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Aircraft exhaust aerosol formation and growth

Abstract

Aerosol formation and growth in the exhaust plume of the ATTAS aircraft at an altitude of approximately 9 km, burning fuels with 2 ppmm sulfur (`low`) and 266 ppmm (`high`) sulfur has been modeled using an aerosol dynamics model for nucleation, vapor condensation and coagulation, coupled to a 2-dimensional, axisymmetric flow code to treat plume dilution and turbulent mixing. For both the `low` and `high` sulfur fuels, approximately 60% of the available water had condensed within the first 200 m downstream of the exhaust exit. The contrail particle diameters ranged between 0.4 to 1.6 {mu}m. However, the size distributions as a function of radial position for the `low` sulfur plume were broader than the corresponding distributions for the `high` sulfur plume. The model results indicate for a fuel sulfur mass loading of 2 ppmm, sulfuric acid remains a viable activating agent and that the differences in the contrail particle size distributions for sulfur mass loadings between 2 ppmm and 260 ppmm would be difficult to detect. (author) 12 refs.
Authors:
Brown, R C; Miake-Lye, R C; Anderson, M R; Kolb, C E [1] 
  1. Aerodyne Research, Inc., Billerica, MA (United States). Center for Chemical and Environmental Physics
Publication Date:
Dec 31, 1997
Product Type:
Conference
Report Number:
ONERA-97-Vol.1; CONF-9610234-
Reference Number:
SCA: 540120; 540110; PA: FRC-98:000124; EDB-98:075991; SN: 98001913098
Resource Relation:
Conference: International colloquium: Impact of aircraft emissions upon the atmosphere, Paris (France), 15-18 Oct 1996; Other Information: PBD: 1997; Related Information: Is Part Of Proceedings of impact of aircraft emissions upon the atmosphere. V. 1; PB: [381] p.
Subject:
54 ENVIRONMENTAL SCIENCES; AIRCRAFT; JET ENGINE FUELS; SULFUR; AEROSOLS; NUCLEATION; VAPOR CONDENSATION; PLUMES; PARTICLE SIZE; EXHAUST GASES; CONCENTRATION RATIO
OSTI ID:
623600
Research Organizations:
Office National d`Etudes et de Recherches Aerospatiales (ONERA), 92 - Chatillon (France)
Country of Origin:
France
Language:
English
Other Identifying Numbers:
Other: ON: DE98731902; TRN: FR9800124
Availability:
OSTI as DE98731902
Submitting Site:
FR
Size:
pp. 201-206
Announcement Date:
Jul 27, 1998

Citation Formats

Brown, R C, Miake-Lye, R C, Anderson, M R, and Kolb, C E. Aircraft exhaust aerosol formation and growth. France: N. p., 1997. Web.
Brown, R C, Miake-Lye, R C, Anderson, M R, & Kolb, C E. Aircraft exhaust aerosol formation and growth. France.
Brown, R C, Miake-Lye, R C, Anderson, M R, and Kolb, C E. 1997. "Aircraft exhaust aerosol formation and growth." France.
@misc{etde_623600,
title = {Aircraft exhaust aerosol formation and growth}
author = {Brown, R C, Miake-Lye, R C, Anderson, M R, and Kolb, C E}
abstractNote = {Aerosol formation and growth in the exhaust plume of the ATTAS aircraft at an altitude of approximately 9 km, burning fuels with 2 ppmm sulfur (`low`) and 266 ppmm (`high`) sulfur has been modeled using an aerosol dynamics model for nucleation, vapor condensation and coagulation, coupled to a 2-dimensional, axisymmetric flow code to treat plume dilution and turbulent mixing. For both the `low` and `high` sulfur fuels, approximately 60% of the available water had condensed within the first 200 m downstream of the exhaust exit. The contrail particle diameters ranged between 0.4 to 1.6 {mu}m. However, the size distributions as a function of radial position for the `low` sulfur plume were broader than the corresponding distributions for the `high` sulfur plume. The model results indicate for a fuel sulfur mass loading of 2 ppmm, sulfuric acid remains a viable activating agent and that the differences in the contrail particle size distributions for sulfur mass loadings between 2 ppmm and 260 ppmm would be difficult to detect. (author) 12 refs.}
place = {France}
year = {1997}
month = {Dec}
}