skip to main content
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Time-resolved photoemission study of the electronic structure and dynamics of chemisorbed alkali atoms on Ru(0001)

; ; ; ; ; ;
Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
Grant/Contract Number:  
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Name: Physical Review B Journal Volume: 93 Journal Issue: 4; Journal ID: ISSN 2469-9950
American Physical Society
Country of Publication:
United States

Citation Formats

Zhang, Shengmin, Wang, Cong, Cui, Xuefeng, Wang, Yanan, Argondizzo, Adam, Zhao, Jin, and Petek, Hrvoje. Time-resolved photoemission study of the electronic structure and dynamics of chemisorbed alkali atoms on Ru(0001). United States: N. p., 2016. Web. doi:10.1103/PhysRevB.93.045401.
Zhang, Shengmin, Wang, Cong, Cui, Xuefeng, Wang, Yanan, Argondizzo, Adam, Zhao, Jin, & Petek, Hrvoje. Time-resolved photoemission study of the electronic structure and dynamics of chemisorbed alkali atoms on Ru(0001). United States. doi:10.1103/PhysRevB.93.045401.
Zhang, Shengmin, Wang, Cong, Cui, Xuefeng, Wang, Yanan, Argondizzo, Adam, Zhao, Jin, and Petek, Hrvoje. Tue . "Time-resolved photoemission study of the electronic structure and dynamics of chemisorbed alkali atoms on Ru(0001)". United States. doi:10.1103/PhysRevB.93.045401.
title = {Time-resolved photoemission study of the electronic structure and dynamics of chemisorbed alkali atoms on Ru(0001)},
author = {Zhang, Shengmin and Wang, Cong and Cui, Xuefeng and Wang, Yanan and Argondizzo, Adam and Zhao, Jin and Petek, Hrvoje},
abstractNote = {},
doi = {10.1103/PhysRevB.93.045401},
journal = {Physical Review B},
number = 4,
volume = 93,
place = {United States},
year = {2016},
month = {1}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: 10.1103/PhysRevB.93.045401

Save / Share:

Works referenced in this record:

Two-Photon Photoemission Study of the Coverage-Dependent Electronic Structure of Chemisorbed Alkali Atoms on a Ag(111) Surface
journal, September 2011

  • Wang, Lei-Ming; Sametoglu, Vahit; Winkelmann, Aimo
  • The Journal of Physical Chemistry A, Vol. 115, Issue 34
  • DOI: 10.1021/jp111932r

Generalized Gradient Approximation Made Simple
journal, October 1996

  • Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
  • Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
  • DOI: 10.1103/PhysRevLett.77.3865

Excited states in the alkali/noble metal surface systems: A model system for the study of charge transfer dynamics at surfaces
journal, January 2007

Unoccupied electronic states of the Cs/Cu(100) and Cs/Cu(111) adsorption systems
journal, December 1997

Electronic structure of adsorbed alkali atoms for comparison with UPS data
journal, June 1979

Position and linewidth of the K-induced 4s resonance on Ag(100): a two-photon photoemission study
journal, March 1993

Long-Lived Excited States at Surfaces: Cs / Cu ( 111 ) and Cs / Cu ( 100 ) Systems
journal, January 2001

Resonances induced by Cs adsorbates on Cu(100): Localization of image potential states
journal, May 2002

From ultrasoft pseudopotentials to the projector augmented-wave method
journal, January 1999

Real-Time Observation of Adsorbate Atom Motion Above a Metal Surface
journal, May 2000

Fundamental physics of vacuum electron sources
journal, November 2005

Transient excitons at metal surfaces
journal, June 2014

  • Cui, Xuefeng; Wang, Cong; Argondizzo, Adam
  • Nature Physics, Vol. 10, Issue 7
  • DOI: 10.1038/nphys2981

Theory of Electrical Double Layers in Adsorbed Films
journal, March 1935

Electronic structure of the Ru(0001) surface
journal, February 2000

Alkali metal adsorption on Ru(001)
journal, July 1987

Ultrafast interferometric pump–probe correlation measurements in systems with broadened bands or continua
journal, January 2000

  • Weida, Miles J.; Ogawa, Susumu; Nagano, Hisashi
  • Journal of the Optical Society of America B, Vol. 17, Issue 8
  • DOI: 10.1364/JOSAB.17.001443

π Resonance of Chemisorbed Alkali Atoms on Noble Metals
journal, December 2008

Bulk and surface electron states in ruthenium
journal, January 1985

A chemical and theoretical way to look at bonding on surfaces
journal, July 1988

S URFACE F EMTOCHEMISTRY : Observation and Quantum Control of Frustrated Desorption of Alkali Atoms from Noble Metals
journal, October 2002

Electronic potential of a chemisorption interface
journal, August 2008

Optical Intersubband Transitions and Femtosecond Dynamics in Ag / Fe(100) Quantum Wells
journal, February 2002

Ab initiomolecular dynamics for liquid metals
journal, January 1993

Phase and Energy Relaxation in an Antibonding Surface State: Cs/Cu(111)
journal, March 1999

Alkali-metal adsorption on Al(111) and Al(100)
journal, April 1994

Cs and CO coadsorbed on Ru(0001): low-energy electron diffraction analysis
journal, July 1995

Photoexcitation of adsorbates on metal surfaces: One-step or three-step
journal, September 2012

  • Petek, Hrvoje
  • The Journal of Chemical Physics, Vol. 137, Issue 9
  • DOI: 10.1063/1.4746801

Scanning tunneling microscopy and kinetic Monte Carlo investigation of cesium superlattices on Ag(111)
journal, December 2008

Detailed features of the surface electronic states of K/Cu(111) by density functional theory
journal, April 2010

Potassium adsorption on Co-covered Ru(0001) surfaces: A combined MQS and TDS study
journal, November 1989

Molecular Electronic Level Alignment at Weakly Coupled Organic Film/Metal Interfaces
journal, October 2014

  • Zhao, Jin; Feng, Min; Dougherty, Daniel Barker
  • ACS Nano, Vol. 8, Issue 10
  • DOI: 10.1021/nn5049969

Current progress in understanding alkali metal adsorption on metal surfaces
journal, February 1997

Ultrafast multiphoton pump-probe photoemission excitation pathways in rutile TiO 2 ( 110 )
journal, April 2015

Lifetime of excited electronic states at surfaces: Comparison between the alkali/Cu(111) systems
journal, June 2002

Surface Femtochemistry:  Frustrated Desorption of Alkali Atoms from Noble Metals
journal, July 2001

  • Petek, H.; Nagano, H.; Weida, M. J.
  • The Journal of Physical Chemistry B, Vol. 105, Issue 29
  • DOI: 10.1021/jp0045235

Alkali-metal adsorption on metals
journal, January 1989

Field-Emission Studies of Electronic Energy Levels of Adsorbed Atoms
journal, March 1970

Collisions of atoms and ions with surfaces under grazing incidence
journal, September 2002

Key ingredients of the alkali atom – metal surface interaction: Chemical bonding versus spectral properties
journal, May 2013

Spectral properties of Cs and Ba on Cu(111) at very low coverage: Two-photon photoemission spectroscopy and electronic structure theory
journal, December 2009

Self-consistent approach for spectral properties of single alkali adatoms on Cu(111)
journal, January 2012

Approach to Alkali-Metal Chemisorption within the Anderson Model
journal, July 1971

Adsorption of H2O on Ru(001)
journal, November 1991

Energy shifts and broadening of atomic levels near metal surfaces
journal, September 1990

The low energy dynamics of adsorbates on metal surfaces investigated with helium atom scattering
journal, April 2003

Resonance lifetime and energy of an excited Cs state on Cu(111)
journal, April 1997

Electronic structure and Fermi surface of Ru(0001) and Ru(100) measured with high-resolution angle-resolved photoemission
journal, December 2013

Time-dependent electron phenomena at surfaces
journal, November 2010

  • Muino, R. D.; Sanchez-Portal, D.; Silkin, V. M.
  • Proceedings of the National Academy of Sciences, Vol. 108, Issue 3
  • DOI: 10.1073/pnas.1008517107

Decay dynamics of photoexcited alkali chemisorbates: Real-time investigations in the femtosecond regime
journal, August 1999

On the Mutual Potential Energy of a Plane Network of Doublets
journal, February 1927

  • Topping, J.
  • Proceedings of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 114, Issue 766
  • DOI: 10.1098/rspa.1927.0025

4 s Valence Level of Adsorbed K Atoms Probed by Metastable-He Deexcitation Spectroscopy
journal, September 1985

Long-lived adsorbate states on metal surfaces
journal, January 2000

  • Gauyacq, Jean-Pierre; Borisov, Andreï G.; Raseev, Georges
  • Faraday Discussions, Vol. 117
  • DOI: 10.1039/b002630l

Ab initio molecular dynamics for open-shell transition metals
journal, November 1993

Time-Resolved Two-Photon Photoemission of Unoccupied Electronic States of Periodically Rippled Graphene on Ru(0001)
journal, January 2012

Ultra-fast dynamics of electron thermalization, cooling and transport effects in Ru(001)
journal, January 2004

  • Lisowski, M.; Loukakos, P. A.; Bovensiepen, U.
  • Applied Physics A: Materials Science & Processing, Vol. 78, Issue 2
  • DOI: 10.1007/s00339-003-2301-7

Adsorption geometry of Cu ( 111 ) Cs studied by scanning tunneling microscopy
journal, June 2006

Nature of the charge localized between alkali adatoms and metal substrates
journal, February 1994

Stabilisation of alkali-adsorbate-induced states on Cu(111) surfaces
journal, June 1999

Ab initio molecular-dynamics simulation of the liquid-metal–amorphous-semiconductor transition in germanium
journal, May 1994

Coverage-dependent electronic structure of Na on Cu(111)
journal, July 1994

Influence of Xe adlayer morphology and electronic structure on image-potential state lifetimes of Ru(0001)
journal, January 2000

Analysis of the electronic structure of copper via two-dimensional photoelectron momentum distribution patterns
journal, April 2012

Hot electron lifetimes in metals probed by time-resolved two-photon photoemission
journal, August 2015

The work function of adsorbed alkalis on metals revisited: a coverage-dependent polarizability approach
journal, November 1997

The role of Auger decay in hot electron excitation in copper
journal, January 2000

Vibrational analysis of cesium on Ru(0001)
journal, February 1996

Unoccupied electronic structure of Ru(0001)
journal, June 2007

Unoccupied electron band structure of Na overlayers on Al(111)
journal, July 1987

Unoccupied electronic band structure of an ordered potassium layer on copper: Cu(111)-(2×2)K
journal, March 1990

Hot-electron dynamics at Cu(100), Cu(110), and Cu(111) surfaces:mComparison of experiment with Fermi-liquid theory
journal, April 1997

Femtosecond time-resolved two-photon photoemission studies of electron dynamics in metals
journal, December 1997

The Superatom States of Fullerenes and Their Hybridization into the Nearly Free Electron Bands of Fullerites
journal, March 2009

  • Zhao, Jin; Feng, Min; Yang, Jinlong
  • ACS Nano, Vol. 3, Issue 4
  • DOI: 10.1021/nn800834k

Highly Ordered, Millimeter-Scale, Continuous, Single-Crystalline Graphene Monolayer Formed on Ru (0001)
journal, December 2008

Adsorption of cesium on Ru(001)
journal, December 1985

Theory of inelastic lifetimes of low-energy electrons in metals
journal, January 2000

Theory of the alkali-metal chemisorption on metal surfaces
journal, October 1988

Theory of atomic chemisorption on simple metals
journal, July 1978

Quantum Control of Nuclear Motion at a Metal Surface
journal, November 2000

  • Petek, H.; Nagano, H.; Weida, M. J.
  • The Journal of Physical Chemistry A, Vol. 104, Issue 45
  • DOI: 10.1021/jp001218a

Ordered phases and phase transitions of cesium on the Cu(111) surface
journal, May 1988

  • Fan, W. C.; Ignatiev, A.
  • Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films, Vol. 6, Issue 3
  • DOI: 10.1116/1.575096

Optical Dephasing in Cu(111) Measured by Interferometric Two-Photon Time-Resolved Photoemission
journal, February 1997