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Title: Design and application of a mobile ground-based observatory for continuous measurements of atmospheric trace gas and criteria pollutant species

Abstract

Ground-based measurements of atmospheric trace gas species and criteria pollutants are essential for understanding emissions dynamics across space and time. Gas composition in the lower 50 m of the atmosphere has the greatest direct impacts on human health as well as ecosystem processes; hence data at this level are necessary for addressing carbon-cycle- and public-health-related questions. However, such surface data are generally associated with stationary measurement towers, where spatial representation is limited due to the high cost of establishing and maintaining an extensive network of measurement stations. We describe here a compact mobile laboratory equipped to provide high-precision, high-frequency, continuous, on-road synchronous measurements of CO2, CO, CH4, H2O, NOx, O3, aerosol, meteorological, and geospatial position data. The mobile laboratory has been deployed across the western USA. In addition to describing the vehicle and its capacity, we present data that illustrate the use of the laboratory as a powerful tool for investigating the spatial structure of urban trace gas emissions and criteria pollutants at spatial scales ranging from single streets to whole ecosystem and regional scales. We assess the magnitude of known point sources of CH4 and also identify fugitive urban CH4 emissions. We illustrate how such a mobile laboratory canmore » be used to better understand emissions dynamics and quantify emissions ratios associated with trace gas emissions from wildfire incidents. Lastly, we discuss additional mobile laboratory applications in health and urban metabolism.« less

Authors:
; ; ; ;
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1213097
Grant/Contract Number:  
SC0005266
Resource Type:
Published Article
Journal Name:
Atmospheric Measurement Techniques (Online)
Additional Journal Information:
Journal Name: Atmospheric Measurement Techniques (Online) Journal Volume: 8 Journal Issue: 8; Journal ID: ISSN 1867-8548
Publisher:
Copernicus Publications, EGU
Country of Publication:
Germany
Language:
English

Citation Formats

Bush, S. E., Hopkins, F. M., Randerson, J. T., Lai, C.-T., and Ehleringer, J. R. Design and application of a mobile ground-based observatory for continuous measurements of atmospheric trace gas and criteria pollutant species. Germany: N. p., 2015. Web. doi:10.5194/amt-8-3481-2015.
Bush, S. E., Hopkins, F. M., Randerson, J. T., Lai, C.-T., & Ehleringer, J. R. Design and application of a mobile ground-based observatory for continuous measurements of atmospheric trace gas and criteria pollutant species. Germany. https://doi.org/10.5194/amt-8-3481-2015
Bush, S. E., Hopkins, F. M., Randerson, J. T., Lai, C.-T., and Ehleringer, J. R. Wed . "Design and application of a mobile ground-based observatory for continuous measurements of atmospheric trace gas and criteria pollutant species". Germany. https://doi.org/10.5194/amt-8-3481-2015.
@article{osti_1213097,
title = {Design and application of a mobile ground-based observatory for continuous measurements of atmospheric trace gas and criteria pollutant species},
author = {Bush, S. E. and Hopkins, F. M. and Randerson, J. T. and Lai, C.-T. and Ehleringer, J. R.},
abstractNote = {Ground-based measurements of atmospheric trace gas species and criteria pollutants are essential for understanding emissions dynamics across space and time. Gas composition in the lower 50 m of the atmosphere has the greatest direct impacts on human health as well as ecosystem processes; hence data at this level are necessary for addressing carbon-cycle- and public-health-related questions. However, such surface data are generally associated with stationary measurement towers, where spatial representation is limited due to the high cost of establishing and maintaining an extensive network of measurement stations. We describe here a compact mobile laboratory equipped to provide high-precision, high-frequency, continuous, on-road synchronous measurements of CO2, CO, CH4, H2O, NOx, O3, aerosol, meteorological, and geospatial position data. The mobile laboratory has been deployed across the western USA. In addition to describing the vehicle and its capacity, we present data that illustrate the use of the laboratory as a powerful tool for investigating the spatial structure of urban trace gas emissions and criteria pollutants at spatial scales ranging from single streets to whole ecosystem and regional scales. We assess the magnitude of known point sources of CH4 and also identify fugitive urban CH4 emissions. We illustrate how such a mobile laboratory can be used to better understand emissions dynamics and quantify emissions ratios associated with trace gas emissions from wildfire incidents. Lastly, we discuss additional mobile laboratory applications in health and urban metabolism.},
doi = {10.5194/amt-8-3481-2015},
journal = {Atmospheric Measurement Techniques (Online)},
number = 8,
volume = 8,
place = {Germany},
year = {Wed Aug 26 00:00:00 EDT 2015},
month = {Wed Aug 26 00:00:00 EDT 2015}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.5194/amt-8-3481-2015

Citation Metrics:
Cited by: 13 works
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