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Crown ethers as size-selective synergists in solvent extraction systems: a new selectivity parameter

Abstract

Mixtures of macrocyclic polyethers (crown ethers) and organic-phase-soluble liquid cation exchangers have been found to produce a synergistic effect in the extraction of metal ions. The synergistic effect is size selective; that is, it tends to be greatest for those ions that best fit the crown ether cavity. The mixtures of a liquid cation exchanger and a crown ether also allow metal ion extraction from common mineral-acid anion systems (NO/sub 3//sup -/, Cl/sup -/, SO/sub 4//sup 2 -/) that would be impossible with the crown ether alone, because of the difficulty of solubilizing those anions in nonpolar solvents. This cooperation makes the use of crown ethers as size-selective coordinators available for process applications. Size selectivity of compounds such as crown ethers may thus become a useful new parameter in designing selective solvent extraction systems. Results are reported for alkali (including Cs) and alkaline earth (including Sr) extraction by HDEHP mixed with various crown ethers.
Authors:
Kinard, W F; McDowell, W J [1] 
  1. Oak Ridge National Lab., TN (USA)
Publication Date:
Jan 01, 1981
Product Type:
Journal Article
Reference Number:
AIX-13-661054; ERA-07-032218; EDB-82-078338
Resource Relation:
Journal Name: J. Inorg. Nucl. Chem.; (United Kingdom); Journal Volume: 43:11
Subject:
37 INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY; CESIUM; SOLVENT EXTRACTION; CHLORIDES; SOLVENT PROPERTIES; HDEHP; NITRATES; POLYETHYLENE GLYCOLS; SYNERGISM; STRONTIUM; SULFATES; DISTRIBUTION FUNCTIONS; MIXTURES; SIZE; ALCOHOLS; ALKALI METALS; ALKALINE EARTH METALS; CHLORINE COMPOUNDS; DISPERSIONS; ELEMENTS; ESTERS; EXTRACTION; FUNCTIONS; GLYCOLS; HALIDES; HALOGEN COMPOUNDS; HYDROXY COMPOUNDS; METALS; NITROGEN COMPOUNDS; ORGANIC COMPOUNDS; ORGANIC PHOSPHORUS COMPOUNDS; ORGANIC POLYMERS; OXYGEN COMPOUNDS; PHOSPHORIC ACID ESTERS; POLYMERS; SEPARATION PROCESSES; SULFUR COMPOUNDS; 400301* - Organic Chemistry- Chemical & Physicochemical Properties- (-1987); 400201 - Chemical & Physicochemical Properties; 400105 - Separation Procedures
OSTI ID:
5582011
Country of Origin:
United Kingdom
Language:
English
Other Identifying Numbers:
Journal ID: CODEN: JINCA
Submitting Site:
INIS
Size:
Pages: 2947-2953
Announcement Date:
Mar 01, 1982

Citation Formats

Kinard, W F, and McDowell, W J. Crown ethers as size-selective synergists in solvent extraction systems: a new selectivity parameter. United Kingdom: N. p., 1981. Web. doi:10.1016/0022-1902(81)80648-3.
Kinard, W F, & McDowell, W J. Crown ethers as size-selective synergists in solvent extraction systems: a new selectivity parameter. United Kingdom. https://doi.org/10.1016/0022-1902(81)80648-3
Kinard, W F, and McDowell, W J. 1981. "Crown ethers as size-selective synergists in solvent extraction systems: a new selectivity parameter." United Kingdom. https://doi.org/10.1016/0022-1902(81)80648-3.
@misc{etde_5582011,
title = {Crown ethers as size-selective synergists in solvent extraction systems: a new selectivity parameter}
author = {Kinard, W F, and McDowell, W J}
abstractNote = {Mixtures of macrocyclic polyethers (crown ethers) and organic-phase-soluble liquid cation exchangers have been found to produce a synergistic effect in the extraction of metal ions. The synergistic effect is size selective; that is, it tends to be greatest for those ions that best fit the crown ether cavity. The mixtures of a liquid cation exchanger and a crown ether also allow metal ion extraction from common mineral-acid anion systems (NO/sub 3//sup -/, Cl/sup -/, SO/sub 4//sup 2 -/) that would be impossible with the crown ether alone, because of the difficulty of solubilizing those anions in nonpolar solvents. This cooperation makes the use of crown ethers as size-selective coordinators available for process applications. Size selectivity of compounds such as crown ethers may thus become a useful new parameter in designing selective solvent extraction systems. Results are reported for alkali (including Cs) and alkaline earth (including Sr) extraction by HDEHP mixed with various crown ethers.}
doi = {10.1016/0022-1902(81)80648-3}
journal = []
volume = {43:11}
journal type = {AC}
place = {United Kingdom}
year = {1981}
month = {Jan}
}