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Title: Hyperspectral image reconstruction for x-ray fluorescence tomography

Abstract

A penalized maximum-likelihood estimation is proposed to perform hyperspectral (spatio-spectral) image reconstruction for X-ray fluorescence tomography. The approach minimizes a Poisson-based negative log-likelihood of the observed photon counts, and uses a penalty term that has the effect of encouraging local continuity of model parameter estimates in both spatial and spectral dimensions simultaneously. The performance of the reconstruction method is demonstrated with experimental data acquired from a seed of arabidopsis thaliana collected at the 13-ID-E microprobe beamline at the Advanced Photon Source. The resulting element distribution estimates with the proposed approach show significantly better reconstruction quality than the conventional analytical inversion approaches, and allows for a high data compression factor which can reduce data acquisition times remarkably. In particular, this technique provides the capability to tomographically reconstruct full energy dispersive spectra without compromising reconstruction artifacts that impact the interpretation of results.

Authors:
 [1];  [2];  [3];  [3];  [1]
+ Show Author Affiliations
  1. Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source
  2. Argonne National Lab. (ANL), Argonne, IL (United States). Mathematics and Computer Science Div.
  3. Univ. of Chicago, Chicago, IL (United States). Center for Advanced Radiation Sources
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1200860
Grant/Contract Number:  
AC02-06CH11357; FG02-94ER14466; EAR1128799
Resource Type:
Accepted Manuscript
Journal Name:
Optics Express
Additional Journal Information:
Journal Volume: 23; Journal Issue: 7; Journal ID: ISSN 1094-4087
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
97 MATHEMATICS AND COMPUTING; 59 BASIC BIOLOGICAL SCIENCES

Citation Formats

Gürsoy, Doǧa, Biçer, Tekin, Lanzirotti, Antonio, Newville, Matthew G., and De Carlo, Francesco. Hyperspectral image reconstruction for x-ray fluorescence tomography. United States: N. p., 2015. Web. doi:10.1364/OE.23.009014.
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Gürsoy, Doǧa, Biçer, Tekin, Lanzirotti, Antonio, Newville, Matthew G., & De Carlo, Francesco. Hyperspectral image reconstruction for x-ray fluorescence tomography. United States. https://doi.org/10.1364/OE.23.009014
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Gürsoy, Doǧa, Biçer, Tekin, Lanzirotti, Antonio, Newville, Matthew G., and De Carlo, Francesco. Thu . "Hyperspectral image reconstruction for x-ray fluorescence tomography". United States. https://doi.org/10.1364/OE.23.009014. https://www.osti.gov/servlets/purl/1200860.
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@article{osti_1200860,
title = {Hyperspectral image reconstruction for x-ray fluorescence tomography},
author = {Gürsoy, Doǧa and Biçer, Tekin and Lanzirotti, Antonio and Newville, Matthew G. and De Carlo, Francesco},
abstractNote = {A penalized maximum-likelihood estimation is proposed to perform hyperspectral (spatio-spectral) image reconstruction for X-ray fluorescence tomography. The approach minimizes a Poisson-based negative log-likelihood of the observed photon counts, and uses a penalty term that has the effect of encouraging local continuity of model parameter estimates in both spatial and spectral dimensions simultaneously. The performance of the reconstruction method is demonstrated with experimental data acquired from a seed of arabidopsis thaliana collected at the 13-ID-E microprobe beamline at the Advanced Photon Source. The resulting element distribution estimates with the proposed approach show significantly better reconstruction quality than the conventional analytical inversion approaches, and allows for a high data compression factor which can reduce data acquisition times remarkably. In particular, this technique provides the capability to tomographically reconstruct full energy dispersive spectra without compromising reconstruction artifacts that impact the interpretation of results.},
doi = {10.1364/OE.23.009014},
journal = {Optics Express},
number = 7,
volume = 23,
place = {United States},
year = {Thu Jan 01 00:00:00 EST 2015},
month = {Thu Jan 01 00:00:00 EST 2015}
}
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https://doi.org/10.1364/OE.23.009014
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    Works referencing / citing this record:

    2016 Atomic Spectrometry Update – a review of advances in X-ray fluorescence spectrometry and its applications
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    Optimization-based simultaneous alignment and reconstruction in multi-element tomography
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    • Optics Letters, Vol. 44, Issue 17
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