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Title: Prospects of nanoscience with nanocrystals

Abstract

Colloidal nanocrystals (NCs, i.e., crystalline nanoparticles) have become an important class of materials with great potential for applications ranging from medicine to electronic and optoelectronic devices. Today’s strong research focus on NCs has been prompted by the tremendous progress in their synthesis. Impressively narrow size distributions of just a few percent, rational shape-engineering, compositional modulation, electronic doping, and tailored surface chemistries are now feasible for a broad range of inorganic compounds. The performance of inorganic NC-based photovoltaic and light-emitting devices has become competitive to other state-of-the-art materials. Semiconductor NCs hold unique promise for near- and mid-infrared technologies, where very few semiconductor materials are available. On a purely fundamental side, new insights into NC growth, chemical transformations, and self-organization can be gained from rapidly progressing in situ characterization and direct imaging techniques. In addition, new phenomena are constantly being discovered in the photophysics of NCs and in the electronic properties of NC solids. In this Nano Focus, we review the state of the art in research on colloidal NCs focusing on the most recent works published in the last 2 years.

Authors:
 [1];  [2];  [3];  [4];  [5];  [6];  [7];  [8];  [9];  [10];  [11];  [12];  [13];  [14];  [10];  [6];  [15]
  1. ETH Zurich, Zurich (Switzerland); EMPA Swiss Federal Laboratories for Materials Science and Technology, Dubendorf (Switzerland)
  2. Italian Inst. of Technology, Genoa (Italy); Delft Univ. of Technology, Delft (The Netherlands)
  3. Catalonia Energy Research Inst., Saint Adria del Besos (Spain); ICREA, Barcelona (Spain)
  4. Ghent Univ., Ghent (Belgium)
  5. Univ. of Chicago, Chicago, IL (United States); Argonne National Lab., Argonne, IL (United States)
  6. Univ. of Pennsylvania, Philadelphia, PA (United States)
  7. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  8. City Univ. of Hong Kong, Kowloon (Hong Kong)
  9. Univ. Grenoble Alpes, Grenoble (France)
  10. Univ. of Texas, Austin, TX (United States)
  11. Univ. of Chicago, Chicago, IL (United States)
  12. ICFO, The Institute of Photonic Sciences, Castelldefels (Spain)
  13. Philipps Universitat Marburg, Marburg (Germany); CIC Biomagune, San Sebastian (Spain)
  14. Inst. for Basic Science, Seoul (Korea); Seoul National Univ. (Korea)
  15. Johannes Kepler Univ. Linz, Linz (Austria); Friedrich-Alexander-Universitat, Erlangen (Germany); Energie Campus Nurnberg, Nurnberg (Germany)
Publication Date:
Research Org.:
Energy Frontier Research Centers (EFRC) (United States). Center for Advanced Solar Photophysics (CASP); Univ. of Texas, Austin, TX (United States); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1210563
Alternate Identifier(s):
OSTI ID: 1215391; OSTI ID: 1215414
Grant/Contract Number:  
AC52-06NA25396; AC02-06CH11357; SC0002158
Resource Type:
Accepted Manuscript
Journal Name:
ACS Nano
Additional Journal Information:
Journal Volume: 9; Journal Issue: 2; Related Information: CASP partners with Los Alamos National Laboratory (lead); University of California, Irvine; University of Colorado; Colorado School of Mines; George Mason University; Los Alamos National Laboratory; University of Minnesota; National Renewable Energy Laboratory; Journal ID: ISSN 1936-0851
Publisher:
American Chemical Society
Country of Publication:
United States
Language:
English
Subject:
77 NANOSCIENCE AND NANOTECHNOLOGY; solar (photovoltaic); solar (fuels); solid state lighting; bio-inspired; electrodes - solar; defects; charge transport; materials and chemistry by design; optics; synthesis (novel materials); synthesis (scalable processing); 36 MATERIALS SCIENCE

Citation Formats

Kovalenko, Maksym V., Manna, Liberato, Cabot, Andreu, Hens, Zeger, Talapin, Dmitri V., Kagan, Cherie R., Klimov, Victor I., Rogach, Andrey L., Reiss, Peter, Milliron, Delia J., Guyot-Sionnnest, Philippe, Konstantatos, Gerasimos, Parak, Wolfgang J., Hyeon, Taeghwan, Korgel, Brian A., Murray, Christopher B., and Heiss, Wolfgang. Prospects of nanoscience with nanocrystals. United States: N. p., 2015. Web. doi:10.1021/nn506223h.
Kovalenko, Maksym V., Manna, Liberato, Cabot, Andreu, Hens, Zeger, Talapin, Dmitri V., Kagan, Cherie R., Klimov, Victor I., Rogach, Andrey L., Reiss, Peter, Milliron, Delia J., Guyot-Sionnnest, Philippe, Konstantatos, Gerasimos, Parak, Wolfgang J., Hyeon, Taeghwan, Korgel, Brian A., Murray, Christopher B., & Heiss, Wolfgang. Prospects of nanoscience with nanocrystals. United States. https://doi.org/10.1021/nn506223h
Kovalenko, Maksym V., Manna, Liberato, Cabot, Andreu, Hens, Zeger, Talapin, Dmitri V., Kagan, Cherie R., Klimov, Victor I., Rogach, Andrey L., Reiss, Peter, Milliron, Delia J., Guyot-Sionnnest, Philippe, Konstantatos, Gerasimos, Parak, Wolfgang J., Hyeon, Taeghwan, Korgel, Brian A., Murray, Christopher B., and Heiss, Wolfgang. Thu . "Prospects of nanoscience with nanocrystals". United States. https://doi.org/10.1021/nn506223h. https://www.osti.gov/servlets/purl/1210563.
@article{osti_1210563,
title = {Prospects of nanoscience with nanocrystals},
author = {Kovalenko, Maksym V. and Manna, Liberato and Cabot, Andreu and Hens, Zeger and Talapin, Dmitri V. and Kagan, Cherie R. and Klimov, Victor I. and Rogach, Andrey L. and Reiss, Peter and Milliron, Delia J. and Guyot-Sionnnest, Philippe and Konstantatos, Gerasimos and Parak, Wolfgang J. and Hyeon, Taeghwan and Korgel, Brian A. and Murray, Christopher B. and Heiss, Wolfgang},
abstractNote = {Colloidal nanocrystals (NCs, i.e., crystalline nanoparticles) have become an important class of materials with great potential for applications ranging from medicine to electronic and optoelectronic devices. Today’s strong research focus on NCs has been prompted by the tremendous progress in their synthesis. Impressively narrow size distributions of just a few percent, rational shape-engineering, compositional modulation, electronic doping, and tailored surface chemistries are now feasible for a broad range of inorganic compounds. The performance of inorganic NC-based photovoltaic and light-emitting devices has become competitive to other state-of-the-art materials. Semiconductor NCs hold unique promise for near- and mid-infrared technologies, where very few semiconductor materials are available. On a purely fundamental side, new insights into NC growth, chemical transformations, and self-organization can be gained from rapidly progressing in situ characterization and direct imaging techniques. In addition, new phenomena are constantly being discovered in the photophysics of NCs and in the electronic properties of NC solids. In this Nano Focus, we review the state of the art in research on colloidal NCs focusing on the most recent works published in the last 2 years.},
doi = {10.1021/nn506223h},
journal = {ACS Nano},
number = 2,
volume = 9,
place = {United States},
year = {Thu Jan 22 00:00:00 EST 2015},
month = {Thu Jan 22 00:00:00 EST 2015}
}

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Organometal Halide Perovskite Quantum Dot Light-Emitting Diodes
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Stable, small, specific, low-valency quantum dots for single-molecule imaging
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Hydrogen bond sensing ability of CdSe/ZnS colloidal quantum dots in ionic medium
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Efficient and Stable White LEDs with Silica-Coated Inorganic Perovskite Quantum Dots
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Engineering uniform nanocrystals: Mechanism of formation and self-assembly into bimetallic nanocrystal superlattices
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Active photonic devices based on colloidal semiconductor nanocrystals and organometallic halide perovskites
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Interplay between spherical confinement and particle shape on the self-assembly of rounded cubes.
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Selective Growth of Metal Sulfide, Metal, and Metal-Alloy on 2D CdS Nanoplates
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Multimetallic Hierarchical Aerogels: Shape Engineering of the Building Blocks for Efficient Electrocatalysis
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Hot injection synthesis of CuInS 2 nanocrystals using metal xanthates and their application in hybrid solar cells
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Understanding quantum confinement and ligand removal in solution-based ZnO thin films from highly stable nanocrystal ink
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Explaining observed stability of excitons in highly excited CdSe nanoplatelets
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Theoretical analysis of screened many-body electrostatic interactions between charged polarizable particles
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Kinetics of the self-assembly of nanocrystal superlattices measured by real-time in situ X-ray scattering
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High luminescence color gradient by physical mixing of two perovskite nanocrystals
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Intra- and inter-nanocrystal charge transport in nanocrystal films
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Augmented band gap tunability in indium-doped zinc sulfide nanocrystals
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Protein-quantum dot nanohybrids for bioanalytical applications: Protein-quantum dot nanohybrids
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A bright future for colloidal quantum dot lasers
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Surface chemistry and buried interfaces in all-inorganic nanocrystalline solids
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In Situ Fabricated Perovskite Nanocrystals: A Revolution in Optical Materials
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Over 800% efficiency enhancement of all-inorganic quantum-dot light emitting diodes with an ultrathin alumina passivating layer
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Determination of association constants towards carbon nanotubes
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All-Inorganic Colloidal Perovskite Quantum Dots: A New Class of Lasing Materials with Favorable Characteristics
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Nanosized Building Blocks for Customizing Novel Antibiofilm Approaches
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Spin Physics of Excitons in Colloidal Nanocrystals
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Kinetics of pressure-induced nanocrystal superlattice formation
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Rod-shaped Zn–Ag–In–Te nanocrystals with wavelength-tunable band-edge photoluminescence in the near-IR region
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Superlattice growth and rearrangement during evaporation-induced nanoparticle self-assembly
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Heavy‐Metal‐Free Colloidal Semiconductor Nanorods: Recent Advances and Future Perspectives
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Nonlinear Optical Properties of Colloidal CH 3 NH 3 PbBr 3 and CsPbBr 3 Quantum Dots: A Comparison Study Using Z-Scan Technique
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Colloidal branched CdSe/CdS ‘nanospiders’ with 2D/1D heterostructure
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Optical properties of nanocrystal films: blue shifted transitions as signature of strong coupling
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Tailoring Copper Nanocrystals towards C 2 Products in Electrochemical CO 2 Reduction
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Determination of quantum yields of semiconductor nanocrystals at the single emitter level via fluorescence correlation spectroscopy
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Direct TEM observation of the “acanthite α-Ag 2 S–argentite β-Ag 2 S” phase transition in a silver sulfide nanoparticle
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When Crystals Go Nano - The Role of Advanced X-ray Total Scattering Methods in Nanotechnology: When Crystals Go Nano - The Role of Advanced X-ray Total Scattering Methods in Nanotechnology
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Genesis, challenges and opportunities for colloidal lead halide perovskite nanocrystals
journal, February 2018

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Novel silicon phases and nanostructures for solar energy conversion
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On the phase control of CuInS 2 nanoparticles from Cu-/In-xanthates
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Humidity-Responsive Single-Nanoparticle-Layer Plasmonic Films
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Superfluorescence from Lead Halide Perovskite Quantum Dot Superlattices
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Dissecting common and divergent molecular pathways elicited by CdSe/ZnS quantum dots in freshwater and marine sentinel invertebrates
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Simultaneous positive and negative optical patterning with dye-sensitized CdSe quantum dots
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Solution-processed silver sulphide nanocrystal film for resistive switching memories
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Synthesis, photophysical properties and surface chemistry of chalcopyrite-type semiconductor nanocrystals
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Cellular interfaces with hydrogen-bonded organic semiconductor hierarchical nanocrystals
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Nucleation of Sodium in a Plasma Stream with Neon
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Mastering heterostructured colloidal nanocrystal properties for light-emitting diodes and solar cells
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Strong Enhancement of PbS Quantum Dot NIR Emission Using Plasmonic Semiconductor Nanocrystals in Nanoporous Silicate Matrix
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Controlled growth of silica–titania hybrid functional nanoparticles through a multistep microfluidic approach
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Continuous-wave infrared optical gain and amplified spontaneous emission at ultralow threshold by colloidal HgTe quantum dots
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Advances in Small Perovskite-Based Lasers
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Enhanced Photoelectrochemical Properties of Zn−Ag−In−Te Nanocrystals with High Energy Photon Excitation
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Composite Polymer Colloids for SERS-Based Applications
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All-Inorganic and Hybrid Capping of Nanocrystals as Key to Their Application-Relevant Processing
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Enhanced mobility CsPbI 3 quantum dot arrays for record-efficiency, high-voltage photovoltaic cells
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Biological synthesis of fluorescent nanoparticles by cadmium and tellurite resistant Antarctic bacteria: exploring novel natural nanofactories
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InPZnS alloy quantum dots with tris(hexylthio)phosphine as a dual anionic precursor
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Synthesis of Cuboctahedral CeO 2 Nanoclusters and Their Assembly into Cuboid Nanoparticles by Oriented Attachment
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Lithiation of Copper Selenide Nanocrystals
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Doped semiconductor nanoparticles synthesized in gas-phase plasmas
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All-Inorganic Bismuth-Based Perovskite Quantum Dots with Bright Blue Photoluminescence and Excellent Stability
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Modulated Triple-Material Nano-Heterostructures: Where Gold Influenced the Chemical Activity of Silver in Nanocrystals
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A facile non-injection phosphorus-free synthesis of semiconductor nanoparticles using new selenium precursors
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Emerging Hierarchical Aerogels: Self-Assembly of Metal and Semiconductor Nanocrystals
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On the kinetics of the removal of ligands from films of colloidal nanocrystals by plasmas
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Temperature-Dependent Exciton and Trap-Related Photoluminescence of CdTe Quantum Dots Embedded in a NaCl Matrix: Implication in Thermometry
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Nanodiamond-Palladium Core-Shell Organohybrid Synthesis: A Mild Vapor-Phase Procedure Enabling Nanolayering Metal onto Functionalized sp 3 -Carbon
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Synthesis and Biomedical Applications of Multifunctional Nanoparticles
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Highly luminescent silica-coated CdS/CdSe/CdS nanoparticles with strong chemical robustness and excellent thermal stability
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Facile synthesized ZnO microcrystals for random microlasers and incandescent-type light sources
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Raman study of laser-induced formation of II–VI nanocrystals in zinc-doped As–S(Se) films
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Tailoring Copper Nanocrystals towards C 2 Products in Electrochemical CO 2 Reduction
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Diameter distribution by deconvolution (DdD): absorption spectra as a practical tool for semiconductor nanoparticle PSD determination
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Diverse Nanoassemblies of Graphene Quantum Dots and Their Mineralogical Counterparts
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Charge transport in strongly coupled quantum dot solids
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Magnetic field-assisted assembly of iron oxide mesocrystals: a matter of nanoparticle shape and magnetic anisotropy
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Emerging Self‐Emissive Technologies for Flexible Displays
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Strong Polarized Photoluminescence from Stretched Perovskite-Nanocrystal-Embedded Polymer Composite Films
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Surface spin magnetism controls the polarized exciton emission from CdSe nanoplatelets
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Mechanism of sulfidation of small zinc oxide nanoparticles
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High-performance thermoelectric nanocomposites from nanocrystal building blocks
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Cd–Cu–Fe–S quaternary nanocrystals exhibiting excellent optical/optoelectronic properties
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Interplay between spherical confinement and particle shape on the self-assembly of rounded cubes
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Identifying and Eliminating Emissive Sub-bandgap States in Thin Films of PbS Nanocrystals
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A Directed Route to Colloidal Nanoparticle Synthesis of the Copper Selenophosphate Cu 3 PSe 4
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Improving the Power‐Conversion Efficiency through Alloying in Common Anion CdZnX (X=S, Se) Nanocrystal Sensitized Solar Cells
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Inkjet printed fluorescent nanorod layers exhibit superior optical performance over quantum dots
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Rb + cations enable the change of luminescence properties in perovskite (Rb x Cs 1−x PbBr 3 ) quantum dots
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All-solution-processed Si films with broadband and omnidirectional light absorption
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Raman study of flash-lamp annealed aqueous Cu 2 ZnSnS 4 nanocrystals
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Architectural Design of Self‐Assembled Hollow Superstructures
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Bioinspired Amyloid Nanodots with Visible Fluorescence
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FeIn 2 S 4 Nanocrystals: A Ternary Metal Chalcogenide Material for Ambipolar Field-Effect Transistors
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Excited-State Dynamics in Colloidal Semiconductor Nanocrystals
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Nonspherical atomic effective pseudopotentials for surface passivation
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A perspective on triplet fusion upconversion: triplet sensitizers beyond quantum dots
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A Directed Route to Colloidal Nanoparticle Synthesis of the Copper Selenophosphate Cu 3 PSe 4
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When Crystals Go Nano - The Role of Advanced X-ray Total Scattering Methods in Nanotechnology
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Excited-State Dynamics in Colloidal Semiconductor Nanocrystals
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Inkjet-printed aligned quantum rod enhancement films for their application in liquid crystal displays
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Superfluorescence from Lead Halide Perovskite Quantum Dot Superlattices
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Brightly Luminescent Core/Shell Nanoplatelets with Continuously Tunable Optical Properties
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Diverse Nanoassemblies of Graphene Quantum Dots and Their Mineralogical Counterparts
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Face the Edges: Catalytic Active Sites of Nanomaterials
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Surfactant-Assisted Cooperative Self-Assembly of Nanoparticles into Active Nanostructures
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The Many “Facets” of Halide Ions in the Chemistry of Colloidal Inorganic Nanocrystals
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Ultrathin One- and Two-Dimensional Colloidal Semiconductor Nanocrystals: Pushing Quantum Confinement to the Limit
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Writing on Nanocrystals: Patterning Colloidal Inorganic Nanocrystal Films through Irradiation-Induced Chemical Transformations of Surface Ligands
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Host–guest chemistry for tuning colloidal solubility, self-organization and photoconductivity of inorganic-capped nanocrystals
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General low-temperature reaction pathway from precursors to monomers before nucleation of compound semiconductor nanocrystals
journal, August 2016

  • Yu, Kui; Liu, Xiangyang; Qi, Ting
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms12223

Optical determination of crystal phase in semiconductor nanocrystals
journal, May 2017

  • Lim, Sung Jun; Schleife, André; Smith, Andrew M.
  • Nature Communications, Vol. 8, Issue 1
  • DOI: 10.1038/ncomms14849

Brightness-equalized quantum dots
journal, October 2015

  • Lim, Sung Jun; Zahid, Mohammad U.; Le, Phuong
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms9210

Cellular interfaces with hydrogen-bonded organic semiconductor hierarchical nanocrystals
journal, July 2017

  • Sytnyk, Mykhailo; Jakešová, Marie; Litviňuková, Monika
  • Nature Communications, Vol. 8, Issue 1
  • DOI: 10.1038/s41467-017-00135-0

Advances in highly doped upconversion nanoparticles
journal, June 2018


Naked Gold Nanoparticles and hot Electrons in Water
journal, May 2018


Size-Dependent Melting Behavior of Colloidal In, Sn and Bi Nanocrystals
journal, November 2015

  • Liu, Minglu; Wang, Robert Y.
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep16353

The Influence of Doping on the Optoelectronic Properties of PbS Colloidal Quantum Dot Solids
journal, January 2016

  • Papagiorgis, P.; Stavrinadis, A.; Othonos, A.
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep18735

Biological synthesis of fluorescent nanoparticles by cadmium and tellurite resistant Antarctic bacteria: exploring novel natural nanofactories
journal, May 2016


Interplay between spherical confinement and particle shape on the self-assembly of rounded cubes.
journalarticle, January 2018

  • Wang, Da; Hermes, Michiel; Kotni, Ramakrishna
  • Springer Science and Business Media LLC
  • DOI: 10.17863/cam.27253

Shape-Controlled Synthesis of Copper Indium Sulfide Nanostructures: Flowers, Platelets and Spheres
journal, December 2019

  • Ning, Jiajia; Kershaw, Stephen V.; Rogach, Andrey L.
  • Nanomaterials, Vol. 9, Issue 12
  • DOI: 10.3390/nano9121779

Fast Anion-Exchange in Highly Luminescent Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, I)
text, January 2015


Impact of Crystal Structure and Particles Shape on the Photoluminescence Intensity of CdSe/CdS Core/Shell Nanocrystals
text, January 2019