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Further assessment of the chemical modelling of iodine in IMPAIR 3 code using ACE/RTF data

Abstract

This paper introduces the assessment of the computer code IMPAIR 3 (Iodine Matter Partitioning And Iodine Release) which simulates physical and chemical iodine processes in a LWR containment with one or more compartments under conditions relevant to a severe accident in a nuclear reactor. The first version was published in 1992 to replace both the multi-compartment code IMPAIR 2/M and the single-compartment code IMPAIR 2.2. IMPAIR 2.2 was restricted to a single pH value specified before programme execution and precluded any variation of pH or calculation of H{sup +} changes during program execution. This restriction is removed in IMPAIR 3. Results of the IMPAIR 2.2 assessment using ACE/RTF Test 2 and the acidic phase of Test 3 B data were presented at the 3rd CSNI Workshop. The purpose of the current assessment is to verify the IMPAIR 3 capability to follow the whole test duration with changing boundary conditions. Besides revisiting ACE/RTF Test 3B, Test 4 data were also used for the current assessment. A limited data analysis was conducted using the outcome of the current ACEX iodine work to understand the iodine behaviour observed during these tests. This paper presents comparisons of the predicted results with the test data.  More>>
Authors:
Cripps, R C; Guentay, S [1] 
  1. Paul Scherrer Inst. (PSI), Villigen (Switzerland)
Publication Date:
Dec 01, 1996
Product Type:
Technical Report
Report Number:
PSI-97-02; CONF-9606320-; NEA/CSNI/R(96)-6.
Reference Number:
SCA: 210100; 210200; 400201; PA: AIX-28:037520; EDB-97:078480; SN: 97001795997
Resource Relation:
Conference: 4. CSNI workshop on the chemistry of iodine in reactor safety, Wuerenlingen (Switzerland), 10-12 Jun 1996; Other Information: PBD: Dec 1996; Related Information: Is Part Of Proceedings of the 4. CSNI workshop on the chemistry of iodine in reactor safety; Guentay, S. [ed.] [Paul Scherrer Inst. (PSI), Villigen (Switzerland)]; PB: 716 p.
Subject:
21 NUCLEAR POWER REACTORS AND ASSOCIATED PLANTS; 40 CHEMISTRY; BWR TYPE REACTORS; REACTOR ACCIDENTS; I CODES; VALIDATION; IODINE; DEPOSITION; ORGANIC COMPOUNDS; PWR TYPE REACTORS; HYPOIODOUS ACID; PAINTS; STAINLESS STEELS; THEORETICAL DATA
OSTI ID:
481718
Research Organizations:
Paul Scherrer Inst. (PSI), Villigen (Switzerland)
Country of Origin:
Switzerland
Language:
English
Other Identifying Numbers:
Other: ON: DE97624048; TRN: CH9700216037520
Availability:
INIS; OSTI as DE97624048
Submitting Site:
CHN
Size:
pp. 437-456
Announcement Date:
Jun 23, 1997

Citation Formats

Cripps, R C, and Guentay, S. Further assessment of the chemical modelling of iodine in IMPAIR 3 code using ACE/RTF data. Switzerland: N. p., 1996. Web.
Cripps, R C, & Guentay, S. Further assessment of the chemical modelling of iodine in IMPAIR 3 code using ACE/RTF data. Switzerland.
Cripps, R C, and Guentay, S. 1996. "Further assessment of the chemical modelling of iodine in IMPAIR 3 code using ACE/RTF data." Switzerland.
@misc{etde_481718,
title = {Further assessment of the chemical modelling of iodine in IMPAIR 3 code using ACE/RTF data}
author = {Cripps, R C, and Guentay, S}
abstractNote = {This paper introduces the assessment of the computer code IMPAIR 3 (Iodine Matter Partitioning And Iodine Release) which simulates physical and chemical iodine processes in a LWR containment with one or more compartments under conditions relevant to a severe accident in a nuclear reactor. The first version was published in 1992 to replace both the multi-compartment code IMPAIR 2/M and the single-compartment code IMPAIR 2.2. IMPAIR 2.2 was restricted to a single pH value specified before programme execution and precluded any variation of pH or calculation of H{sup +} changes during program execution. This restriction is removed in IMPAIR 3. Results of the IMPAIR 2.2 assessment using ACE/RTF Test 2 and the acidic phase of Test 3 B data were presented at the 3rd CSNI Workshop. The purpose of the current assessment is to verify the IMPAIR 3 capability to follow the whole test duration with changing boundary conditions. Besides revisiting ACE/RTF Test 3B, Test 4 data were also used for the current assessment. A limited data analysis was conducted using the outcome of the current ACEX iodine work to understand the iodine behaviour observed during these tests. This paper presents comparisons of the predicted results with the test data. The code capabilities are demonstrated to focus on still unresolved modelling problems. The unclear behaviour observed in the gaseous molecular iodine behaviour and its inconclusive effect on the calculated behaviour in the acidic phase of the Test 4 and importance of the catalytic effect of stainless steel are also indicated. (author) 18 figs., 1 tab., 11 refs.}
place = {Switzerland}
year = {1996}
month = {Dec}
}