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Occurrence and retention of radionuclides in the sediments of White Oak Lake

Abstract

As a result of the discharges of large volumes of low-level radioactive liquid wastes to surface streams at the Oak Ridge National Laboratory, large quantities of radionuclides have accumulated in the bottom sediments of White Oak Lake. Ruthenium-106 (1038 C) and cesium-137 (704 C) account for more than 90% of the total activity now present at the site, while /sup 60/Co(152 C), the rare earths (17 C, exclusive of /sup 90/Y), and /sup 90/Sr(15 C) make up the remainder. More than half of the activity is associated with the upper 6-in. sediment layer, while progressively smaller quantities of activity are found with depth. The ruthenium, which is restricted to a small area in the now dry upper lake bed, is partially water soluble; however, its rate of movement through the soil is slow enough so that radioactive decay reduces the concentration of that reaching surface streams to insignificant levels. Most of the /sup 137/Cs occupies highly selective exchange sites on the illitic fraction of the clay in the sediment and can be desorbed only by disruption of the lattice structure. Only a small fraction of the /sup 60/Co in the soil was found to be exchangeable. It is, therefore, unlikely  More>>
Publication Date:
Jun 01, 1965
Product Type:
Journal Article
Reference Number:
EDB-82-079207
Resource Relation:
Journal Name: Health Phys.; (United Kingdom); Journal Volume: 11
Subject:
54 ENVIRONMENTAL SCIENCES; LAKES; SEDIMENTS; ORNL; RADIOACTIVE WASTE DISPOSAL; RADIOISOTOPES; RADIOECOLOGICAL CONCENTRATION; RADIONUCLIDE MIGRATION; CESIUM 137; COBALT 60; LIQUID WASTES; RUTHENIUM 106; SPATIAL DISTRIBUTION; STRONTIUM 90; ALKALI METAL ISOTOPES; ALKALINE EARTH ISOTOPES; BETA DECAY RADIOISOTOPES; BETA-MINUS DECAY RADIOISOTOPES; CESIUM ISOTOPES; COBALT ISOTOPES; DISTRIBUTION; ECOLOGICAL CONCENTRATION; ENVIRONMENTAL TRANSPORT; EVEN-EVEN NUCLEI; INTERMEDIATE MASS NUCLEI; INTERNAL CONVERSION RADIOISOTOPES; ISOMERIC TRANSITION ISOTOPES; ISOTOPES; MANAGEMENT; MASS TRANSFER; MINUTES LIVING RADIOISOTOPES; NATIONAL ORGANIZATIONS; NUCLEI; ODD-EVEN NUCLEI; ODD-ODD NUCLEI; RUTHENIUM ISOTOPES; STRONTIUM ISOTOPES; SURFACE WATERS; US AEC; US DOE; US ERDA; US ORGANIZATIONS; WASTE DISPOSAL; WASTE MANAGEMENT; WASTES; YEARS LIVING RADIOISOTOPES; 520302* - Environment, Aquatic- Radioactive Materials Monitoring & Transport- Aquatic Ecosystems & Food Chains- (-1987)
OSTI ID:
5505457
Research Organizations:
Oak Ridge National Lab., TN
Country of Origin:
United Kingdom
Language:
English
Other Identifying Numbers:
Journal ID: CODEN: HLTPA
Submitting Site:
ORNL
Size:
Pages: 567-577
Announcement Date:
May 01, 1982

Citation Formats

Lomenick, T F, and Gardiner, D A. Occurrence and retention of radionuclides in the sediments of White Oak Lake. United Kingdom: N. p., 1965. Web.
Lomenick, T F, & Gardiner, D A. Occurrence and retention of radionuclides in the sediments of White Oak Lake. United Kingdom.
Lomenick, T F, and Gardiner, D A. 1965. "Occurrence and retention of radionuclides in the sediments of White Oak Lake." United Kingdom.
@misc{etde_5505457,
title = {Occurrence and retention of radionuclides in the sediments of White Oak Lake}
author = {Lomenick, T F, and Gardiner, D A}
abstractNote = {As a result of the discharges of large volumes of low-level radioactive liquid wastes to surface streams at the Oak Ridge National Laboratory, large quantities of radionuclides have accumulated in the bottom sediments of White Oak Lake. Ruthenium-106 (1038 C) and cesium-137 (704 C) account for more than 90% of the total activity now present at the site, while /sup 60/Co(152 C), the rare earths (17 C, exclusive of /sup 90/Y), and /sup 90/Sr(15 C) make up the remainder. More than half of the activity is associated with the upper 6-in. sediment layer, while progressively smaller quantities of activity are found with depth. The ruthenium, which is restricted to a small area in the now dry upper lake bed, is partially water soluble; however, its rate of movement through the soil is slow enough so that radioactive decay reduces the concentration of that reaching surface streams to insignificant levels. Most of the /sup 137/Cs occupies highly selective exchange sites on the illitic fraction of the clay in the sediment and can be desorbed only by disruption of the lattice structure. Only a small fraction of the /sup 60/Co in the soil was found to be exchangeable. It is, therefore, unlikely that any large fraction of the /sup 137/Cs or /sup 60/Co would move from the area except through erosion of the sediment. About one-half of the /sup 90/Sr and the rare earths in the sediment appears to be exchangeable, while the other half is in the form of slightly soluble salts. Through leaching by ground water, a slow depletion of strontium from the dry part of the lake bed occurs. The accumulation of radionuclides in the sediments of White Oak Lake illustrates the effectiveness of relatively quiescent bodies of water in concentrating activity in stream beds and in retarding the downstream movement of these materials.}
journal = []
volume = {11}
journal type = {AC}
place = {United Kingdom}
year = {1965}
month = {Jun}
}