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Experiments to investigate the effects of small changes in fuel stoichiometry on fission gas release

Abstract

Fuel pin failure in-reactor leads to fission product and in the case of a PWR fuel debris release to the coolant. For economic reasons immediate shutdown and discharge of failed fuel needs to be avoided but this needs to be counter-balanced against the increasing dose to operators. PWR practice is to continue running wit failed rods, monitoring coolant activity, and only shutting down the reactor and discharging the fuel when circuit activity levels become unacceptable. The rate of fission product release under failed fuel conditions is of key importance and considerable effort has been directed towards establishing the dependency of release on temperature, heating rate, burn-up, and also the extent of fuel oxidation. As a precursor to a possible wider investigation of this area, a small programme was mounted during 1992/1993 to confirm whether small changes in the oxidation state of the fuel, for example those caused by minor cladding defects, would significantly effect fuel behaviour during postulated design basis faults. The objective of the programme was to determine the effects of small departures from stoichiometric fuel composition on fission gas release, and to compare the results with the current methodology for calculating releases under fault conditions. A total of  More>>
Authors:
Copeland, P S; Smith, R C [1] 
  1. Windscale Lab., AEA Technology, Seascale, Cumbria (United Kingdom)
Publication Date:
Aug 01, 1997
Product Type:
Technical Report
Report Number:
IAEA-TECDOC-957; CONF-9409411-
Reference Number:
SCA: 210200; PA: AIX-28:068470; EDB-97:129937; SN: 97001863076
Resource Relation:
Conference: IAEA technical committee meeting on water reactor fuel element modelling at high burnup and its experimental support, Windermere (United Kingdom), 19-23 Sep 1994; Other Information: PBD: Aug 1997; Related Information: Is Part Of Water reactor fuel element modelling at high burnup and its experimental support. Proceedings of a technical committee meeting; PB: 559 p.
Subject:
21 NUCLEAR POWER REACTORS AND ASSOCIATED PLANTS; FISSION PRODUCT RELEASE; STOICHIOMETRY; FUEL PELLETS; OXIDATION; VARIATIONS; BURNUP; EXPERIMENTAL DATA; GASES; PWR TYPE REACTORS; TEMPERATURE DEPENDENCE
OSTI ID:
534364
Research Organizations:
International Atomic Energy Agency, Vienna (Austria)
Country of Origin:
IAEA
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 1011-4289; Other: ON: DE98602336; TRN: XA9744817068470
Availability:
INIS; OSTI as DE98602336
Submitting Site:
INIS
Size:
pp. 443-454
Announcement Date:
Oct 31, 1997

Citation Formats

Copeland, P S, and Smith, R C. Experiments to investigate the effects of small changes in fuel stoichiometry on fission gas release. IAEA: N. p., 1997. Web.
Copeland, P S, & Smith, R C. Experiments to investigate the effects of small changes in fuel stoichiometry on fission gas release. IAEA.
Copeland, P S, and Smith, R C. 1997. "Experiments to investigate the effects of small changes in fuel stoichiometry on fission gas release." IAEA.
@misc{etde_534364,
title = {Experiments to investigate the effects of small changes in fuel stoichiometry on fission gas release}
author = {Copeland, P S, and Smith, R C}
abstractNote = {Fuel pin failure in-reactor leads to fission product and in the case of a PWR fuel debris release to the coolant. For economic reasons immediate shutdown and discharge of failed fuel needs to be avoided but this needs to be counter-balanced against the increasing dose to operators. PWR practice is to continue running wit failed rods, monitoring coolant activity, and only shutting down the reactor and discharging the fuel when circuit activity levels become unacceptable. The rate of fission product release under failed fuel conditions is of key importance and considerable effort has been directed towards establishing the dependency of release on temperature, heating rate, burn-up, and also the extent of fuel oxidation. As a precursor to a possible wider investigation of this area, a small programme was mounted during 1992/1993 to confirm whether small changes in the oxidation state of the fuel, for example those caused by minor cladding defects, would significantly effect fuel behaviour during postulated design basis faults. The objective of the programme was to determine the effects of small departures from stoichiometric fuel composition on fission gas release, and to compare the results with the current methodology for calculating releases under fault conditions. A total of eight experiments was performed. Two were intended as baseline tests to provide a reference with which to compare the effect of oxidation state influenced behaviour with that of thermal effects. It was found that small changes in stoichiometry of {sup {approx}}1 x 10{sup -6} had little or no effect on release but that changes of {sup {approx}} 1 x 10{sup -4} were observed to increase the diffusion coefficient, for {sup 85}Kr, by up to an order of magnitude and hence greatly increase the release rate. The stoichiometry of the sample used in these tests was, for convenience, adjusted using He/H{sub 2}/H{sub 2}O atmospheres. (Abstract Truncated)}
place = {IAEA}
year = {1997}
month = {Aug}
}