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Highly stable and efficient Ag/AgCl-TiO{sub 2} photocatalyst: Preparation, characterization, and application in the treatment of aqueous hazardous pollutants

Abstract

Graphical abstract: A new plasmonic photocatalyst of Ag-AgCl/TiO{sub 2} was prepared by deposition-precipitation and photoreduction. This photocatalyst exhibited efficient photocatalytic activity for the degradation of 4-chlorophenol and photoreduction Cr(VI) under visible light irradiation. Highlights: Black-Right-Pointing-Pointer The preparation procedure for Ag-AgCl/TiO{sub 2} was convenient and feasible. Black-Right-Pointing-Pointer Ag-AgCl/TiO{sub 2} was very efficient under visible-light irradiation. Black-Right-Pointing-Pointer Ag-AgCl/TiO{sub 2} can photodegrade 4-chlorophenol and Cr(VI) effectively. Black-Right-Pointing-Pointer The surface plasmon resonance effect of Ag{sup 0} nanoparticles played a key role. - Abstract: A new plasmonic photocatalyst of Ag-AgCl-TiO{sub 2} was prepared by deposition-precipitation and photoreduction. This photocatalyst exhibited efficient photocatalytic activity for the degradation of 4-chlorophenol and photoreduction of Cr(VI) ion under visible light irradiation. Its high photocatalytic activity can be attributed to the surface plasmon resonance effect of Ag nanoparticles, which were highly dispersed on the surface of Ag-AgCl-TiO{sub 2}. N{sub 2} adsorption and desorption isotherm spectra, X-ray diffraction, X-ray photoelectron spectroscopy, and transmission electron microscopy were used to determine the correlation between the micro-structure and the catalytic properties of the as-prepared photocatalysts.
Authors:
Guo, Jian-Feng; Ma, Bowen; Yin, Anyuan; Fan, Kangnian; [1]  Dai, Wei-Lin [1] 
  1. Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, Shanghai 200433 (China)
Publication Date:
Apr 15, 2012
Product Type:
Journal Article
Resource Relation:
Journal Name: Journal of Hazardous Materials; Journal Volume: 211-212; Other Information: Copyright (c) 2011 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
Subject:
37 INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY; ADSORPTION; DESORPTION; IRRADIATION; ISOTHERMS; MICROSTRUCTURE; NANOSTRUCTURES; PARTICLES; PHOTOCATALYSIS; POLLUTANTS; SILVER CHLORIDES; SPECTRA; SURFACES; TITANIUM OXIDES; TRANSMISSION ELECTRON MICROSCOPY; X-RAY DIFFRACTION; X-RAY PHOTOELECTRON SPECTROSCOPY
OSTI ID:
22154057
Country of Origin:
Netherlands
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0304-3894; CODEN: JHMAD9; Other: PII: S0304-3894(11)01462-2; TRN: NL12S2025108191
Availability:
Available from http://dx.doi.org/10.1016/j.jhazmat.2011.11.082
Submitting Site:
NLN
Size:
page(s) 77-82
Announcement Date:
Nov 21, 2013

Citation Formats

Guo, Jian-Feng, Ma, Bowen, Yin, Anyuan, Fan, Kangnian, and Dai, Wei-Lin. Highly stable and efficient Ag/AgCl-TiO{sub 2} photocatalyst: Preparation, characterization, and application in the treatment of aqueous hazardous pollutants. Netherlands: N. p., 2012. Web. doi:10.1016/J.JHAZMAT.2011.11.082.
Guo, Jian-Feng, Ma, Bowen, Yin, Anyuan, Fan, Kangnian, & Dai, Wei-Lin. Highly stable and efficient Ag/AgCl-TiO{sub 2} photocatalyst: Preparation, characterization, and application in the treatment of aqueous hazardous pollutants. Netherlands. https://doi.org/10.1016/J.JHAZMAT.2011.11.082
Guo, Jian-Feng, Ma, Bowen, Yin, Anyuan, Fan, Kangnian, and Dai, Wei-Lin. 2012. "Highly stable and efficient Ag/AgCl-TiO{sub 2} photocatalyst: Preparation, characterization, and application in the treatment of aqueous hazardous pollutants." Netherlands. https://doi.org/10.1016/J.JHAZMAT.2011.11.082.
@misc{etde_22154057,
title = {Highly stable and efficient Ag/AgCl-TiO{sub 2} photocatalyst: Preparation, characterization, and application in the treatment of aqueous hazardous pollutants}
author = {Guo, Jian-Feng, Ma, Bowen, Yin, Anyuan, Fan, Kangnian, and Dai, Wei-Lin}
abstractNote = {Graphical abstract: A new plasmonic photocatalyst of Ag-AgCl/TiO{sub 2} was prepared by deposition-precipitation and photoreduction. This photocatalyst exhibited efficient photocatalytic activity for the degradation of 4-chlorophenol and photoreduction Cr(VI) under visible light irradiation. Highlights: Black-Right-Pointing-Pointer The preparation procedure for Ag-AgCl/TiO{sub 2} was convenient and feasible. Black-Right-Pointing-Pointer Ag-AgCl/TiO{sub 2} was very efficient under visible-light irradiation. Black-Right-Pointing-Pointer Ag-AgCl/TiO{sub 2} can photodegrade 4-chlorophenol and Cr(VI) effectively. Black-Right-Pointing-Pointer The surface plasmon resonance effect of Ag{sup 0} nanoparticles played a key role. - Abstract: A new plasmonic photocatalyst of Ag-AgCl-TiO{sub 2} was prepared by deposition-precipitation and photoreduction. This photocatalyst exhibited efficient photocatalytic activity for the degradation of 4-chlorophenol and photoreduction of Cr(VI) ion under visible light irradiation. Its high photocatalytic activity can be attributed to the surface plasmon resonance effect of Ag nanoparticles, which were highly dispersed on the surface of Ag-AgCl-TiO{sub 2}. N{sub 2} adsorption and desorption isotherm spectra, X-ray diffraction, X-ray photoelectron spectroscopy, and transmission electron microscopy were used to determine the correlation between the micro-structure and the catalytic properties of the as-prepared photocatalysts.}
doi = {10.1016/J.JHAZMAT.2011.11.082}
journal = []
volume = {211-212}
journal type = {AC}
place = {Netherlands}
year = {2012}
month = {Apr}
}