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Title: Excitation-energy dependence of fission in the mercury region

Abstract

Recent experiments on β-delayed fission reported an asymmetric mass yield in the neutron-deficient nucleus 180Hg. Earlier experiments in the mass region A = 190–200 close to the β-stability line, using the (p,f) and (α,f) reactions, observed a more symmetric distribution of fission fragments. While the β-delayed fission of 180Hg can be associated with relatively low excitation energy, this is not the case for light-ion reactions, which result in warm compound nuclei. Here, the low-energy fission of 180,198Hg has been successfully described by theory in terms of strong shell effects in pre-scission configurations associated with dinuclear structures.

Authors:
 [1];  [2];  [3];  [4];  [5]
  1. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of Tennessee, Knoxville, TN (United States)
  2. Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Warsaw, Warsaw (Poland)
  3. Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Kashmir, Srinagar (India)
  4. Univ. of Tennessee, Knoxville, TN (United States); Maria Curie-Sklodowska Univ., Lublin (Poland)
  5. Maria Curie-Sklodowska Univ., Lublin (Poland)
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Oak Ridge Leadership Computing Facility (OLCF); Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC); USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1454619
Alternate Identifier(s):
OSTI ID: 1180093
Report Number(s):
LLNL-JRNL-656299
Journal ID: ISSN 0556-2813; PRVCAN; 777127; TRN: US1901095
Grant/Contract Number:  
AC52-07NA27344; FG02-96ER40963; NA0001820; SC0008499; FC52-08NA28752
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review C, Nuclear Physics
Additional Journal Information:
Journal Volume: 90; Journal Issue: 2; Journal ID: ISSN 0556-2813
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Citation Formats

McDonnell, J. D., Nazarewicz, W., Sheikh, J. A., Staszczak, A., and Warda, M. Excitation-energy dependence of fission in the mercury region. United States: N. p., 2014. Web. doi:10.1103/PhysRevC.90.021302.
McDonnell, J. D., Nazarewicz, W., Sheikh, J. A., Staszczak, A., & Warda, M. Excitation-energy dependence of fission in the mercury region. United States. https://doi.org/10.1103/PhysRevC.90.021302
McDonnell, J. D., Nazarewicz, W., Sheikh, J. A., Staszczak, A., and Warda, M. Fri . "Excitation-energy dependence of fission in the mercury region". United States. https://doi.org/10.1103/PhysRevC.90.021302. https://www.osti.gov/servlets/purl/1454619.
@article{osti_1454619,
title = {Excitation-energy dependence of fission in the mercury region},
author = {McDonnell, J. D. and Nazarewicz, W. and Sheikh, J. A. and Staszczak, A. and Warda, M.},
abstractNote = {Recent experiments on β-delayed fission reported an asymmetric mass yield in the neutron-deficient nucleus 180Hg. Earlier experiments in the mass region A = 190–200 close to the β-stability line, using the (p,f) and (α,f) reactions, observed a more symmetric distribution of fission fragments. While the β-delayed fission of 180Hg can be associated with relatively low excitation energy, this is not the case for light-ion reactions, which result in warm compound nuclei. Here, the low-energy fission of 180,198Hg has been successfully described by theory in terms of strong shell effects in pre-scission configurations associated with dinuclear structures.},
doi = {10.1103/PhysRevC.90.021302},
journal = {Physical Review C, Nuclear Physics},
number = 2,
volume = 90,
place = {United States},
year = {Fri Aug 29 00:00:00 EDT 2014},
month = {Fri Aug 29 00:00:00 EDT 2014}
}

Journal Article:

Citation Metrics:
Cited by: 56 works
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Figures / Tables:

FIG. 1 FIG. 1: (Color online) Ground-state potential-energy surfaces for (a) 180Hg and (b) 198Hg in the ($Q_{20}$, $Q_{30}$) plane calculated in HFB-SkM*. The static fission pathway aEF corresponding to asymmetric elongated fragments is marked.

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Works referenced in this record:

β -delayed fission of 192 , 194 At
journal, January 2013


β -delayed fission of 186 , 188 Bi isotopes
journal, January 2013


Diabaticity of nuclear motion: problems and perspectives
journal, May 1993


Prescission shapes of symmetrically fissioning very heavy nuclei
journal, February 1988


Shell effects in the symmetric-modal fission of pre-actinide nuclei
journal, September 1998


Nuclear ground-state properties from mean-field calculations
journal, September 2002

  • Dobaczewski, J.; Nazarewicz, W.; Stoitsov, M. V.
  • The European Physical Journal A, Vol. 15, Issue 1-2
  • DOI: 10.1140/epja/i2001-10218-8

Microscopic analysis of collective dynamics in low energy fission
journal, October 1984


Colloquium : Beta-delayed fission of atomic nuclei
journal, October 2013


Finite-temperature HFB theory
journal, January 1981


Surface symmetry energy of nuclear energy density functionals
journal, March 2011


β -delayed fission of 180 Tl
journal, October 2013


Temperature-dependent Hartree-Fock-Bogoliubov calculations in hot rotating nuclei
journal, March 1986


Fission Barriers of Compound Superheavy Nuclei
journal, May 2009


Contrasting fission potential-energy structure of actinides and mercury isotopes
journal, August 2012


β -delayed fission and α decay of 178 Tl
journal, October 2013


Shell corrections for finite-depth deformed potentials: Green’s function oscillator expansion method
journal, May 2000


Thermal fission pathways in [sup 232]Th
conference, January 2009

  • McDonnell, J. D.; Nazarewicz, W.; Sheikh, J. A.
  • 4TH INTERNATIONAL WORKSHOP ON NUCLEAR FISSION AND FISSION-PRODUCT SPECTROSCOPY, AIP Conference Proceedings
  • DOI: 10.1063/1.3258254

The Ame2003 atomic mass evaluation
journal, December 2003


Microscopic calculations of fission barriers and critical angular momenta for excited heavy nuclear systems
journal, March 1981


Role of deformed shell effects on the mass asymmetry in nuclear fission of mercury isotopes
journal, December 2012


Scission-point model of nuclear fission based on deformed-shell effects
journal, November 1976


Towards a better parametrisation of Skyrme-like effective forces: A critical study of the SkM force
journal, September 1982


Funny Hills: The Shell-Correction Approach to Nuclear Shell Effects and Its Applications to the Fission Process
journal, April 1972


Augmented Lagrangian method for constrained nuclear density functional theory
journal, August 2010


Experimental evidence for the separability of compound-nucleus and fragment properties in fission
journal, July 2008


Third minima in thorium and uranium isotopes in a self-consistent theory
journal, May 2013


Systematic study of fission barriers of excited superheavy nuclei
journal, July 2009


Microscopic description of complex nuclear decay: Multimodal fission
journal, July 2009


Solution of the Skyrme–Hartree–Fock–Bogolyubov equations in the Cartesian deformed harmonic-oscillator basis.
journal, January 2012

  • Schunck, N.; Dobaczewski, J.; McDonnell, J.
  • Computer Physics Communications, Vol. 183, Issue 1
  • DOI: 10.1016/j.cpc.2011.08.013

Mass distributions for induced fission of different Hg isotopes
journal, October 2012


Calculated fission yields of neutron-deficient mercury isotopes
journal, February 2012


Nuclear fission modes and fragment mass asymmetries in a five-dimensional deformation space
journal, February 2001

  • Möller, P.; Madland, D. G.; Sierk, A. J.
  • Nature, Vol. 409, Issue 6822
  • DOI: 10.1038/35057204

Isotopic and isotonic effects in fission-fragment mass yields of actinide nuclei
journal, November 2002


New Type of Asymmetric Fission in Proton-Rich Nuclei
journal, December 2010


Fission modes of mercury isotopes
journal, August 2012


Isospin dependence of mass-distribution shape of fission fragments of Hg isotopes
journal, October 2013


Works referencing / citing this record:

Microscopic theory of nuclear fission: a review
journal, October 2016


r -process nucleosynthesis: connecting rare-isotope beam facilities with the cosmos
journal, July 2019

  • Horowitz, C. J.; Arcones, A.; Côté, B.
  • Journal of Physics G: Nuclear and Particle Physics, Vol. 46, Issue 8
  • DOI: 10.1088/1361-6471/ab0849

Nuclear fission: a review of experimental advances and phenomenology
journal, November 2017

  • Andreyev, A. N.; Nishio, K.; Schmidt, K-H
  • Reports on Progress in Physics, Vol. 81, Issue 1
  • DOI: 10.1088/1361-6633/aa82eb

Review on the progress in nuclear fission—experimental methods and theoretical descriptions
journal, September 2018


Asymmetric fission around lead: The case of Po 198
journal, December 2019


Performance of the Fourier shape parametrization for the fission process
journal, March 2017


On possible shape isomers in the Pt-Ra region of nuclei
journal, April 2017


Multi-dimensional fission model with a complex absorbing potential
text, January 2015


Fission dynamics within time-dependent Hartree-Fock: deformation-induced fission
text, January 2015


Microscopic Theory of Nuclear Fission: A Review
text, January 2015


Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.