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Occurrences of nitrosamines in chlorinated and chloraminated drinking water in three representative cities, China

Abstract

An investigation of the occurrence of nine nitrosamines in drinking water following different water treatment processes was conducted using samples from seven drinking water treatment plants in three cities and tap waters in one city in China. The total nitrosamine levels ranged from not detected (n.d.) to 43.45 ng/L. The species and concentrations of the nine nitrosamines varied with disinfection methods and source waters. N-nitrosodimethylamine (NDMA), which is the nitrosamines of greatest concern, was identified in raw water, disinfecting water, finished water and tap water samples, ranging from 0.8 to 21.6, 0.12 to 24.2, n.d. to 8.8, and n.d. to 13.3 ng/L, respectively. Chloramination alone produced the most significant amounts of NDMA, while ozonation followed by chloramination led to moderately reduced levels. Additionally, chlorination produced relatively less NDMA, while low pressure ultraviolet radiation followed by chlorination could also significantly reduce them. Total organic carbon is one of the most important factors influencing nitrosamines formation in disinfecting water. In contrast, the addition of chlorine following any other disinfection was found to increase the formation of the other eight species of nitrosamines. The three nitrosamines recommended for monitoring by the US EPA were detected in the tap water samples, but most were  More>>
Publication Date:
Oct 15, 2012
Product Type:
Journal Article
Resource Relation:
Journal Name: Science of the Total Environment; Journal Volume: 437; Other Information: Copyright (c) 2012 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
Subject:
54 ENVIRONMENTAL SCIENCES; BY-PRODUCTS; CHLORINATION; CHLORINE; CONCENTRATION RATIO; DRINKING WATER; ECOLOGICAL CONCENTRATION; HEALTH HAZARDS; NITROSAMINES; ORGANIC MATTER; PUBLIC HEALTH; URBAN AREAS; WATER TREATMENT
OSTI ID:
22192250
Country of Origin:
Netherlands
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0048-9697; CODEN: STENDL; Other: PII: S0048-9697(12)01094-7; TRN: NL13R7191016739
Availability:
Available from http://dx.doi.org/10.1016/j.scitotenv.2012.08.023
Submitting Site:
NLN
Size:
page(s) 219-225
Announcement Date:
Feb 20, 2014

Citation Formats

Luo, Qian, Wang, Donghong, and Wang, Zijian. Occurrences of nitrosamines in chlorinated and chloraminated drinking water in three representative cities, China. Netherlands: N. p., 2012. Web. doi:10.1016/J.SCITOTENV.2012.08.023.
Luo, Qian, Wang, Donghong, & Wang, Zijian. Occurrences of nitrosamines in chlorinated and chloraminated drinking water in three representative cities, China. Netherlands. https://doi.org/10.1016/J.SCITOTENV.2012.08.023
Luo, Qian, Wang, Donghong, and Wang, Zijian. 2012. "Occurrences of nitrosamines in chlorinated and chloraminated drinking water in three representative cities, China." Netherlands. https://doi.org/10.1016/J.SCITOTENV.2012.08.023.
@misc{etde_22192250,
title = {Occurrences of nitrosamines in chlorinated and chloraminated drinking water in three representative cities, China}
author = {Luo, Qian, Wang, Donghong, and Wang, Zijian}
abstractNote = {An investigation of the occurrence of nine nitrosamines in drinking water following different water treatment processes was conducted using samples from seven drinking water treatment plants in three cities and tap waters in one city in China. The total nitrosamine levels ranged from not detected (n.d.) to 43.45 ng/L. The species and concentrations of the nine nitrosamines varied with disinfection methods and source waters. N-nitrosodimethylamine (NDMA), which is the nitrosamines of greatest concern, was identified in raw water, disinfecting water, finished water and tap water samples, ranging from 0.8 to 21.6, 0.12 to 24.2, n.d. to 8.8, and n.d. to 13.3 ng/L, respectively. Chloramination alone produced the most significant amounts of NDMA, while ozonation followed by chloramination led to moderately reduced levels. Additionally, chlorination produced relatively less NDMA, while low pressure ultraviolet radiation followed by chlorination could also significantly reduce them. Total organic carbon is one of the most important factors influencing nitrosamines formation in disinfecting water. In contrast, the addition of chlorine following any other disinfection was found to increase the formation of the other eight species of nitrosamines. The three nitrosamines recommended for monitoring by the US EPA were detected in the tap water samples, but most were present at levels below those that pose a risk to human health. Nevertheless, the occurrence and concentration of nitrosamines regulated in the Drinking Water Contaminant Candidate List could cause some potential human effects and therefore warrant attention. Highlights: Black-Right-Pointing-Pointer Nitrosamines in disinfected drinking water in three Chinese cities were investigated. Black-Right-Pointing-Pointer Some nitrosamines could be detected in raw water. Black-Right-Pointing-Pointer Advanced treatment affects nitrosamine levels both positively and negatively. Black-Right-Pointing-Pointer Organic matters contribute to increased nitrosamine level. Black-Right-Pointing-Pointer Nitrosamine levels in this study were below the EPA MAC but are still significant.}
doi = {10.1016/J.SCITOTENV.2012.08.023}
journal = []
volume = {437}
journal type = {AC}
place = {Netherlands}
year = {2012}
month = {Oct}
}