2013

Columnar Antiferromagnetic Order and Spin Supersolid Phase on the Extended Shastry-Sutherland Lattice journal, May 2013

Rare-earth–boron bonding and 4f state trends in R B 4 tetraborides journal, January 2008

Rotating magnetocaloric effect and unusual magnetic features in metallic strongly anisotropic geometrically frustrated TmB4 journal, July 2018

Title: Origin of modulated phases and magnetic hysteresis in TmB₄

Spin liquids in frustrated magnets
journal, March 2010

Introduction to Frustrated Magnetism
book, January 2011

Exact Dimer Ground State and Quantized Magnetization Plateaus in the Two-Dimensional Spin System ${SrCu}_{2} ({BO}_{3})_{2}$
journal, April 1999

Magnetic Superstructure in the Two-Dimensional Quantum Antiferromagnet SrCu2(BO3)2
journal, October 2002

Fractalization drives crystalline states in a frustrated spin system
journal, December 2008

Incomplete Devil’s Staircase in the Magnetization Curve of ${SrCu}_{2} ({BO}_{3})_{2}$
journal, February 2013

Magnetic Structure and Phase Diagram of TmB ₄
journal, January 2008

Highly anisotropic magnetic phase diagram of a 2-dimensional orthogonal dimer system TmB4
journal, March 2007

Fractional Magnetization Plateaus and Magnetic Order in the Shastry-Sutherland Magnet ${TmB}_{4}$
journal, October 2008

Complex Magnetic Structures of a Shastry–Sutherland Lattice TmB ₄ Studied by Powder Neutron Diffraction Analysis
journal, February 2009

Anisotropy and metamagnetism in the RNi2Ge2 (R=Y, La–Nd, Sm–Lu) series
journal, October 1999

Systematic study of anisotropic transport and magnetic properties of RAgSb2 (R=Y, La–Nd, Sm, Gd–Tm)
journal, October 1999

Angular dependence of metamagnetic transitions in ${DyAgSb}_{2}$
journal, January 1999

Angular dependence of metamagnetic transitions in ${HoNi}_{2}$ $B_{2}$ C
journal, January 1997

Magnetic properties of the spin- $\frac{1}{2}$ XXZ model on the Shastry-Sutherland lattice: Effect of long-range interactions
journal, November 2009

Monte Carlo Study of the Axial Next-Nearest-Neighbor Ising Model
journal, May 2010

Finite-temperature phase transition to the $m = \frac{1}{2}$ plateau phase in the spin- $\frac{1}{2}$ $X X Z$ model on the Shastry-Sutherland lattices
journal, December 2010

Phases and magnetization process of an anisotropic Shastry-Sutherland model
journal, December 2008

Magnetization plateau of the classical Ising model on the Shastry-Sutherland lattice: A tensor renormalization-group approach
journal, March 2009

Ground States of the Ising Model on the Shastry-Sutherland Lattice and the Origin of the Fractional Magnetization Plateaus in Rare-Earth-Metal Tetraborides
journal, October 2012

Dynamic magnetization process in the frustrated Shastry-Sutherland system TmB ₄
journal, May 2013

Columnar Antiferromagnetic Order and Spin Supersolid Phase on the Extended Shastry-Sutherland Lattice
journal, May 2013

Rare-earth–boron bonding and 4f state trends in $R B_{4}$ tetraborides
journal, January 2008

Rotating magnetocaloric effect and unusual magnetic features in metallic strongly anisotropic geometrically frustrated TmB4
journal, July 2018