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Dispersion of sulphur in the northern hemisphere. A study with a 3-dimensional time-resolved model

Abstract

This thesis on atmospheric dispersion of sulphur presents a calculation of intercontinental transport of oxidized sulphur and allocates different contributions to sulphur background levels over Europe. It is found that a significant fraction of anthropogenic sulphur (AS) is transported out of continental boundaries thus affecting the background levels over major parts of the northern hemisphere. Over Europe, the contribution of AS from North America is similar in amount to that of Asian AS and natural sources from the North Atlantic Ocean. Although the yearly contribution of intercontinental transport to deposition of sulphur over Europe is quite small, it can be much more important over certain areas and seasons and is comparable to the contributions from individual European countries. The calculations are based on a three-dimensional Eulerian time-resolved model that describes sulphur dispersion in the atmosphere in connection with large-scale synoptic flows and agree well with observations. The thesis emphasizes the role of synoptic scale atmospheric motions in determining intercontinental transport of sulphur. It indicates the need to resolve individual cyclones and anticyclones in order to describe the dispersion and distribution of atmospheric sulphur in the northern hemisphere and stresses the value of comparing model calculations with observations, both in atmospheric  More>>
Authors:
Publication Date:
Dec 31, 1995
Product Type:
Thesis/Dissertation
Report Number:
NEI-NO-658
Reference Number:
SCA: 540120; PA: NW-96:005256; EDB-96:152249; NTS-97:003550; SN: 96001673576
Resource Relation:
Other Information: DN: Reprints of 4 previously printed papers are attached; TH: Thesis (Dr.Scient.); PBD: 1995
Subject:
54 ENVIRONMENTAL SCIENCES; ATMOSPHERIC CHEMISTRY; ENVIRONMENTAL TRANSPORT; SULFUR COMPOUNDS; DEPOSITION; LONG-RANGE TRANSPORT; MATHEMATICAL MODELS; COMPUTERIZED SIMULATION; AIR POLLUTION; NUMERICAL SOLUTION
OSTI ID:
377633
Research Organizations:
Oslo Univ. (Norway)
Country of Origin:
Norway
Language:
English
Other Identifying Numbers:
Other: ON: DE97703328; TRN: NO9605256
Availability:
OSTI as DE97703328
Submitting Site:
NW
Size:
160 p.
Announcement Date:
Oct 23, 1996

Citation Formats

Tarrason, L. Dispersion of sulphur in the northern hemisphere. A study with a 3-dimensional time-resolved model. Norway: N. p., 1995. Web.
Tarrason, L. Dispersion of sulphur in the northern hemisphere. A study with a 3-dimensional time-resolved model. Norway.
Tarrason, L. 1995. "Dispersion of sulphur in the northern hemisphere. A study with a 3-dimensional time-resolved model." Norway.
@misc{etde_377633,
title = {Dispersion of sulphur in the northern hemisphere. A study with a 3-dimensional time-resolved model}
author = {Tarrason, L}
abstractNote = {This thesis on atmospheric dispersion of sulphur presents a calculation of intercontinental transport of oxidized sulphur and allocates different contributions to sulphur background levels over Europe. It is found that a significant fraction of anthropogenic sulphur (AS) is transported out of continental boundaries thus affecting the background levels over major parts of the northern hemisphere. Over Europe, the contribution of AS from North America is similar in amount to that of Asian AS and natural sources from the North Atlantic Ocean. Although the yearly contribution of intercontinental transport to deposition of sulphur over Europe is quite small, it can be much more important over certain areas and seasons and is comparable to the contributions from individual European countries. The calculations are based on a three-dimensional Eulerian time-resolved model that describes sulphur dispersion in the atmosphere in connection with large-scale synoptic flows and agree well with observations. The thesis emphasizes the role of synoptic scale atmospheric motions in determining intercontinental transport of sulphur. It indicates the need to resolve individual cyclones and anticyclones in order to describe the dispersion and distribution of atmospheric sulphur in the northern hemisphere and stresses the value of comparing model calculations with observations, both in atmospheric chemistry studies and in climate applications. 260 refs., 50 figs., 17 tabs.}
place = {Norway}
year = {1995}
month = {Dec}
}