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Sulphur dioxide removal by turbulent transfer over grass, snow, and water surfaces

Abstract

Vertical gradients of sulphur dioxide concentration have been measured over grass, snow, and water surfaces in order to assess the importance of these surfaces as SO/sub 2/ sinks. Concentrations were usually found to be lower near the surface indicating that removal occurs there. Vertical concentration gradients, normalized with repect to the concentration at 8 m, were generally greatest over water and least over snow, independent of meteorological conditions, suggesting that a water surface is the strongest SO/sub 2/ sink, with grass next, and snow weakest. The turbulent transfer of SO/sub 2/ to the interface is discussed in relation to stability of the lower atmosphere and physical and chemical properties of the surfaces. Using a bulk aerodynamic transfer approach similar to that for water vapour, values of SO/sub 2/ flux averaged over periods of from one to several hours were found to be of the order of 1 microgram/M/sup 2//S to the water and grass surfaces, and an order of magnitude smaller to the snow surface. Deposition velocities were found to be of the order of 1 cm/s.
Publication Date:
Jan 01, 1974
Product Type:
Journal Article
Reference Number:
EDB-84-150240
Resource Relation:
Journal Name: Tellus; (Sweden); Journal Volume: 26
Subject:
54 ENVIRONMENTAL SCIENCES; SULFUR DIOXIDE; ECOLOGICAL CONCENTRATION; AIR-WATER INTERACTIONS; DEPOSITION; GRASS; SINKS; SNOW; WATER; ATMOSPHERIC PRECIPITATIONS; CHALCOGENIDES; HYDROGEN COMPOUNDS; OXIDES; OXYGEN COMPOUNDS; PLANTS; SULFUR COMPOUNDS; SULFUR OXIDES; 500200* - Environment, Atmospheric- Chemicals Monitoring & Transport- (-1989)
OSTI ID:
6608829
Country of Origin:
Sweden
Language:
English
Other Identifying Numbers:
Journal ID: CODEN: TELLA
Submitting Site:
HEDB
Size:
Pages: 196-205
Announcement Date:
Aug 01, 1983

Citation Formats

Whelpdale, D M, and Shaw, R W. Sulphur dioxide removal by turbulent transfer over grass, snow, and water surfaces. Sweden: N. p., 1974. Web. doi:10.1111/j.2153-3490.1974.tb01967.x.
Whelpdale, D M, & Shaw, R W. Sulphur dioxide removal by turbulent transfer over grass, snow, and water surfaces. Sweden. https://doi.org/10.1111/j.2153-3490.1974.tb01967.x
Whelpdale, D M, and Shaw, R W. 1974. "Sulphur dioxide removal by turbulent transfer over grass, snow, and water surfaces." Sweden. https://doi.org/10.1111/j.2153-3490.1974.tb01967.x.
@misc{etde_6608829,
title = {Sulphur dioxide removal by turbulent transfer over grass, snow, and water surfaces}
author = {Whelpdale, D M, and Shaw, R W}
abstractNote = {Vertical gradients of sulphur dioxide concentration have been measured over grass, snow, and water surfaces in order to assess the importance of these surfaces as SO/sub 2/ sinks. Concentrations were usually found to be lower near the surface indicating that removal occurs there. Vertical concentration gradients, normalized with repect to the concentration at 8 m, were generally greatest over water and least over snow, independent of meteorological conditions, suggesting that a water surface is the strongest SO/sub 2/ sink, with grass next, and snow weakest. The turbulent transfer of SO/sub 2/ to the interface is discussed in relation to stability of the lower atmosphere and physical and chemical properties of the surfaces. Using a bulk aerodynamic transfer approach similar to that for water vapour, values of SO/sub 2/ flux averaged over periods of from one to several hours were found to be of the order of 1 microgram/M/sup 2//S to the water and grass surfaces, and an order of magnitude smaller to the snow surface. Deposition velocities were found to be of the order of 1 cm/s.}
doi = {10.1111/j.2153-3490.1974.tb01967.x}
journal = []
volume = {26}
journal type = {AC}
place = {Sweden}
year = {1974}
month = {Jan}
}