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Title: Exploring two-dimensional electron gases with two-dimensional Fourier transform spectroscopy

The dephasing of excitons in a modulation doped single quantum well was carefully measured using time integrated four-wave mixing (FWM) and two-dimensional Fourier transform (2DFT) spectroscopy. These are the first 2DFT measurements performed on a modulation doped single quantum well. The inhomogeneous and homogeneous excitonic line widths were obtained from the diagonal and cross-diagonal profiles of the 2DFT spectra. The laser excitation density and temperature were varied and 2DFT spectra were collected. A very rapid increase of the dephasing decay, and as a result, an increase in the cross-diagonal 2DFT linewidths with temperature was observed. Furthermore, the lineshapes of the 2DFT spectra suggest the presence of excitation induced dephasing and excitation induced shift.
Authors:
 [1] ;  [1] ;  [2] ;  [3] ;  [2] ;  [1]
  1. Univ. of South Florida, Tampa, FL (United States)
  2. Univ. of Alabama at Birmingham, Birmingham, AL (United States)
  3. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Publication Date:
Report Number(s):
SAND-2013-4782J
Journal ID: ISSN 0021-9606; JCPSA6; 456279
Grant/Contract Number:
AC04-94AL85000
Type:
Accepted Manuscript
Journal Name:
Journal of Chemical Physics
Additional Journal Information:
Journal Volume: 141; Journal Issue: 13; Journal ID: ISSN 0021-9606
Publisher:
American Institute of Physics (AIP)
Research Org:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org:
USDOE National Nuclear Security Administration (NNSA)
Country of Publication:
United States
Language:
English
Subject:
77 NANOSCIENCE AND NANOTECHNOLOGY; quantum wells; four wave mixing; polarization; doping; dephasing
OSTI Identifier:
1083698
Alternate Identifier(s):
OSTI ID: 1223047

Paul, J., Dey, P., Tokumoto, T., Reno, J. L., Hilton, D. J., and Karaiskaj, D.. Exploring two-dimensional electron gases with two-dimensional Fourier transform spectroscopy. United States: N. p., Web. doi:10.1063/1.4896777.
Paul, J., Dey, P., Tokumoto, T., Reno, J. L., Hilton, D. J., & Karaiskaj, D.. Exploring two-dimensional electron gases with two-dimensional Fourier transform spectroscopy. United States. doi:10.1063/1.4896777.
Paul, J., Dey, P., Tokumoto, T., Reno, J. L., Hilton, D. J., and Karaiskaj, D.. 2014. "Exploring two-dimensional electron gases with two-dimensional Fourier transform spectroscopy". United States. doi:10.1063/1.4896777. https://www.osti.gov/servlets/purl/1083698.
@article{osti_1083698,
title = {Exploring two-dimensional electron gases with two-dimensional Fourier transform spectroscopy},
author = {Paul, J. and Dey, P. and Tokumoto, T. and Reno, J. L. and Hilton, D. J. and Karaiskaj, D.},
abstractNote = {The dephasing of excitons in a modulation doped single quantum well was carefully measured using time integrated four-wave mixing (FWM) and two-dimensional Fourier transform (2DFT) spectroscopy. These are the first 2DFT measurements performed on a modulation doped single quantum well. The inhomogeneous and homogeneous excitonic line widths were obtained from the diagonal and cross-diagonal profiles of the 2DFT spectra. The laser excitation density and temperature were varied and 2DFT spectra were collected. A very rapid increase of the dephasing decay, and as a result, an increase in the cross-diagonal 2DFT linewidths with temperature was observed. Furthermore, the lineshapes of the 2DFT spectra suggest the presence of excitation induced dephasing and excitation induced shift.},
doi = {10.1063/1.4896777},
journal = {Journal of Chemical Physics},
number = 13,
volume = 141,
place = {United States},
year = {2014},
month = {10}
}