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Preparation of ultrafine iron particles by chemical vapor deposition of Fe(CO) sub 5. Fe(CO) sub 5 wo gebryo to suru kiso kagaku hanno ni yoru tetsuchobiryushi no seisei

Abstract

An ultrafine iron particle preparing process was developed, which wses gaseous phase pyrolysis in magnetic field of iron pentacarbonyl, Fe(CO){sub 5}, based on the fact that Fe(CO){sub 5} has peculiar characters that its boiling point is as low as 103{degree}C, and starts decomposing in a low temperature zone of 100{degree}C or lower. Vaporizing and introducing into a reactor an fe(CO){sub 5}, andPyrolyzing it at 200-600{degree}C while being diluted with nitrogen and applied with a magnetic field produced uitrafine iron particles of a necklace-like chain comprisinh primary particles having diameter of 15 to 25 nm with 10 to 40 of them linked in a straight chain. It was found that the specific surface area is 30-50 m{sup 2}/g, with the diameter converted from the specific surface area being relatively close to the average diameter obtained from TEM photograph, and that the particle has few pores. Magnetically the iron powder has a coercivity of 123-131 KA/m and a specific saturation magnetization of 120-140 Am{sup 2}/kg, and is expected to be applied as a high density magnetic recording medium. 5 refs.,8 figs., 3 tabs.
Publication Date:
Nov 10, 1991
Product Type:
Journal Article
Reference Number:
NEDO-91-914499; EDB-92-068738
Resource Relation:
Journal Name: Kagaku Kogaku Ronbunshu; (Japan); Journal Volume: 17:6
Subject:
36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY; IRON; CARBONYLS; DECOMPOSITION; VAPORS; PARTICULATES; CHAINS; COERCIVE FORCE; PARTICLE SIZE; PRODUCTION; SURFACE AREA; INERT ATMOSPHERE; MAGNETIC FIELDS; CHEMICAL REACTIONS; ELEMENTS; FLUIDS; GASES; METALS; PARTICLES; SIZE; SURFACE PROPERTIES; TRANSITION ELEMENTS; 360101* - Metals & Alloys- Preparation & Fabrication; 400800 - Combustion, Pyrolysis, & High-Temperature Chemistry
OSTI ID:
5636480
Country of Origin:
Japan
Language:
Japanese
Other Identifying Numbers:
Journal ID: ISSN 0386-216X; CODEN: KKRBA
Submitting Site:
NEDO
Size:
Pages: 1074-1079
Announcement Date:
May 15, 1992

Citation Formats

Sawada, Y, and Kageyama, Y. (Mitsubishi Petrochemical Co. Ltd., Tokyo (Japan)): Iwata, M. (Nagoya University, Nagoya (Japan). Faculty of Engineering). Preparation of ultrafine iron particles by chemical vapor deposition of Fe(CO) sub 5. Fe(CO) sub 5 wo gebryo to suru kiso kagaku hanno ni yoru tetsuchobiryushi no seisei. Japan: N. p., 1991. Web.
Sawada, Y, & Kageyama, Y. (Mitsubishi Petrochemical Co. Ltd., Tokyo (Japan)): Iwata, M. (Nagoya University, Nagoya (Japan). Faculty of Engineering). Preparation of ultrafine iron particles by chemical vapor deposition of Fe(CO) sub 5. Fe(CO) sub 5 wo gebryo to suru kiso kagaku hanno ni yoru tetsuchobiryushi no seisei. Japan.
Sawada, Y, and Kageyama, Y. (Mitsubishi Petrochemical Co. Ltd., Tokyo (Japan)): Iwata, M. (Nagoya University, Nagoya (Japan). Faculty of Engineering). 1991. "Preparation of ultrafine iron particles by chemical vapor deposition of Fe(CO) sub 5. Fe(CO) sub 5 wo gebryo to suru kiso kagaku hanno ni yoru tetsuchobiryushi no seisei." Japan.
@misc{etde_5636480,
title = {Preparation of ultrafine iron particles by chemical vapor deposition of Fe(CO) sub 5. Fe(CO) sub 5 wo gebryo to suru kiso kagaku hanno ni yoru tetsuchobiryushi no seisei}
author = {Sawada, Y, and Kageyama, Y. (Mitsubishi Petrochemical Co. Ltd., Tokyo (Japan)): Iwata, M. (Nagoya University, Nagoya (Japan). Faculty of Engineering)}
abstractNote = {An ultrafine iron particle preparing process was developed, which wses gaseous phase pyrolysis in magnetic field of iron pentacarbonyl, Fe(CO){sub 5}, based on the fact that Fe(CO){sub 5} has peculiar characters that its boiling point is as low as 103{degree}C, and starts decomposing in a low temperature zone of 100{degree}C or lower. Vaporizing and introducing into a reactor an fe(CO){sub 5}, andPyrolyzing it at 200-600{degree}C while being diluted with nitrogen and applied with a magnetic field produced uitrafine iron particles of a necklace-like chain comprisinh primary particles having diameter of 15 to 25 nm with 10 to 40 of them linked in a straight chain. It was found that the specific surface area is 30-50 m{sup 2}/g, with the diameter converted from the specific surface area being relatively close to the average diameter obtained from TEM photograph, and that the particle has few pores. Magnetically the iron powder has a coercivity of 123-131 KA/m and a specific saturation magnetization of 120-140 Am{sup 2}/kg, and is expected to be applied as a high density magnetic recording medium. 5 refs.,8 figs., 3 tabs.}
journal = []
volume = {17:6}
journal type = {AC}
place = {Japan}
year = {1991}
month = {Nov}
}