Speciation of Sulfur in Biochar Produced from Pyrolysis and Gasification of Oak and Corn Stover

Cheah, Singfoong; Malone, Shealyn C.; Feik, Calvin J.

doi:10.1021/es500073r

Title: Speciation of Sulfur in Biochar Produced from Pyrolysis and Gasification of Oak and Corn Stover

Authors:

Cheah, Singfoong ^[1]; Malone, Shealyn C. ^[1]; Feik, Calvin J. ^[1]

National Renewable Energy Laboratory, 15013 Denver West Parkway, MS 3322, Golden, Colorado 80401, United States

Publication Date:: Tue Jul 08 00:00:00 EDT 2014

Sponsoring Org.:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Bioenergy Technologies Office (BETO)

OSTI Identifier:: 1179593

Grant/Contract Number:: AC36-08GO28308

Resource Type:: Published Article

Journal Name:: Environmental Science and Technology

Additional Journal Information:: Journal Name: Environmental Science and Technology Journal Volume: 48 Journal Issue: 15; Journal ID: ISSN 0013-936X

Publisher:: American Chemical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Cheah, Singfoong, Malone, Shealyn C., and Feik, Calvin J. Speciation of Sulfur in Biochar Produced from Pyrolysis and Gasification of Oak and Corn Stover.  United States: N. p., 2014. 
Web.  doi:10.1021/es500073r.

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                    Cheah, Singfoong, Malone, Shealyn C., & Feik, Calvin J. Speciation of Sulfur in Biochar Produced from Pyrolysis and Gasification of Oak and Corn Stover.  United States.  https://doi.org/10.1021/es500073r

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                    Cheah, Singfoong, Malone, Shealyn C., and Feik, Calvin J. Tue .  
"Speciation of Sulfur in Biochar Produced from Pyrolysis and Gasification of Oak and Corn Stover".  United States.  https://doi.org/10.1021/es500073r.

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@article{osti_1179593,

  title        = {Speciation of Sulfur in Biochar Produced from Pyrolysis and Gasification of Oak and Corn Stover},

  author       = {Cheah, Singfoong and Malone, Shealyn C. and Feik, Calvin J.},

  abstractNote = {},

  doi          = {10.1021/es500073r},

  journal      = {Environmental Science and Technology},

  number       = 15,

  volume       = 48,

  place        = {United States},

  year         = {Tue Jul 08 00:00:00 EDT 2014},

  month        = {Tue Jul 08 00:00:00 EDT 2014}

}

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Citation Formats

ATHENA , ARTEMIS , HEPHAESTUS : data analysis for X-ray absorption spectroscopy using IFEFFIT journal, June 2005

Determination of selected elements in whole coal and in coal ash from the eight Argonne Premium coal samples by atomic absorption spectrometry, atomic emission spectrometry, and ion-selective electrode journal, September 1990

Chemistry, thermodynamics and kinetics of reactions of sulphur in coal-gas reactions: A review journal, April 1978

Catalytic and Noncatalytic Gasification of Pyrolysis Oil journal, June 2007

Study on the fate of metal elements from biomass in a bench-scale fluidized bed gasifier journal, June 2013

Historical Developments in Hydroprocessing Bio-oils journal, May 2007

Sulfur Transformations during Thermal Conversion of Herbaceous Biomass journal, April 2004

Sulfur: not a “silent” element any more journal, January 2006

Characterization of biochar from fast pyrolysis and gasification systems journal, October 2009

Ligand K-edge x-ray absorption spectroscopic studies: metal-ligand covalency in a series of transition metal tetrachlorides journal, March 1995

Physiological functions of mineral macronutrients journal, June 2009

Review of the pyrolysis platform for coproducing bio-oil and biochar journal, September 2009

Temperature and source material influence ecological attributes of ponderosa pine and Douglas-fir charcoal journal, August 2006

Synthesis of Transportation Fuels from Biomass: Chemistry, Catalysts, and Engineering journal, September 2006

Determination of Forms of Sulfur in Coal journal, January 1977

Dairy-Manure Derived Biochar Effectively Sorbs Lead and Atrazine journal, March 2009

Fast pyrolysis processes for biomass journal, March 2000

Pilot-Scale Gasification of Corn Stover, Switchgrass, Wheat Straw, and Wood: 1. Parametric Study and Comparison with Literature journal, February 2010

Water, alkali and char in flash pyrolysis oils journal, January 1994

Real-Time and Post-reaction Microscopic Structural Analysis of Biomass Undergoing Pyrolysis journal, July 2009

Characterization of Biochars Produced from Cornstovers for Soil Amendment journal, October 2010

A unified, global model for the pyrolysis of cellulose journal, January 1994

Pilot Scale Production of Mixed Alcohols from Wood journal, January 2014

Transformation and Release to the Gas Phase of Cl, K, and S during Combustion of Annual Biomass journal, September 2004

Review of Mid- to High-Temperature Sulfur Sorbents for Desulfurization of Biomass- and Coal-derived Syngas journal, November 2009

Imaging of mineral-enriched biochar by FTIR, Raman and SEM–EDX journal, September 2012

Investigation of Sulfur Retention and the Effect of Inorganic Matter during Pyrolysis of South Australian Low-Rank Coals journal, September 1998

Techno-economic comparison of biomass-to-transportation fuels via pyrolysis, gasification, and biochemical pathways journal, November 2010

Biomass gasification with pure steam in fluidised bed: 12 variables that affect the effectiveness of the biomass gasifier journal, January 2008

Sulfur K-edge x-ray absorption spectroscopy of petroleum asphaltenes and model compounds journal, April 1989

Evaluation of Catalyst Deactivation during Catalytic Steam Reforming of Biomass-Derived Syngas journal, October 2005

SIXPack a Graphical User Interface for XAS Analysis Using IFEFFIT journal, January 2005

Chemical Equilibrium Prediction of Potassium, Sodium, and Chlorine Concentrations in the Product Gas from Biomass Gasification journal, December 2007

A handful of carbon journal, May 2007

Nickel cerium olivine catalyst for catalytic gasification of biomass journal, May 2013

Dynamic Molecular Structure of Plant Biomass-Derived Black Carbon (Biochar) journal, February 2010

Nitrogen and Sulfur Fertilization and Dynamics in a Brazilian Entisol under Pasture journal, July 2010

Sulfur forms in organic substrates affecting S mineralization in soil journal, June 2013

Sulfur Speciation in Soil by S K -Edge XANES Spectroscopy: Comparison of Spectral Deconvolution and Linear Combination Fitting journal, April 2011

Bio-energy in the black journal, September 2007

Transformation of Sulfur Species during Steam/Air Regeneration on a Ni Biomass Conditioning Catalyst journal, June 2012

Sampling of Powders and Bulk Materials book, January 1986

Decomposition of pyrite and trapping of sulphur in a coal matrix during pyrolysis of coal journal, November 1984

Elucidation of Biomass Pyrolysis Products Using a Laminar Entrained Flow Reactor and Char Particle Imaging journal, January 2011

ATHENA , ARTEMIS , HEPHAESTUS : data analysis for X-ray absorption spectroscopy using IFEFFIT
journal, June 2005

Determination of selected elements in whole coal and in coal ash from the eight Argonne Premium coal samples by atomic absorption spectrometry, atomic emission spectrometry, and ion-selective electrode
journal, September 1990

Chemistry, thermodynamics and kinetics of reactions of sulphur in coal-gas reactions: A review
journal, April 1978

Catalytic and Noncatalytic Gasification of Pyrolysis Oil
journal, June 2007

Study on the fate of metal elements from biomass in a bench-scale fluidized bed gasifier
journal, June 2013

Historical Developments in Hydroprocessing Bio-oils
journal, May 2007

Sulfur Transformations during Thermal Conversion of Herbaceous Biomass
journal, April 2004

Sulfur: not a “silent” element any more
journal, January 2006

Characterization of biochar from fast pyrolysis and gasification systems
journal, October 2009

Ligand K-edge x-ray absorption spectroscopic studies: metal-ligand covalency in a series of transition metal tetrachlorides
journal, March 1995

Physiological functions of mineral macronutrients
journal, June 2009

Review of the pyrolysis platform for coproducing bio-oil and biochar
journal, September 2009

Temperature and source material influence ecological attributes of ponderosa pine and Douglas-fir charcoal
journal, August 2006

Synthesis of Transportation Fuels from Biomass: Chemistry, Catalysts, and Engineering
journal, September 2006

Determination of Forms of Sulfur in Coal
journal, January 1977

Dairy-Manure Derived Biochar Effectively Sorbs Lead and Atrazine
journal, March 2009

Fast pyrolysis processes for biomass
journal, March 2000

Pilot-Scale Gasification of Corn Stover, Switchgrass, Wheat Straw, and Wood: 1. Parametric Study and Comparison with Literature
journal, February 2010

Water, alkali and char in flash pyrolysis oils
journal, January 1994

Real-Time and Post-reaction Microscopic Structural Analysis of Biomass Undergoing Pyrolysis
journal, July 2009

Characterization of Biochars Produced from Cornstovers for Soil Amendment
journal, October 2010

A unified, global model for the pyrolysis of cellulose
journal, January 1994

Pilot Scale Production of Mixed Alcohols from Wood
journal, January 2014

Transformation and Release to the Gas Phase of Cl, K, and S during Combustion of Annual Biomass
journal, September 2004

Review of Mid- to High-Temperature Sulfur Sorbents for Desulfurization of Biomass- and Coal-derived Syngas
journal, November 2009

Imaging of mineral-enriched biochar by FTIR, Raman and SEM–EDX
journal, September 2012

Investigation of Sulfur Retention and the Effect of Inorganic Matter during Pyrolysis of South Australian Low-Rank Coals
journal, September 1998

Techno-economic comparison of biomass-to-transportation fuels via pyrolysis, gasification, and biochemical pathways
journal, November 2010

Biomass gasification with pure steam in fluidised bed: 12 variables that affect the effectiveness of the biomass gasifier
journal, January 2008

Sulfur K-edge x-ray absorption spectroscopy of petroleum asphaltenes and model compounds
journal, April 1989

Evaluation of Catalyst Deactivation during Catalytic Steam Reforming of Biomass-Derived Syngas
journal, October 2005

SIXPack a Graphical User Interface for XAS Analysis Using IFEFFIT
journal, January 2005

Chemical Equilibrium Prediction of Potassium, Sodium, and Chlorine Concentrations in the Product Gas from Biomass Gasification
journal, December 2007

A handful of carbon
journal, May 2007

Nickel cerium olivine catalyst for catalytic gasification of biomass
journal, May 2013

Dynamic Molecular Structure of Plant Biomass-Derived Black Carbon (Biochar)
journal, February 2010

Nitrogen and Sulfur Fertilization and Dynamics in a Brazilian Entisol under Pasture
journal, July 2010

Sulfur forms in organic substrates affecting S mineralization in soil
journal, June 2013

Sulfur Speciation in Soil by S K -Edge XANES Spectroscopy: Comparison of Spectral Deconvolution and Linear Combination Fitting
journal, April 2011

Bio-energy in the black
journal, September 2007

Transformation of Sulfur Species during Steam/Air Regeneration on a Ni Biomass Conditioning Catalyst
journal, June 2012

Sampling of Powders and Bulk Materials
book, January 1986

Decomposition of pyrite and trapping of sulphur in a coal matrix during pyrolysis of coal
journal, November 1984

Elucidation of Biomass Pyrolysis Products Using a Laminar Entrained Flow Reactor and Char Particle Imaging
journal, January 2011