Spectral reconstruction analysis for enhancing signal-to-noise in time-resolved spectroscopies

doi:10.1063/1.4931581

Title: Spectral reconstruction analysis for enhancing signal-to-noise in time-resolved spectroscopies

Authors:

^[1]; Smith, Jonathan M. ^[1]; Dai, Hai-Lung ^[1]

Department of Chemistry, Temple University, 1901 N. 13th Street, Philadelphia, Pennsylvania 19122, USA

Publication Date:: 2015-09-29

Sponsoring Org.:: USDOE

OSTI Identifier:: 1229685

Grant/Contract Number:: DEFG 02-86ER 134584

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: The Journal of Chemical Physics

Additional Journal Information:: Journal Name: The Journal of Chemical Physics Journal Volume: 143 Journal Issue: 12; Journal ID: ISSN 0021-9606

Publisher:: American Institute of Physics

Country of Publication:: United States

Language:: English

Citation Formats


                    Wilhelm, Michael J., Smith, Jonathan M., and Dai, Hai-Lung. Spectral reconstruction analysis for enhancing signal-to-noise in time-resolved spectroscopies.  United States: N. p., 2015. 
        Web.  doi:10.1063/1.4931581.

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                    Wilhelm, Michael J., Smith, Jonathan M., & Dai, Hai-Lung. Spectral reconstruction analysis for enhancing signal-to-noise in time-resolved spectroscopies.  United States.  doi:10.1063/1.4931581.

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                    Wilhelm, Michael J., Smith, Jonathan M., and Dai, Hai-Lung. Tue .  
        "Spectral reconstruction analysis for enhancing signal-to-noise in time-resolved spectroscopies".  United States.  doi:10.1063/1.4931581.

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@article{osti_1229685,

  title        = {Spectral reconstruction analysis for enhancing signal-to-noise in time-resolved spectroscopies},

  author       = {Wilhelm, Michael J. and Smith, Jonathan M. and Dai, Hai-Lung},

  abstractNote = {},

  doi          = {10.1063/1.4931581},

  journal      = {The Journal of Chemical Physics},

  number       = 12,

  volume       = 143,

  place        = {United States},

  year         = {2015},

  month        = {9}

}

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DOI: 10.1063/1.4931581

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Title: Spectral reconstruction analysis for enhancing signal-to-noise in time-resolved spectroscopies

Citation Formats

X-ray photoelectron spectroscopic studies of the heterogenous reaction of gaseous nitric acid with sodium chloride: Kinetics and contribution to the chemistry of the marine troposphere journal, July 1994

HCN elimination from vinyl cyanide: product energy partitioning, the role of hydrogen–deuterium exchange reactions and a new pathway journal, January 2015

Strong combination-band IR emission from highly vibrationally excited acetylene journal, January 2010

Synchrotron Infrared Measurements of Dense Hydrogen to 360 GPa journal, April 2012

Temperature dependence of the CN stretching vibration of a nitrile-derivatized phenylalanine in water journal, April 2003

Following protein folding in real time using NMR spectroscopy journal, October 1995

The 193 nm photolysis of NO2: NO(ν) vibrational distribution, O(1D) quantum yield and emission from vibrationally excited NO2 journal, July 2005

A new approach toward transition state spectroscopy journal, January 2013

Time‐resolved Fourier transform spectroscopy with 0.25 cm −1 spectral and <10 −7 s time resolution in the visible region journal, June 1992

The unimolecular dissociation of vinylcyanide: A theoretical investigation of a complex multichannel reaction journal, February 1999

Fast events in protein folding initiated by nanosecond laser photolysis. journal, December 1993

T HE D YNAMICS OF “S TRETCHED M OLECULES ”: Experimental Studies of Highly Vibrationally Excited Molecules With Stimulated Emission Pumping journal, October 2001

Chemical Activation through Super Energy Transfer Collisions journal, January 2014

Vibrational relaxation of NO (v = 1–16) with NO, N2O, NO2, He and Ar studied by time-resolved Fourier transform infrared emission journal, January 2009

Time-Resolved Molecular Frame Dynamics of Fixed-in-Space CS2 Molecules journal, March 2009

-Helix formation in a photoswitchable peptide tracked from picoseconds to microseconds by time-resolved IR spectroscopy journal, February 2005

Gas-phase photodissociation of CH 3 COCN at 308 nm by time-resolved Fourier-transform infrared emission spectroscopy journal, January 2012

Vibrational Energy Flow in Highly Excited Molecules: Role of Intramolecular Vibrational Redistribution journal, January 1996

The Two Competitive Photodissociation Channels in Cyano Carbonyls (NCC(O)X, X = CH 3 , CH(CH 3 ) 2 , C(CH 3 ) 3 , OCH 3 ) at 193 nm. A Study by Photofragment Translational Energy Spectroscopy journal, March 2000

Collisional Energy Transfer from Highly Vibrationally Excited Radicals Is Very Efficient journal, December 2012

Raman scattering cross section of adsorbed pyridine molecules on a smooth silver surface journal, June 1981

Photodissociation of acrylonitrile at 193 nm: A photofragment translational spectroscopy study using synchrotron radiation for product photoionization journal, April 1998

Infrared Absorption Spectrum of the Simplest Criegee Intermediate CH2OO journal, April 2013

Photolysis of Astrophysically Relevant Acrylonitrile: A Matrix Experimental Study journal, March 2014

Photodissociation of vinyl cyanide at 193 nm: Nascent product distributions of the molecular elimination channels journal, January 2009

Discerning vibronic molecular dynamics using time-resolved photoelectron spectroscopy journal, September 1999

Reaction of Bromide with Bromate in Thin-Film Water journal, September 2010

Signal-to-noise enhancement in time-resolved IR emission spectra through two-dimensional correlation analysis journal, July 2008

Monitoring the Kinetics of Ion-Dependent Protein Folding by Time-Resolved NMR Spectroscopy at Atomic Resolution journal, July 2000

The ν1 CH stretching mode of the ketenyl (HCCO) radical journal, February 2008

Measuring Picosecond Isomerization Kinetics via Broadband Microwave Spectroscopy journal, May 2008

Ab Initio and RRKM Study of the HCN/HNC Elimination Channels from Vinyl Cyanide journal, February 2011

X-ray photoelectron spectroscopic studies of the heterogenous reaction of gaseous nitric acid with sodium chloride: Kinetics and contribution to the chemistry of the marine troposphere
journal, July 1994

HCN elimination from vinyl cyanide: product energy partitioning, the role of hydrogen–deuterium exchange reactions and a new pathway
journal, January 2015

Strong combination-band IR emission from highly vibrationally excited acetylene
journal, January 2010

Synchrotron Infrared Measurements of Dense Hydrogen to 360 GPa
journal, April 2012

Temperature dependence of the CN stretching vibration of a nitrile-derivatized phenylalanine in water
journal, April 2003

Following protein folding in real time using NMR spectroscopy
journal, October 1995

The 193 nm photolysis of NO2: NO(ν) vibrational distribution, O(1D) quantum yield and emission from vibrationally excited NO2
journal, July 2005

A new approach toward transition state spectroscopy
journal, January 2013

Time‐resolved Fourier transform spectroscopy with 0.25 cm ⁻¹ spectral and <10 ⁻⁷ s time resolution in the visible region
journal, June 1992

The unimolecular dissociation of vinylcyanide: A theoretical investigation of a complex multichannel reaction
journal, February 1999

Fast events in protein folding initiated by nanosecond laser photolysis.
journal, December 1993

T HE D YNAMICS OF “S TRETCHED M OLECULES ”: Experimental Studies of Highly Vibrationally Excited Molecules With Stimulated Emission Pumping
journal, October 2001

Chemical Activation through Super Energy Transfer Collisions
journal, January 2014

Vibrational relaxation of NO (v = 1–16) with NO, N2O, NO2, He and Ar studied by time-resolved Fourier transform infrared emission
journal, January 2009

Time-Resolved Molecular Frame Dynamics of Fixed-in-Space CS2 Molecules
journal, March 2009

-Helix formation in a photoswitchable peptide tracked from picoseconds to microseconds by time-resolved IR spectroscopy
journal, February 2005

Gas-phase photodissociation of CH ₃ COCN at 308 nm by time-resolved Fourier-transform infrared emission spectroscopy
journal, January 2012

Vibrational Energy Flow in Highly Excited Molecules: Role of Intramolecular Vibrational Redistribution
journal, January 1996

The Two Competitive Photodissociation Channels in Cyano Carbonyls (NCC(O)X, X = CH ₃ , CH(CH ₃ ) ₂ , C(CH ₃ ) ₃ , OCH ₃ ) at 193 nm. A Study by Photofragment Translational Energy Spectroscopy
journal, March 2000

Collisional Energy Transfer from Highly Vibrationally Excited Radicals Is Very Efficient
journal, December 2012

Raman scattering cross section of adsorbed pyridine molecules on a smooth silver surface
journal, June 1981

Photodissociation of acrylonitrile at 193 nm: A photofragment translational spectroscopy study using synchrotron radiation for product photoionization
journal, April 1998

Infrared Absorption Spectrum of the Simplest Criegee Intermediate CH2OO
journal, April 2013

Photolysis of Astrophysically Relevant Acrylonitrile: A Matrix Experimental Study
journal, March 2014

Photodissociation of vinyl cyanide at 193 nm: Nascent product distributions of the molecular elimination channels
journal, January 2009

Discerning vibronic molecular dynamics using time-resolved photoelectron spectroscopy
journal, September 1999

Reaction of Bromide with Bromate in Thin-Film Water
journal, September 2010

Signal-to-noise enhancement in time-resolved IR emission spectra through two-dimensional correlation analysis
journal, July 2008

Monitoring the Kinetics of Ion-Dependent Protein Folding by Time-Resolved NMR Spectroscopy at Atomic Resolution
journal, July 2000

The ν1 CH stretching mode of the ketenyl (HCCO) radical
journal, February 2008

Measuring Picosecond Isomerization Kinetics via Broadband Microwave Spectroscopy
journal, May 2008

Ab Initio and RRKM Study of the HCN/HNC Elimination Channels from Vinyl Cyanide
journal, February 2011