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ESR studies of N,H, and D atoms trapped in solid molecular N{sub 2} matrix; Issledovanie metodom EhPR atomov N,H i D, zakhvachennykh v matritse tverdogo molekulyarnogo azota

Abstract

Nitrogen, hydrogen and deuterium atoms are matrix-isolated in solid N{sub 2} by deposition from gas phase and studied by electron spin resonance (ESR). These atoms are found to be trapped at the substitutional position of the cryo crystal lattice. The ESR line-widths of the N atoms in the recorded spectra appear to be one-fourth as those cites by most authors. It is shown that a calculation is possible which gives a theoretical linewidth matching the experimental one. Two distinct types of matrix surrounding are possible for the substitutional nitrogen atoms, one of which being consistent with the non distorted N{sub 2} crystal lattice. Hydrogen and deuterium ESR linewidths are found to broaden due to the zero point vibration of the atoms. Spin-lattice relaxation times of N,H, and D atoms in solid N{sub 2} matrix are presented.
Authors:
Dmitriev, Yu A; Zhitnikov, R A [1] 
  1. AN SSSR, Leningrad (Russian Federation). Fiziko-Tekhnicheskij Inst
Publication Date:
Jan 01, 1998
Product Type:
Journal Article
Reference Number:
SCA: 665100; 664100; PA: AIX-30:010420; EDB-99:033118; SN: 99002069464
Resource Relation:
Journal Name: Fizika Nizkikh Temperatur; Journal Volume: 24; Journal Issue: 1; Other Information: PBD: Jan 1998
Subject:
66 PHYSICS; CRYSTAL LATTICES; DEUTERIUM; ELECTRON SPIN RESONANCE; HYDROGEN; HYPERFINE STRUCTURE; MATRIX ISOLATION; NITROGEN; SPIN-LATTICE RELAXATION; TEMPERATURE DEPENDENCE
OSTI ID:
318318
Country of Origin:
Ukraine
Language:
Russian
Other Identifying Numbers:
Journal ID: FNTAA5; ISSN 0132-6414; TRN: UA9900306010420
Submitting Site:
INIS
Size:
pp. 58-66
Announcement Date:
Mar 24, 1999

Citation Formats

Dmitriev, Yu A, and Zhitnikov, R A. ESR studies of N,H, and D atoms trapped in solid molecular N{sub 2} matrix; Issledovanie metodom EhPR atomov N,H i D, zakhvachennykh v matritse tverdogo molekulyarnogo azota. Ukraine: N. p., 1998. Web.
Dmitriev, Yu A, & Zhitnikov, R A. ESR studies of N,H, and D atoms trapped in solid molecular N{sub 2} matrix; Issledovanie metodom EhPR atomov N,H i D, zakhvachennykh v matritse tverdogo molekulyarnogo azota. Ukraine.
Dmitriev, Yu A, and Zhitnikov, R A. 1998. "ESR studies of N,H, and D atoms trapped in solid molecular N{sub 2} matrix; Issledovanie metodom EhPR atomov N,H i D, zakhvachennykh v matritse tverdogo molekulyarnogo azota." Ukraine.
@misc{etde_318318,
title = {ESR studies of N,H, and D atoms trapped in solid molecular N{sub 2} matrix; Issledovanie metodom EhPR atomov N,H i D, zakhvachennykh v matritse tverdogo molekulyarnogo azota}
author = {Dmitriev, Yu A, and Zhitnikov, R A}
abstractNote = {Nitrogen, hydrogen and deuterium atoms are matrix-isolated in solid N{sub 2} by deposition from gas phase and studied by electron spin resonance (ESR). These atoms are found to be trapped at the substitutional position of the cryo crystal lattice. The ESR line-widths of the N atoms in the recorded spectra appear to be one-fourth as those cites by most authors. It is shown that a calculation is possible which gives a theoretical linewidth matching the experimental one. Two distinct types of matrix surrounding are possible for the substitutional nitrogen atoms, one of which being consistent with the non distorted N{sub 2} crystal lattice. Hydrogen and deuterium ESR linewidths are found to broaden due to the zero point vibration of the atoms. Spin-lattice relaxation times of N,H, and D atoms in solid N{sub 2} matrix are presented.}
journal = []
issue = {1}
volume = {24}
journal type = {AC}
place = {Ukraine}
year = {1998}
month = {Jan}
}