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Identifying the mechanisms of p-to-n conversion in unipolar graphene field-effect transistors

Abstract

The mechanisms of p-to-n conversion and vice versa in unipolar graphene field-effect transistors (GFETs) were systematically studied using Raman spectroscopy. Unipolar p-type GFETs are achieved by decorating the graphene surface with a thin layer of titanium (Ti) film, resulting in a Raman D peak. The D peak is observed to recover by annealing the GFET in nitrogen ambient followed by silicon nitride (Si{sub 3}N{sub 4}) deposition, suggesting that the Ti adatoms are being partially removed. Furthermore, unipolar n-type GFETs are obtained after the passivation on p-type GFETs. The threshold voltage of the n-type GFET is dependent on the thickness of the Si{sub 3}N{sub 4} layer, which increases as the thickness decreases. A comparison between the Si{sub 3}N{sub 4} and SiO{sub 2} passivation layers shows that SiO{sub 2} passivation does not convert the GFET into n-type graphene, which identifies the significance of ammonia (NH{sub 3}) for the formation of the n-type GFETs. This study provides an insight into the mechanism of controlling the conduction behavior of unipolar GFETs. (paper)
Authors:
Yap, Ray Chin Chong; Li, Hong; Chow, Wai Leong; Lu, Cong Xiang; Tay, Beng Kang; Teo, Edwin Hang Tong, E-mail: ebktay@ntu.edu.sg [1] 
  1. School of Electrical and Electronic Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798 (Singapore)
Publication Date:
May 17, 2013
Product Type:
Journal Article
Resource Relation:
Journal Name: Nanotechnology (Print); Journal Volume: 24; Journal Issue: 19; Other Information: Country of input: International Atomic Energy Agency (IAEA)
Subject:
36 MATERIALS SCIENCE; 77 NANOSCIENCE AND NANOTECHNOLOGY; AMMONIA; COMPARATIVE EVALUATIONS; CONVERSION; DEPOSITION; ELECTRIC POTENTIAL; FIELD EFFECT TRANSISTORS; GRAPHENE; LAYERS; PASSIVATION; PEAKS; RAMAN SPECTROSCOPY; SILICA; SILICON NITRIDES; SILICON OXIDES; SURFACES; THICKNESS; THIN FILMS; TITANIUM
OSTI ID:
22114738
Country of Origin:
United Kingdom
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0957-4484; TRN: GB13P1897071389
Availability:
Available from http://dx.doi.org/10.1088/0957-4484/24/19/195202
Submitting Site:
INIS
Size:
[7 page(s)]
Announcement Date:
Jul 29, 2013

Citation Formats

Yap, Ray Chin Chong, Li, Hong, Chow, Wai Leong, Lu, Cong Xiang, Tay, Beng Kang, and Teo, Edwin Hang Tong, E-mail: ebktay@ntu.edu.sg. Identifying the mechanisms of p-to-n conversion in unipolar graphene field-effect transistors. United Kingdom: N. p., 2013. Web. doi:10.1088/0957-4484/24/19/195202.
Yap, Ray Chin Chong, Li, Hong, Chow, Wai Leong, Lu, Cong Xiang, Tay, Beng Kang, & Teo, Edwin Hang Tong, E-mail: ebktay@ntu.edu.sg. Identifying the mechanisms of p-to-n conversion in unipolar graphene field-effect transistors. United Kingdom. https://doi.org/10.1088/0957-4484/24/19/195202
Yap, Ray Chin Chong, Li, Hong, Chow, Wai Leong, Lu, Cong Xiang, Tay, Beng Kang, and Teo, Edwin Hang Tong, E-mail: ebktay@ntu.edu.sg. 2013. "Identifying the mechanisms of p-to-n conversion in unipolar graphene field-effect transistors." United Kingdom. https://doi.org/10.1088/0957-4484/24/19/195202.
@misc{etde_22114738,
title = {Identifying the mechanisms of p-to-n conversion in unipolar graphene field-effect transistors}
author = {Yap, Ray Chin Chong, Li, Hong, Chow, Wai Leong, Lu, Cong Xiang, Tay, Beng Kang, and Teo, Edwin Hang Tong, E-mail: ebktay@ntu.edu.sg}
abstractNote = {The mechanisms of p-to-n conversion and vice versa in unipolar graphene field-effect transistors (GFETs) were systematically studied using Raman spectroscopy. Unipolar p-type GFETs are achieved by decorating the graphene surface with a thin layer of titanium (Ti) film, resulting in a Raman D peak. The D peak is observed to recover by annealing the GFET in nitrogen ambient followed by silicon nitride (Si{sub 3}N{sub 4}) deposition, suggesting that the Ti adatoms are being partially removed. Furthermore, unipolar n-type GFETs are obtained after the passivation on p-type GFETs. The threshold voltage of the n-type GFET is dependent on the thickness of the Si{sub 3}N{sub 4} layer, which increases as the thickness decreases. A comparison between the Si{sub 3}N{sub 4} and SiO{sub 2} passivation layers shows that SiO{sub 2} passivation does not convert the GFET into n-type graphene, which identifies the significance of ammonia (NH{sub 3}) for the formation of the n-type GFETs. This study provides an insight into the mechanism of controlling the conduction behavior of unipolar GFETs. (paper)}
doi = {10.1088/0957-4484/24/19/195202}
journal = []
issue = {19}
volume = {24}
journal type = {AC}
place = {United Kingdom}
year = {2013}
month = {May}
}