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Retention in Solid KIO{sub 3} Activated with Fast and Slow Neutrons; Retention dans KIO{sub 3} Solide Active par des Neutrons Rapides et des Neutrons Lents; 0423 0414 0415 0420 0416 0410 041d 0418 0415 0412 0422 0412 0415 0420 0414 041e 041c KIO{sub 3}, 0410 041a 0422 0418 0412 0418 0420 041e 0412 0410 041d 041d 041e 041c 0411 042b 0421 0422 0420 042b 041c 0418 0418 041c 0415 0414 041b 0415 041d 041d 042b 041c 0418 041d 0415 0418 0422 0420 041e 041d 0410 041c 0418 ; Retencion en KIO{sub 3} Solido Activado con Neutrones Rapidos y Lentos

Conference:

Abstract

A simple model of recoil reactions in a solid would suggest that primary (unannealed) retention should demonstrate isotope effects (which would presumably be due to the way in which the product nucleus loses its excess nuclear energy), and that this quantity should be insensitive to the condition of the crystal lattice. On the other hand, annealing in this simple model should be dependent on the condition (and pretreatment) of the crystal, but show the same behaviour for different isotopes. A test for these arguments is provided by a series of experiments in which solid KIO{sub 3} was activated by means of fast and thermal neutrons. With fast neutrons the retention of I{sup 128} was appreciably higher than that of I{sup 126} but the retention of I{sup 128} obtained with thermal neutrons was even higher than that obtained with fast neutrons. This indicates that apart form the decay scheme the recoil energy may also constitute a factor determining the retention. The annealing of I{sup 128} and I{sup 126} (both obtained with fast neutrons) also proved to be different. Under post-irradiation treatment at temperatures up to 100 Degree-Sign C the retention of both isotopes increased by the same percentage of the total  More>>
Authors:
Aten, A.H.W. Jr.; Lindner-Groen, M.; Lindner, L. [1] 
  1. Instituut voor Kernphysisch Onderzoek, Amsterdam (Netherlands)
Publication Date:
Apr 15, 1965
Product Type:
Conference
Report Number:
IAEA-SM-57/31
Resource Relation:
Conference: Symposium on Chemical Effects Associated with Nuclear Reactions and Radioactive Transformations, Heidelberg (Germany), 7-11 Dec 1964; Other Information: 8 refs., 3 figs.; Related Information: In: Chemical Effects of Nuclear Transformations. Vol. II. Proceedings of the Symposium on Chemical Effects Associated with Nuclear Reactions and Radioactive Transformations| 572 p.
Subject:
36 MATERIALS SCIENCE; 38 RADIATION CHEMISTRY, RADIOCHEMISTRY AND NUCLEAR CHEMISTRY; ANNEALING; CRYSTAL LATTICES; CRYSTALS; FAST NEUTRONS; HEATING; IODINE 126; IODINE 128; IRRADIATION; ISOTOPE EFFECTS; RECOILS; RETENTION; SLOW NEUTRONS; THERMAL NEUTRONS
OSTI ID:
22184021
Research Organizations:
International Atomic Energy Agency, Vienna (Austria); Joint Commission on Applied Radioactivity of the International Council of Scientific Unions, Paris (France)
Country of Origin:
IAEA
Language:
English
Other Identifying Numbers:
Other: ISSN 0074-1884; TRN: XA13M3325008556
Submitting Site:
INIS
Size:
page(s) 125-131
Announcement Date:
Jan 30, 2014

Conference:

Citation Formats

Aten, A.H.W. Jr., Lindner-Groen, M., and Lindner, L. Retention in Solid KIO{sub 3} Activated with Fast and Slow Neutrons; Retention dans KIO{sub 3} Solide Active par des Neutrons Rapides et des Neutrons Lents; 0423 0414 0415 0420 0416 0410 041d 0418 0415 0412 0422 0412 0415 0420 0414 041e 041c KIO{sub 3}, 0410 041a 0422 0418 0412 0418 0420 041e 0412 0410 041d 041d 041e 041c 0411 042b 0421 0422 0420 042b 041c 0418 0418 041c 0415 0414 041b 0415 041d 041d 042b 041c 0418 041d 0415 0418 0422 0420 041e 041d 0410 041c 0418 ; Retencion en KIO{sub 3} Solido Activado con Neutrones Rapidos y Lentos. IAEA: N. p., 1965. Web.
Aten, A.H.W. Jr., Lindner-Groen, M., & Lindner, L. Retention in Solid KIO{sub 3} Activated with Fast and Slow Neutrons; Retention dans KIO{sub 3} Solide Active par des Neutrons Rapides et des Neutrons Lents; 0423 0414 0415 0420 0416 0410 041d 0418 0415 0412 0422 0412 0415 0420 0414 041e 041c KIO{sub 3}, 0410 041a 0422 0418 0412 0418 0420 041e 0412 0410 041d 041d 041e 041c 0411 042b 0421 0422 0420 042b 041c 0418 0418 041c 0415 0414 041b 0415 041d 041d 042b 041c 0418 041d 0415 0418 0422 0420 041e 041d 0410 041c 0418 ; Retencion en KIO{sub 3} Solido Activado con Neutrones Rapidos y Lentos. IAEA.
Aten, A.H.W. Jr., Lindner-Groen, M., and Lindner, L. 1965. "Retention in Solid KIO{sub 3} Activated with Fast and Slow Neutrons; Retention dans KIO{sub 3} Solide Active par des Neutrons Rapides et des Neutrons Lents; 0423 0414 0415 0420 0416 0410 041d 0418 0415 0412 0422 0412 0415 0420 0414 041e 041c KIO{sub 3}, 0410 041a 0422 0418 0412 0418 0420 041e 0412 0410 041d 041d 041e 041c 0411 042b 0421 0422 0420 042b 041c 0418 0418 041c 0415 0414 041b 0415 041d 041d 042b 041c 0418 041d 0415 0418 0422 0420 041e 041d 0410 041c 0418 ; Retencion en KIO{sub 3} Solido Activado con Neutrones Rapidos y Lentos." IAEA.
@misc{etde_22184021,
title = {Retention in Solid KIO{sub 3} Activated with Fast and Slow Neutrons; Retention dans KIO{sub 3} Solide Active par des Neutrons Rapides et des Neutrons Lents; 0423 0414 0415 0420 0416 0410 041d 0418 0415 0412 0422 0412 0415 0420 0414 041e 041c KIO{sub 3}, 0410 041a 0422 0418 0412 0418 0420 041e 0412 0410 041d 041d 041e 041c 0411 042b 0421 0422 0420 042b 041c 0418 0418 041c 0415 0414 041b 0415 041d 041d 042b 041c 0418 041d 0415 0418 0422 0420 041e 041d 0410 041c 0418 ; Retencion en KIO{sub 3} Solido Activado con Neutrones Rapidos y Lentos}
author = {Aten, A.H.W. Jr., Lindner-Groen, M., and Lindner, L.}
abstractNote = {A simple model of recoil reactions in a solid would suggest that primary (unannealed) retention should demonstrate isotope effects (which would presumably be due to the way in which the product nucleus loses its excess nuclear energy), and that this quantity should be insensitive to the condition of the crystal lattice. On the other hand, annealing in this simple model should be dependent on the condition (and pretreatment) of the crystal, but show the same behaviour for different isotopes. A test for these arguments is provided by a series of experiments in which solid KIO{sub 3} was activated by means of fast and thermal neutrons. With fast neutrons the retention of I{sup 128} was appreciably higher than that of I{sup 126} but the retention of I{sup 128} obtained with thermal neutrons was even higher than that obtained with fast neutrons. This indicates that apart form the decay scheme the recoil energy may also constitute a factor determining the retention. The annealing of I{sup 128} and I{sup 126} (both obtained with fast neutrons) also proved to be different. Under post-irradiation treatment at temperatures up to 100 Degree-Sign C the retention of both isotopes increased by the same percentage of the total activity, i.e. the difference in retention remained constant. Thus the fraction of the I{sup 126} which is reduced by the recoil process in excess of the reduced fraction of I{sup 128} is much less affected by heating than the fraction which is reduced in both isotopes. It is evident that such complicated chemical behaviour of the radioactive recoil atom can only be explained by a fairly detailed model. (author) [French] Un modele simple de reactions de recul dans un solide donnerait a penser que la retention primaire (sans recuit) devrait manifester des effets isotopiques (probablement dus a la maniere dont le noyau du produit perd son excedent d'energie nucleaire) et que cette valeur devrait etre independante de l'etat du reseau cristallin. En revanche, dans ce modele simple, le recuit devrait etre fonction de l'etat (et du traitement prealable) du cristal, mais devrait se comporter de la meme facon pour differents isotopes. A l'appui de ces arguments, on peut citer une serie d'experiences pour lesquelles KIO{sub 3} solide a ete active au moyen de neutrons thermiques et de neutrons rapides. Avec des neutrons rapides, la retention de {sup 128}I a ete notablement plus elevee que celle de {sup 126}I, mais la retention de {sup 128}I obtenue a l'aide de neutrons thermiques est encore superieure a celle obtenue au moyen de neutrons rapides. Ces resultats montrent qu'independamment de la decroissance, l'energie de recul peut aussi etre un facteur dont depend la retention. Le recuit de {sup 128}I et celui de {sup 126}I (obtenus tous deux a l'aide de neutrons rapides) s'averent etre egalement differents. Lorsque les deux radioisotopes ont ete traites apres irradiation a des temperatures allant jusqu'a 100 Degree-Sign C, leur retention a augmente dans la meme proportion que l'activite totale, c'est-a-dire que la difference de retention est restee constante. Ainsi, la fraction de {sup 128}I reduite par le processus de recul qui est en exces par rapport a la fraction de {sup 126}I reduite est beaucoup moins influencee par le chauffage que ne l'est la fraction qui est reduite dans les deux radioisotopes a la fois. Il est evident qu'un comportement chimique aussi complique de l'atome chaud de recul ne peut etre explique que par un modele tres detaille. (author) [Spanish] La aplicacion de un modelo simple de reaccion de retroceso en un solido sugiere que la retencion primaria (sin recocido) deberia reflejar los efectos isotopicos (que dependerian probablemente de la forma en que el nucleo producido pierde su exceso de energia nuclear), y que esta cantidad deberia ser independiente del estado de la red cristalina. En cambio, la regeneracion por recocido en este modelo simple deberia depender del estado (y tratamiento previo) del cristal, y presentar caracteristicas identicas para los diferentes isotopos. Para comprobar estas hipotesis se ha realizado una serie de experimentos en los que se activo KIO{sub 3} solido con neutrones rapidos y termicos. En el caso de los neutrones rapidos, la retencion de {sup 128}I fue sensiblemente mayor que la de {sup 126}I, pero la retencion de {sup 128}I alcanzada con los neutrones termicos fue aun mas elevada que la obtenida con los neutrones rapidos. Este hecho indica que, aparte del esquema de desintegracion, la energia de retroceso tambien puede constituir un factor determinante de la retencion. Tambien difieren los efectos del recocido en el {sup 128}I y en el {sup 126}I (obtenidos ambos con neutrones rapidos). Por tratamiento postirradiatorio a temperaturas de hasta 100 Degree-Sign C, la retencion de ambos isotopos referida a la actividad total aumento en la misma proporcion, esto es, la diferencia de retencion permanecio constante. Por tanto, la parte de la fraccion de {sup 126}I reducida por el proceso de retroceso que excede de la fraccion de {sup 128}I reducida, resulta mucho menos afectada por el calentamiento que la fraccion reducida de ambos isotopos. Es evidente que solo un modelo bastante detallado permite explicar ese comportamiento quimico tan complicado del atomo radiactivo de retroceso. (author) [Russian] Prostaja model' vzaimodejstvij jader otdachi v tverdom tele predpolagaet, chto osnovnoe (neotozhzhennoe) uderzhanie dolzhno pokazat' izotopnye jeffekty (kotorye, verojatno, byli by svjazany so sposobom poteri jadrom produkta svoej izbytochnoj jadernoj jenergii) i chto jeto kolichestvo dolzhno byt' nechuvstvitel'nym k usloviju kristallicheskoj reshetki. S drugoj storony, otzhig v jetoj prostoj modeli dolzhen zaviset' ot uslovija (i predvaritel'noj obrabotki) kristalla, no pokazyvat' to zhe samoe povedenie dlja razlichnyh izotopov . Proverka jetih argumentov daetsja posredstvom provedenija serii opytov, v kotoryh tverdyj KJO{sub 3} aktivirovalsja s pomoshh'ju bystryh i teplovyh nejtronov. Pri bystryh nejtronah uderzhanie joda-128 bylo znachitel'no vyshe, chem uderzhanie joda-126, no uderzhanie joda-128 s pomoshh'ju teplovyh nejtronov bylo dazhe vyshe, chem uderzhanie, poluchennoe s pomoshh'ju bystryh nejtronov. Jeto ukazyvaet, chto, pomimo shemy raspada, jenergija otdachi mozhet takzhe sostavljat' faktor, opredeljajushhij uderzhanie. Otzhig joda-128 i Joda-126 (oba polucheny s pomoshh'ju bystryh nejtronov) takzhe okazalsja razlichnym. Pri obrabotke posle obluchenija pri temperaturah do 100 Degree-Sign C uderzhanie oboih izotopov vozrastalo na odin i tot zhe procent obshhej aktivnosti, t.e. raznica v uderzhanii ostavalas' postojannoj. Takim obrazom frakcija joda-126, kotoraja umen'shalas' processom otdachi, bol'she umen'shennoj frakcii joda-128, znachitel'no men'she podvergalas' vozdejstviju nagreva, chem frakcija, kotoraja umen'shaetsja v oboih izotopah. Ochevidno, chto takoe slozhnoe himicheskoe povedenie radioaktivnogo atoma otdachi mozhno ob{sup j}asnit' tol'ko s pomoshh'ju dostatochnoj detal'noj modeli. (author)}
place = {IAEA}
year = {1965}
month = {Apr}
}