Lithium-Sulfur Batteries: from Liquid to Solid Cells?
Abstract
Lithium-sulfur (Li-S) batteries supply a theoretical specific energy 5 times higher than that of lithium-ion batteries (2,500 vs. ~500 Wh kg-1). However, the insulating properties and polysulfide shuttle effects of the sulfur cathode and the safety concerns of the lithium anode in liquid electrolytes are still key limitations to practical use of traditional Li-S batteries. In this review, we start with a brief discussion on fundamentals of Li-S batteries and key challenges associated with the conventional liquid cells. Then, we introduce the most recent progresses in the liquid systems, including the sulfur positive electrodes, the lithium negative electrodes, and the electrolytes and binders. We discuss the significance of investigating electrode reaction mechanisms in liquid cells using in-situ techniques to monitor the compositional and morphological changes. By moving from the traditional liquid cells to recent solid cells, we discuss the importance of this game-changing shift with positive advances in both solid electrolytes and electrode materials. Finally, the opportunities and perspectives for future research on Li-S batteries are presented.
- Authors:
-
- Zhejiang Univ., Hangzhou (China).
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE); USDOE Office of Science (SC)
- OSTI Identifier:
- 1185628
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Materials Chemistry. A
- Additional Journal Information:
- Journal Volume: 3; Journal Issue: 3; Journal ID: ISSN 2050-7488
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; batteries; solid electrolyte; electrical energy storage; lithium-sulfur batteries
Citation Formats
Lin, Zhan, and Liang, Chengdu. Lithium-Sulfur Batteries: from Liquid to Solid Cells?. United States: N. p., 2014.
Web. doi:10.1039/C4TA04727C.
Lin, Zhan, & Liang, Chengdu. Lithium-Sulfur Batteries: from Liquid to Solid Cells?. United States. https://doi.org/10.1039/C4TA04727C
Lin, Zhan, and Liang, Chengdu. Tue .
"Lithium-Sulfur Batteries: from Liquid to Solid Cells?". United States. https://doi.org/10.1039/C4TA04727C. https://www.osti.gov/servlets/purl/1185628.
@article{osti_1185628,
title = {Lithium-Sulfur Batteries: from Liquid to Solid Cells?},
author = {Lin, Zhan and Liang, Chengdu},
abstractNote = {Lithium-sulfur (Li-S) batteries supply a theoretical specific energy 5 times higher than that of lithium-ion batteries (2,500 vs. ~500 Wh kg-1). However, the insulating properties and polysulfide shuttle effects of the sulfur cathode and the safety concerns of the lithium anode in liquid electrolytes are still key limitations to practical use of traditional Li-S batteries. In this review, we start with a brief discussion on fundamentals of Li-S batteries and key challenges associated with the conventional liquid cells. Then, we introduce the most recent progresses in the liquid systems, including the sulfur positive electrodes, the lithium negative electrodes, and the electrolytes and binders. We discuss the significance of investigating electrode reaction mechanisms in liquid cells using in-situ techniques to monitor the compositional and morphological changes. By moving from the traditional liquid cells to recent solid cells, we discuss the importance of this game-changing shift with positive advances in both solid electrolytes and electrode materials. Finally, the opportunities and perspectives for future research on Li-S batteries are presented.},
doi = {10.1039/C4TA04727C},
journal = {Journal of Materials Chemistry. A},
number = 3,
volume = 3,
place = {United States},
year = {Tue Nov 11 00:00:00 EST 2014},
month = {Tue Nov 11 00:00:00 EST 2014}
}
Web of Science
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Rational Design of Si/SiO 2 @Hierarchical Porous Carbon Spheres as Efficient Polysulfide Reservoirs for High-Performance Li-S Battery
journal, February 2016
- Rehman, Sarish; Guo, Shaojun; Hou, Yanglong
- Advanced Materials, Vol. 28, Issue 16
Recent Developments of the Lithium Metal Anode for Rechargeable Non-Aqueous Batteries
journal, July 2016
- Zhang, Kai; Lee, Gi-Hyeok; Park, Mihui
- Advanced Energy Materials, Vol. 6, Issue 20
Deciphering the Reaction Mechanism of Lithium–Sulfur Batteries by In Situ/Operando Synchrotron‐Based Characterization Techniques
journal, March 2019
- Yan, Yingying; Cheng, Chen; Zhang, Liang
- Advanced Energy Materials, Vol. 9, Issue 18
Freestanding reduced graphene oxide–sulfur composite films for highly stable lithium–sulfur batteries
journal, January 2017
- Luo, Shuwen; Yao, Minjie; Lei, Song
- Nanoscale, Vol. 9, Issue 14
A PPy/ZnO functional interlayer to enhance electrochemical performance of lithium/sulfur batteries
journal, October 2018
- Yin, Fuxing; Ren, Jun; Zhang, Yongguang
- Nanoscale Research Letters, Vol. 13, Issue 1
High-Performance All-Solid-State Lithium-Sulfur Batteries Enabled by Amorphous Sulfur-Coated Reduced Graphene Oxide Cathodes
journal, May 2017
- Yao, Xiayin; Huang, Ning; Han, Fudong
- Advanced Energy Materials, Vol. 7, Issue 17
Review on High-Loading and High-Energy Lithium-Sulfur Batteries
journal, May 2017
- Peng, Hong-Jie; Huang, Jia-Qi; Cheng, Xin-Bing
- Advanced Energy Materials, Vol. 7, Issue 24
Sulfur-Immobilized Nitrogen and Oxygen Co-Doped Hierarchically Porous Biomass Carbon for Lithium-Sulfur Batteries: Influence of Sulfur Content and Distribution on Its Performance
journal, November 2017
- Chulliyote, Reshma; Hareendrakrishnakumar, Haritha; Raja, Murugan
- ChemistrySelect, Vol. 2, Issue 32
Structural Reorganization–Based Nanomaterials as Anodes for Lithium‐Ion Batteries: Design, Preparation, and Performance
journal, September 2019
- Han, Yu; Huang, Guoyong; Xu, Shengming
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Janus Separator of Polypropylene-Supported Cellular Graphene Framework for Sulfur Cathodes with High Utilization in Lithium-Sulfur Batteries
journal, October 2015
- Peng, Hong-Jie; Wang, Dai-Wei; Huang, Jia-Qi
- Advanced Science, Vol. 3, Issue 1
Rational Design of a Dual-Function Hybrid Cathode Substrate for Lithium-Sulfur Batteries
journal, June 2018
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- Advanced Energy Materials, Vol. 8, Issue 24
Housing Sulfur in Polymer Composite Frameworks for Li–S Batteries
journal, February 2019
- Hencz, Luke; Chen, Hao; Ling, Han Yeu
- Nano-Micro Letters, Vol. 11, Issue 1
Functional Mesoporous Carbon-Coated Separator for Long-Life, High-Energy Lithium-Sulfur Batteries
journal, July 2015
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- Advanced Functional Materials, Vol. 25, Issue 33
Sulfiphilic Few‐Layered MoSe 2 Nanoflakes Decorated rGO as a Highly Efficient Sulfur Host for Lithium‐Sulfur Batteries
journal, August 2019
- Tian, Wenzhi; Xi, Baojuan; Feng, Zhenyu
- Advanced Energy Materials, Vol. 9, Issue 36
A review of solid electrolytes for safe lithium-sulfur batteries
journal, November 2017
- Sun, Ying-Zhi; Huang, Jia-Qi; Zhao, Chen-Zi
- Science China Chemistry, Vol. 60, Issue 12
Hierarchical TiO2 spheres as highly efficient polysulfide host for lithium-sulfur batteries
journal, March 2016
- Yang, Zhi-Zheng; Wang, Hui-Yuan; Lu, Lun
- Scientific Reports, Vol. 6, Issue 1
Li 2 S–Embedded copper metal–organic framework cathode with superior electrochemical performance for Li–S batteries
journal, January 2018
- Feng, Yan; Zhang, Yuliang; Du, Guixiang
- New Journal of Chemistry, Vol. 42, Issue 16
Rational design of a mesoporous silica-based cathode for efficient trapping of polysulfides in Li–S batteries
journal, January 2020
- Chen, Chao; Xu, Huifang; Zhang, Bingkai
- Chemical Communications, Vol. 56, Issue 5