Evaluation of the ²³⁹Pu prompt fission neutron spectrum induced by neutrons of 500 keV and associated covariances
Abstract
We present evaluations of the prompt fission neutron spectrum (PFNS) of ²³⁹Pu induced by 500 keV neutrons, and associated covariances. In a previous evaluation by Talou et al. 2010, surprisingly low evaluated uncertainties were obtained, partly due to simplifying assumptions in the quantification of uncertainties from experiment and model. Therefore, special emphasis is placed here on a thorough uncertainty quantification of experimental data and of the Los Alamos model predicted values entering the evaluation. In addition, the Los Alamos model was extended and an evaluation technique was employed that takes into account the qualitative differences between normalized model predicted values and experimental shape data. These improvements lead to changes in the evaluated PFNS and overall larger evaluated uncertainties than in the previous work. However, these evaluated uncertainties are still smaller than those obtained in a statistical analysis using experimental information only, due to strong model correlations. Hence, suggestions to estimate model defect uncertainties are presented, which lead to more reasonable evaluated uncertainties. The calculated keff of selected criticality benchmarks obtained with these new evaluations agree with each other within their uncertainties despite the different approaches to estimate model defect uncertainties. The keff one standard deviations overlap with some of thosemore »
- Authors:
-
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Proton Source (APS)
- Vienna International Centre, Vienna (Austria)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1193393
- Alternate Identifier(s):
- OSTI ID: 1247271
- Report Number(s):
- LA-UR-14-22817
Journal ID: ISSN 0168-9002; PII: S016890021500532X
- Grant/Contract Number:
- AC52-06NA25396
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment
- Additional Journal Information:
- Journal Volume: 791; Journal Issue: C; Journal ID: ISSN 0168-9002
- Publisher:
- Elsevier
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 73 NUCLEAR PHYSICS AND RADIATION PHYSICS; nuclear data evaluation; ²³⁹Pu prompt fission neutron spectrum; uncertainty quantification
Citation Formats
Neudecker, D., Talou, P., Kawano, T., Smith, D. L., Capote, R., Rising, M. E., and Kahler, A. C. Evaluation of the ²³⁹Pu prompt fission neutron spectrum induced by neutrons of 500 keV and associated covariances. United States: N. p., 2015.
Web. doi:10.1016/j.nima.2015.04.044.
Neudecker, D., Talou, P., Kawano, T., Smith, D. L., Capote, R., Rising, M. E., & Kahler, A. C. Evaluation of the ²³⁹Pu prompt fission neutron spectrum induced by neutrons of 500 keV and associated covariances. United States. https://doi.org/10.1016/j.nima.2015.04.044
Neudecker, D., Talou, P., Kawano, T., Smith, D. L., Capote, R., Rising, M. E., and Kahler, A. C. Sat .
"Evaluation of the ²³⁹Pu prompt fission neutron spectrum induced by neutrons of 500 keV and associated covariances". United States. https://doi.org/10.1016/j.nima.2015.04.044. https://www.osti.gov/servlets/purl/1193393.
@article{osti_1193393,
title = {Evaluation of the ²³⁹Pu prompt fission neutron spectrum induced by neutrons of 500 keV and associated covariances},
author = {Neudecker, D. and Talou, P. and Kawano, T. and Smith, D. L. and Capote, R. and Rising, M. E. and Kahler, A. C.},
abstractNote = {We present evaluations of the prompt fission neutron spectrum (PFNS) of ²³⁹Pu induced by 500 keV neutrons, and associated covariances. In a previous evaluation by Talou et al. 2010, surprisingly low evaluated uncertainties were obtained, partly due to simplifying assumptions in the quantification of uncertainties from experiment and model. Therefore, special emphasis is placed here on a thorough uncertainty quantification of experimental data and of the Los Alamos model predicted values entering the evaluation. In addition, the Los Alamos model was extended and an evaluation technique was employed that takes into account the qualitative differences between normalized model predicted values and experimental shape data. These improvements lead to changes in the evaluated PFNS and overall larger evaluated uncertainties than in the previous work. However, these evaluated uncertainties are still smaller than those obtained in a statistical analysis using experimental information only, due to strong model correlations. Hence, suggestions to estimate model defect uncertainties are presented, which lead to more reasonable evaluated uncertainties. The calculated keff of selected criticality benchmarks obtained with these new evaluations agree with each other within their uncertainties despite the different approaches to estimate model defect uncertainties. The keff one standard deviations overlap with some of those obtained using ENDF/B-VII.1, albeit their mean values are further away from unity. Spectral indexes for the Jezebel critical assembly calculated with the newly evaluated PFNS agree with the experimental data for selected (n,γ) and (n,f) reactions, and show improvements for high-energy threshold (n,2n) reactions compared to ENDF/B-VII.1.},
doi = {10.1016/j.nima.2015.04.044},
journal = {Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment},
number = C,
volume = 791,
place = {United States},
year = {Sat Aug 01 00:00:00 EDT 2015},
month = {Sat Aug 01 00:00:00 EDT 2015}
}
Web of Science
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Works referencing / citing this record:
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