You need JavaScript to view this

Resonant Impulsive Stimulated Raman Scattering

Abstract

Using a femtosecond dye laser, we observe in real-time vibrational oscillations excited by impulsive stimulated Raman scattering (ISRS) close to an electronic resonance. We perform single-beam Raman excitation and probe the driven coherence by a polarization-sensitive detection. We demonstrate for the first time impulsively Raman-induced dichroism, birefringence as well as frequency and time delay shifts. We analyse the characteristics of resonant ISRS on a vibrational mode of a dye molecule (malachite green) in solution.
Publication Date:
Mar 15, 1988
Product Type:
Journal Article
Reference Number:
FRD-88-001597; EDB-88-117943
Resource Relation:
Journal Name: Europhy. Lett.; (France); Journal Volume: 5:6
Subject:
74 ATOMIC AND MOLECULAR PHYSICS; MOLECULES; RAMAN EFFECT; EXCITATION; VIBRATIONAL STATES; ENERGY LEVELS; ENERGY-LEVEL TRANSITIONS; EXCITED STATES; 640302* - Atomic, Molecular & Chemical Physics- Atomic & Molecular Properties & Theory
OSTI ID:
7222314
Research Organizations:
Ecole Polytechnique, 91 - Palaiseau (France)
Country of Origin:
France
Language:
English
Other Identifying Numbers:
Journal ID: CODEN: EULEE
Submitting Site:
FRN
Size:
Pages: 523-528
Announcement Date:

Citation Formats

Mokhtari, A, and Chesnoy, J. Resonant Impulsive Stimulated Raman Scattering. France: N. p., 1988. Web. doi:10.1209/0295-5075/5/6/008.
Mokhtari, A, & Chesnoy, J. Resonant Impulsive Stimulated Raman Scattering. France. doi:10.1209/0295-5075/5/6/008.
Mokhtari, A, and Chesnoy, J. 1988. "Resonant Impulsive Stimulated Raman Scattering." France. doi:10.1209/0295-5075/5/6/008. https://www.osti.gov/servlets/purl/10.1209/0295-5075/5/6/008.
@misc{etde_7222314,
title = {Resonant Impulsive Stimulated Raman Scattering}
author = {Mokhtari, A, and Chesnoy, J}
abstractNote = {Using a femtosecond dye laser, we observe in real-time vibrational oscillations excited by impulsive stimulated Raman scattering (ISRS) close to an electronic resonance. We perform single-beam Raman excitation and probe the driven coherence by a polarization-sensitive detection. We demonstrate for the first time impulsively Raman-induced dichroism, birefringence as well as frequency and time delay shifts. We analyse the characteristics of resonant ISRS on a vibrational mode of a dye molecule (malachite green) in solution.}
doi = {10.1209/0295-5075/5/6/008}
journal = {Europhy. Lett.; (France)}
volume = {5:6}
journal type = {AC}
place = {France}
year = {1988}
month = {Mar}
}