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COOH-functionalisation of silica particles

Abstract

In this study COOH-functionalised silica is synthesised using phosphonateN-(phosphonomethyl)iminodiacetic acid (PMIDA) in an aqueous solution. The presence of PMIDA on the silica particles was verified using Fourier Transform Infrared Spectroscopy, X-ray Photoelectron Spectroscopy and titration. Experimentally, surface concentrations of COOH functional groups of up to about 3 mmol/g{sub silica} were achieved, whereas theoretical calculation of the maximum COOH functional group concentration gave about 1 mmol/g{sub silica}. The discrepancy may be caused by PMIDA multilayer formation on the particle.
Authors:
Majewski, Peter; [1]  Albrecht, Trent; [2]  Weber, Siegfried [3] 
  1. School of Advanced Manufacturing and Mechanical Engineering, Mawson Institute, University of South Australia, Adelaide (Australia)
  2. Ian Wark Research Institute, University of South Australia, Adelaide (Australia)
  3. Department of Biotechnology, University of Applied Sciences, Mannheim (Germany)
Publication Date:
Sep 01, 2011
Product Type:
Journal Article
Resource Relation:
Journal Name: Applied Surface Science; Journal Volume: 257; Journal Issue: 22; Other Information: Copyright (c) 2011 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; AQUEOUS SOLUTIONS; CARBON MONOXIDE; FOURIER TRANSFORM SPECTROMETERS; LAYERS; SILICA; SURFACES; SYNTHESIS; X-RAY PHOTOELECTRON SPECTROSCOPY
OSTI ID:
22070467
Country of Origin:
Netherlands
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0169-4332; CODEN: ASUSEE; Other: PII: S0169-4332(11)00696-9; TRN: NL12R0325030202
Availability:
Available from http://dx.doi.org/10.1016/j.apsusc.2011.04.145
Submitting Site:
NLN
Size:
page(s) 9282-9286
Announcement Date:
Mar 14, 2013

Citation Formats

Majewski, Peter, Albrecht, Trent, and Weber, Siegfried. COOH-functionalisation of silica particles. Netherlands: N. p., 2011. Web. doi:10.1016/J.APSUSC.2011.04.145.
Majewski, Peter, Albrecht, Trent, & Weber, Siegfried. COOH-functionalisation of silica particles. Netherlands. https://doi.org/10.1016/J.APSUSC.2011.04.145
Majewski, Peter, Albrecht, Trent, and Weber, Siegfried. 2011. "COOH-functionalisation of silica particles." Netherlands. https://doi.org/10.1016/J.APSUSC.2011.04.145.
@misc{etde_22070467,
title = {COOH-functionalisation of silica particles}
author = {Majewski, Peter, Albrecht, Trent, and Weber, Siegfried}
abstractNote = {In this study COOH-functionalised silica is synthesised using phosphonateN-(phosphonomethyl)iminodiacetic acid (PMIDA) in an aqueous solution. The presence of PMIDA on the silica particles was verified using Fourier Transform Infrared Spectroscopy, X-ray Photoelectron Spectroscopy and titration. Experimentally, surface concentrations of COOH functional groups of up to about 3 mmol/g{sub silica} were achieved, whereas theoretical calculation of the maximum COOH functional group concentration gave about 1 mmol/g{sub silica}. The discrepancy may be caused by PMIDA multilayer formation on the particle.}
doi = {10.1016/J.APSUSC.2011.04.145}
journal = []
issue = {22}
volume = {257}
journal type = {AC}
place = {Netherlands}
year = {2011}
month = {Sep}
}