Tunable electronic correlation effects in nanotube-light interactions
Abstract
Electronic many-body correlation effects in one-dimensional (1D) systems such as carbon nanotubes have been predicted to strongly modify the nature of photoexcited states. In this work we directly probe this effect using broadband elastic light scattering from individual suspended carbon nanotubes under electrostatic gating conditions. We observe significant shifts in optical transition energies, as well as line broadening, as the carrier density is increased. These effects demonstrate the role of screening of many-body electronic interactions on the different length scales, a feature inherent to quasi-1D systems. Our findings further demonstrate the possibility of electrical tuning of optical transitions and provide a basis for understanding of various optical phenomena in carbon nanotubes and other quasi-1D systems in the presence of charge carrier doping.
- Authors:
-
- Kyoto Univ. (Japan); Nagoya Univ. (Japan); Columbia Univ., New York, NY (United States)
- Columbia Univ., New York, NY (United States); SanDisk, Milpitas, CA (United States)
- Columbia Univ., New York, NY (United States)
- Hokkaido Univ., Sapporo (Japan)
- IBM, Yorktown Heights, NY (United States). Thomas J. Watson Research Center; Skolkovo Inst. of Science and Technology (Russia)
- Univ. of Utah, Salt Lake City, UT (United States); Columbia Univ., New York, NY (United States)
- Columbia Univ., New York, NY (United States); National Center for Nanoscience and Technology, Beijing (China)
- National Centre for Scientific Research (CNRS), Strasbourg (France)
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Re-Defining Photovoltaic Efficiency Through Molecule Scale Control (RPEMSC)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
- OSTI Identifier:
- 1370391
- Alternate Identifier(s):
- OSTI ID: 1225131
- Grant/Contract Number:
- SC0001085; DMR-1106225
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review. B, Condensed Matter and Materials Physics
- Additional Journal Information:
- Journal Volume: 92; Journal Issue: 20; Related Information: RPEMSC partners with Columbia University (lead); Brookhaven National Laboratory; Purdue University; Journal ID: ISSN 1098-0121
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Miyauchi, Yuhei, Zhang, Zhengyi, Takekoshi, Mitsuhide, Tomio, Yuh, Suzuura, Hidekatsu, Perebeinos, Vasili, Deshpande, Vikram V., Lu, Chenguang, Berciaud, Stéphane, Kim, Philip, Hone, James, and Heinz, Tony F. Tunable electronic correlation effects in nanotube-light interactions. United States: N. p., 2015.
Web. doi:10.1103/PhysRevB.92.205407.
Miyauchi, Yuhei, Zhang, Zhengyi, Takekoshi, Mitsuhide, Tomio, Yuh, Suzuura, Hidekatsu, Perebeinos, Vasili, Deshpande, Vikram V., Lu, Chenguang, Berciaud, Stéphane, Kim, Philip, Hone, James, & Heinz, Tony F. Tunable electronic correlation effects in nanotube-light interactions. United States. https://doi.org/10.1103/PhysRevB.92.205407
Miyauchi, Yuhei, Zhang, Zhengyi, Takekoshi, Mitsuhide, Tomio, Yuh, Suzuura, Hidekatsu, Perebeinos, Vasili, Deshpande, Vikram V., Lu, Chenguang, Berciaud, Stéphane, Kim, Philip, Hone, James, and Heinz, Tony F. Wed .
"Tunable electronic correlation effects in nanotube-light interactions". United States. https://doi.org/10.1103/PhysRevB.92.205407. https://www.osti.gov/servlets/purl/1370391.
@article{osti_1370391,
title = {Tunable electronic correlation effects in nanotube-light interactions},
author = {Miyauchi, Yuhei and Zhang, Zhengyi and Takekoshi, Mitsuhide and Tomio, Yuh and Suzuura, Hidekatsu and Perebeinos, Vasili and Deshpande, Vikram V. and Lu, Chenguang and Berciaud, Stéphane and Kim, Philip and Hone, James and Heinz, Tony F.},
abstractNote = {Electronic many-body correlation effects in one-dimensional (1D) systems such as carbon nanotubes have been predicted to strongly modify the nature of photoexcited states. In this work we directly probe this effect using broadband elastic light scattering from individual suspended carbon nanotubes under electrostatic gating conditions. We observe significant shifts in optical transition energies, as well as line broadening, as the carrier density is increased. These effects demonstrate the role of screening of many-body electronic interactions on the different length scales, a feature inherent to quasi-1D systems. Our findings further demonstrate the possibility of electrical tuning of optical transitions and provide a basis for understanding of various optical phenomena in carbon nanotubes and other quasi-1D systems in the presence of charge carrier doping.},
doi = {10.1103/PhysRevB.92.205407},
journal = {Physical Review. B, Condensed Matter and Materials Physics},
number = 20,
volume = 92,
place = {United States},
year = {Wed Nov 04 00:00:00 EST 2015},
month = {Wed Nov 04 00:00:00 EST 2015}
}
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Works referencing / citing this record:
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