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A cheap asymmetric supercapacitor with high energy at high power: Activated carbon//K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O

Abstract

Studies of the electrochemical behavior of K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O in K{sub 2}SO{sub 4} show the reversible intercalation/deintercalation of K{sup +}-ions in the lattice. An asymmetric supercapacitor activated carbon (AC)/0.5 mol l{sup -1} K{sub 2}SO{sub 4}/K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O was assembled and tested successfully. It shows an energy density of 25.3 Wh kg{sup -1} at a power density of 140 W kg{sup -1}; at the same time it keeps a very good rate behavior with an energy density of 17.6 Wh kg{sup -1} at a power density of 2 kW kg{sup -1} based on the total mass of the active electrode materials, which is higher than that of AC/0.5 mol l{sup -1} Li{sub 2}SO{sub 4}/LiMn{sub 2}O{sub 4}. In addition, this asymmetric supercapacitor shows excellent cycling behavior without the need to remove oxygen from the electrolyte solution. This can be ascribed in part to the stability of the lamellar structure of K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O. This asymmetric aqueous capacitor has great promise for practical applications due to high energy density at high power density. (author)
Authors:
Qu, Qunting; Li, Lei; Tian, Shu; Guo, Wenling; Wu, Yuping; [1]  Holze, Rudolf [2] 
  1. New Energy and Materials Laboratory (NEML), Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, Shanghai 200433 (China)
  2. Technische Universitaet Chemnitz, Institut fuer Chemie, D-09107 Chemnitz (Germany)
Publication Date:
May 01, 2010
Product Type:
Journal Article
Resource Relation:
Journal Name: Journal of Power Sources; Journal Volume: 195; Journal Issue: 9; Other Information: Elsevier Ltd. All rights reserved
Subject:
25 ENERGY STORAGE; ACTIVATED CARBON; ENERGY DENSITY; POWER DENSITY; ELECTRODES; ELECTROLYTES; STABILITY; CAPACITORS; ELECTROCHEMISTRY; LITHIUM SULFATES; LITHIUM OXIDES; MANGANESE OXIDES; Supercapacitor; K{sub 0.27}MnO{sub 2}; K{sup +}; Electrochemical behavior; Aqueous electrolyte
OSTI ID:
21253027
Country of Origin:
Netherlands
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0378-7753; JPSODZ; TRN: NL10V3218
Availability:
Available from: http://dx.doi.org/10.1016/j.jpowsour.2009.10.108
Submitting Site:
ECN
Size:
page(s) 2789-2794
Announcement Date:
Jan 25, 2010

Citation Formats

Qu, Qunting, Li, Lei, Tian, Shu, Guo, Wenling, Wu, Yuping, and Holze, Rudolf. A cheap asymmetric supercapacitor with high energy at high power: Activated carbon//K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O. Netherlands: N. p., 2010. Web. doi:10.1016/J.JPOWSOUR.2009.10.108.
Qu, Qunting, Li, Lei, Tian, Shu, Guo, Wenling, Wu, Yuping, & Holze, Rudolf. A cheap asymmetric supercapacitor with high energy at high power: Activated carbon//K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O. Netherlands. https://doi.org/10.1016/J.JPOWSOUR.2009.10.108
Qu, Qunting, Li, Lei, Tian, Shu, Guo, Wenling, Wu, Yuping, and Holze, Rudolf. 2010. "A cheap asymmetric supercapacitor with high energy at high power: Activated carbon//K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O." Netherlands. https://doi.org/10.1016/J.JPOWSOUR.2009.10.108.
@misc{etde_21253027,
title = {A cheap asymmetric supercapacitor with high energy at high power: Activated carbon//K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O}
author = {Qu, Qunting, Li, Lei, Tian, Shu, Guo, Wenling, Wu, Yuping, and Holze, Rudolf}
abstractNote = {Studies of the electrochemical behavior of K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O in K{sub 2}SO{sub 4} show the reversible intercalation/deintercalation of K{sup +}-ions in the lattice. An asymmetric supercapacitor activated carbon (AC)/0.5 mol l{sup -1} K{sub 2}SO{sub 4}/K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O was assembled and tested successfully. It shows an energy density of 25.3 Wh kg{sup -1} at a power density of 140 W kg{sup -1}; at the same time it keeps a very good rate behavior with an energy density of 17.6 Wh kg{sup -1} at a power density of 2 kW kg{sup -1} based on the total mass of the active electrode materials, which is higher than that of AC/0.5 mol l{sup -1} Li{sub 2}SO{sub 4}/LiMn{sub 2}O{sub 4}. In addition, this asymmetric supercapacitor shows excellent cycling behavior without the need to remove oxygen from the electrolyte solution. This can be ascribed in part to the stability of the lamellar structure of K{sub 0.27}MnO{sub 2}.0.6H{sub 2}O. This asymmetric aqueous capacitor has great promise for practical applications due to high energy density at high power density. (author)}
doi = {10.1016/J.JPOWSOUR.2009.10.108}
journal = []
issue = {9}
volume = {195}
place = {Netherlands}
year = {2010}
month = {May}
}