DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Observation of femtosecond molecular dynamics via pump–probe gas phase x-ray scattering

Authors:
; ; ; ; ; ;
Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1238868
Grant/Contract Number:  
AC02-76SF00515
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Journal of Physics. B, Atomic, Molecular and Optical Physics
Additional Journal Information:
Journal Name: Journal of Physics. B, Atomic, Molecular and Optical Physics Journal Volume: 49 Journal Issue: 3; Journal ID: ISSN 0953-4075
Publisher:
IOP Publishing
Country of Publication:
United Kingdom
Language:
English

Citation Formats

Budarz, J. M., Minitti, M. P., Cofer-Shabica, D. V., Stankus, B., Kirrander, A., Hastings, J. B., and Weber, P. M. Observation of femtosecond molecular dynamics via pump–probe gas phase x-ray scattering. United Kingdom: N. p., 2016. Web. doi:10.1088/0953-4075/49/3/034001.
Budarz, J. M., Minitti, M. P., Cofer-Shabica, D. V., Stankus, B., Kirrander, A., Hastings, J. B., & Weber, P. M. Observation of femtosecond molecular dynamics via pump–probe gas phase x-ray scattering. United Kingdom. https://doi.org/10.1088/0953-4075/49/3/034001
Budarz, J. M., Minitti, M. P., Cofer-Shabica, D. V., Stankus, B., Kirrander, A., Hastings, J. B., and Weber, P. M. Fri . "Observation of femtosecond molecular dynamics via pump–probe gas phase x-ray scattering". United Kingdom. https://doi.org/10.1088/0953-4075/49/3/034001.
@article{osti_1238868,
title = {Observation of femtosecond molecular dynamics via pump–probe gas phase x-ray scattering},
author = {Budarz, J. M. and Minitti, M. P. and Cofer-Shabica, D. V. and Stankus, B. and Kirrander, A. and Hastings, J. B. and Weber, P. M.},
abstractNote = {},
doi = {10.1088/0953-4075/49/3/034001},
journal = {Journal of Physics. B, Atomic, Molecular and Optical Physics},
number = 3,
volume = 49,
place = {United Kingdom},
year = {Fri Jan 08 00:00:00 EST 2016},
month = {Fri Jan 08 00:00:00 EST 2016}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1088/0953-4075/49/3/034001

Citation Metrics:
Cited by: 49 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Single mimivirus particles intercepted and imaged with an X-ray laser
journal, February 2011

  • Seibert, M. Marvin; Ekeberg, Tomas; Maia, Filipe R. N. C.
  • Nature, Vol. 470, Issue 7332
  • DOI: 10.1038/nature09748

Ultrafast Diffraction Imaging of the Electrocyclic Ring-Opening Reaction of 1,3-Cyclohexadiene
journal, May 2001

  • Dudek, Ray C.; Weber, Peter M.
  • The Journal of Physical Chemistry A, Vol. 105, Issue 17
  • DOI: 10.1021/jp010122t

Femtosecond real‐time probing of reactions. II. The dissociation reaction of ICN
journal, November 1988

  • Dantus, Marcos; Rosker, Mark J.; Zewail, Ahmed H.
  • The Journal of Chemical Physics, Vol. 89, Issue 10, p. 6128-6140
  • DOI: 10.1063/1.455428

Crystal structure of rhodopsin bound to arrestin by femtosecond X-ray laser
journal, July 2015

  • Kang, Yanyong; Zhou, X. Edward; Gao, Xiang
  • Nature, Vol. 523, Issue 7562
  • DOI: 10.1038/nature14656

Theory of time-resolved inelastic x-ray diffraction
journal, February 2010


From the (1B) Spectroscopic State to the Photochemical Product of the Ultrafast Ring-Opening of 1,3-Cyclohexadiene: A Spectral Observation of the Complete Reaction Path
journal, August 2015

  • Pemberton, Christine C.; Zhang, Yao; Saita, Kenichiro
  • The Journal of Physical Chemistry A, Vol. 119, Issue 33
  • DOI: 10.1021/acs.jpca.5b05672

Optical laser systems at the Linac Coherent Light Source
journal, April 2015

  • Minitti, Michael P.; Robinson, Joseph S.; Coffee, Ryan N.
  • Journal of Synchrotron Radiation, Vol. 22, Issue 3
  • DOI: 10.1107/S1600577515006244

Zerstreuung von Röntgenstrahlen
journal, January 1915


Femtochemistry:  Recent Progress in Studies of Dynamics and Control of Reactions and Their Transition States
journal, January 1996

  • Zewail, Ahmed H.
  • The Journal of Physical Chemistry, Vol. 100, Issue 31
  • DOI: 10.1021/jp960658s

Femtosecond X-ray protein nanocrystallography
journal, February 2011

  • Chapman, Henry N.; Fromme, Petra; Barty, Anton
  • Nature, Vol. 470, Issue 7332, p. 73-77
  • DOI: 10.1038/nature09750

Ultrafast Structural Pathway of Charge Transfer in N , N , N ′, N ′-Tetramethylethylenediamine
journal, March 2015

  • Cheng, Xinxin; Zhang, Yao; Gao, Yan
  • The Journal of Physical Chemistry A, Vol. 119, Issue 12
  • DOI: 10.1021/acs.jpca.5b01797

Ultrafast X-ray Diffraction Theory
journal, November 1998

  • Cao, Jianshu; Wilson, Kent R.
  • The Journal of Physical Chemistry A, Vol. 102, Issue 47
  • DOI: 10.1021/jp982054p

Time-Resolved Molecular Frame Dynamics of Fixed-in-Space CS2 Molecules
journal, March 2009


Observation of restricted IVR in large molecules: Quasi-periodic behavior, phase-shifted and non-phase-shifted quantum beats
journal, November 1983


The Formation of Warm Dense Matter: Experimental Evidence for Electronic Bond Hardening in Gold
journal, February 2009


Femtosecond Multidimensional Imaging of a Molecular Dissociation
journal, January 2006


X-ray detectors at the Linac Coherent Light Source
journal, April 2015

  • Blaj, Gabriel; Caragiulo, Pietro; Carini, Gabriella
  • Journal of Synchrotron Radiation, Vol. 22, Issue 3
  • DOI: 10.1107/S1600577515005317

Far-UV Photochemical Bond Cleavage of n -Amyl Nitrite: Bypassing a Repulsive Surface
journal, January 2012

  • Minitti, Michael P.; Zhang, Yao; Rosenberg, Martin
  • The Journal of Physical Chemistry A, Vol. 116, Issue 2
  • DOI: 10.1021/jp209727g

Reaction Path of a sub-200 fs Photochemical Electrocyclic Reaction
journal, May 2001

  • Garavelli, M.; Page, C. S.; Celani, P.
  • The Journal of Physical Chemistry A, Vol. 105, Issue 18
  • DOI: 10.1021/jp010359p

Direct Imaging of Transient Molecular Structures with Ultrafast Diffraction
journal, January 2001


Ultrafast electron optics: Propagation dynamics of femtosecond electron packets
journal, August 2002

  • Siwick, Bradley J.; Dwyer, Jason R.; Jordan, Robert E.
  • Journal of Applied Physics, Vol. 92, Issue 3
  • DOI: 10.1063/1.1487437

Ultrafast X-ray Diffraction of Transient Molecular Structures in Solution
journal, August 2005


An Atomic-Level View of Melting Using Femtosecond Electron Diffraction
journal, November 2003

  • Siwick, Bradley J.; Dwyer, Jason R.; Jordan, Robert E.
  • Science, Vol. 302, Issue 5649
  • DOI: 10.1126/science.1090052

Imaging Molecular Motion: Femtosecond X-Ray Scattering of an Electrocyclic Chemical Reaction
journal, June 2015


Spectral encoding method for measuring the relative arrival time between x-ray/optical pulses
journal, August 2014

  • Bionta, M. R.; Hartmann, N.; Weaver, M.
  • Review of Scientific Instruments, Vol. 85, Issue 8
  • DOI: 10.1063/1.4893657

Selforganization of matter and the evolution of biological macromolecules
journal, October 1971


Pixel array detector for X-ray free electron laser experiments
journal, September 2011

  • Philipp, Hugh T.; Hromalik, Marianne; Tate, Mark
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 649, Issue 1
  • DOI: 10.1016/j.nima.2010.11.189

Ultrafast structural dynamics with table top femtosecond hard X-ray and electron diffraction setups
journal, July 2013


Single-electron pulses for ultrafast diffraction
journal, November 2010

  • Aidelsburger, M.; Kirchner, F. O.; Krausz, F.
  • Proceedings of the National Academy of Sciences, Vol. 107, Issue 46
  • DOI: 10.1073/pnas.1010165107

The Ultrafast Pathway of Photon-Induced Electrocyclic Ring-Opening Reactions: The Case of 1,3-Cyclohexadiene
journal, May 2011


First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010


De novo protein crystal structure determination from X-ray free-electron laser data
journal, November 2013

  • Barends, Thomas R. M.; Foucar, Lutz; Botha, Sabine
  • Nature, Vol. 505, Issue 7482
  • DOI: 10.1038/nature12773

Ultrafast diffraction and structural dynamics: The nature of complex molecules far from equilibrium
journal, June 2001

  • Ruan, C. -Y.; Lobastov, V. A.; Srinivasan, R.
  • Proceedings of the National Academy of Sciences, Vol. 98, Issue 13
  • DOI: 10.1073/pnas.131192898

Energy Flow and Fragmentation Dynamics of N,N -Dimethylisopropylamine
journal, March 2006

  • Gosselin, Jaimie L.; Minitti, Michael P.; Rudakov, Fedor M.
  • The Journal of Physical Chemistry A, Vol. 110, Issue 12
  • DOI: 10.1021/jp0574706

Ultrafast time-resolved electron diffraction with megavolt electron beams
journal, October 2006

  • Hastings, J. B.; Rudakov, F. M.; Dowell, D. H.
  • Applied Physics Letters, Vol. 89, Issue 18
  • DOI: 10.1063/1.2372697

X-Ray Interactions: Photoabsorption, Scattering, Transmission, and Reflection at E = 50-30,000 eV, Z = 1-92
journal, July 1993

  • Henke, B. L.; Gullikson, E. M.; Davis, J. C.
  • Atomic Data and Nuclear Data Tables, Vol. 54, Issue 2, p. 181-342
  • DOI: 10.1006/adnd.1993.1013

Ultrafast X-ray Auger probing of photoexcited molecular dynamics
journal, June 2014

  • McFarland, B. K.; Farrell, J. P.; Miyabe, S.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5235

Time-Resolved Electron Diffraction from Selectively Aligned Molecules
journal, May 2009


Mega-electron-volt ultrafast electron diffraction at SLAC National Accelerator Laboratory
journal, July 2015

  • Weathersby, S. P.; Brown, G.; Centurion, M.
  • Review of Scientific Instruments, Vol. 86, Issue 7
  • DOI: 10.1063/1.4926994

Mechanism and Dynamics of Azobenzene Photoisomerization
journal, July 2003

  • Schultz, Thomas; Quenneville, Jason; Levine, Benjamin
  • Journal of the American Chemical Society, Vol. 125, Issue 27
  • DOI: 10.1021/ja021363x

Stable transmission of radio frequency signals on fiber links using interferometric delay sensing
journal, January 2009

  • Wilcox, Russell; Byrd, J. M.; Doolittle, Lawrence
  • Optics Letters, Vol. 34, Issue 20
  • DOI: 10.1364/OL.34.003050

The diffraction signatures of individual vibrational modes in polyatomic molecules
journal, January 2000

  • Ryu, Seol; Weber, Peter M.; Stratt, Richard M.
  • The Journal of Chemical Physics, Vol. 112, Issue 3
  • DOI: 10.1063/1.480678

Toward structural femtosecond chemical dynamics: imaging chemistry in space and time
journal, January 2014

  • Minitti, Michael P.; Budarz, James M.; Kirrander, Adam
  • Faraday Discuss., Vol. 171
  • DOI: 10.1039/C4FD00030G

Femtosecond electron diffraction studies of strongly driven structural phase transitions
journal, April 2004


Electronically Driven Structure Changes of Si Captured by Femtosecond Electron Diffraction
journal, April 2008


The X-ray Pump–Probe instrument at the Linac Coherent Light Source
journal, April 2015

  • Chollet, Matthieu; Alonso-Mori, Roberto; Cammarata, Marco
  • Journal of Synchrotron Radiation, Vol. 22, Issue 3
  • DOI: 10.1107/S1600577515005135

Chemical reaction dynamics I and electron dynamics in molecules: general discussion
journal, January 2014

  • Vendrell, Oriol; Küpper, Jochen; Wolf, Martin
  • Faraday Discuss., Vol. 171
  • DOI: 10.1039/C4FD90014F

Femtochemistry:  Atomic-Scale Dynamics of the Chemical Bond
journal, June 2000

  • Zewail, Ahmed H.
  • The Journal of Physical Chemistry A, Vol. 104, Issue 24
  • DOI: 10.1021/jp001460h

Compression of Subrelativistic Space-Charge-Dominated Electron Bunches for Single-Shot Femtosecond Electron Diffraction
journal, December 2010


Ultrafast Bond Softening in Bismuth: Mapping a Solid's Interatomic Potential with X-rays
journal, February 2007


Mean amplitudes of vibration of SF6 and intramolecular multiple scattering
journal, December 1981

  • Miller, Bruce R.; Fink, M.
  • The Journal of Chemical Physics, Vol. 75, Issue 11
  • DOI: 10.1063/1.441976

Time-resolved imaging of purely valence-electron dynamics during a chemical reaction
journal, April 2011

  • Hockett, Paul; Bisgaard, Christer Z.; Clarkin, Owen J.
  • Nature Physics, Vol. 7, Issue 8
  • DOI: 10.1038/nphys1980

Ring-Closing Reaction in Diarylethene Captured by Femtosecond Electron Crystallography
journal, September 2013

  • Jean-Ruel, Hubert; Gao, Meng; Kochman, Michal A.
  • The Journal of Physical Chemistry B, Vol. 117, Issue 49
  • DOI: 10.1021/jp409245h

Ultrafast Electron Diffraction (UED): A New Development for the 4D Determination of Transient Molecular Structures
journal, June 2003

  • Srinivasan, Ramesh; Lobastov, Vladimir A.; Ruan, Chong-Yu
  • Helvetica Chimica Acta, Vol. 86, Issue 6
  • DOI: 10.1002/hlca.200390147