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Decrease of the Curie temperature in La{sub 0.67}Sr{sub 0.33}MnO{sub 3} thin films induced by Au capping

Abstract

Ferromagnetism of La{sub 0.67}Sr{sub 0.33}MnO{sub 3} is extremely sensitive to external perturbations like substrate-induced strain, charge injection and chemical interactions with neighbour layers. In this paper we discuss the perturbation induced by the presence of a metallic overlayer, typically deposited for electric contacts, in the prototypical case of the Au/La{sub 0.67}Sr{sub 0.33}MnO{sub 3} interface. In particular we found a sizable decrease of the Curie temperature in thin films of La{sub 0.67}Sr{sub 0.33}MnO{sub 3} after gold capping: 65 K for 5 nm thickness of the manganite. Apart from chemical reactions at the interface, charge injection-depletion induced by the difference in the work function between Au and La{sub 0.67}Sr{sub 0.33}MnO{sub 3} could partially explain this phenomenon.
Authors:
Brivio, S; Cantoni, M; Petti, D; Cattoni, A; [1]  Bertacco, R. , E-mail: riccardo.bertacco@polimi.it; [1]  Finazzi, M; Ciccacci, F; [1]  Sidorenko, A; Allodi, G; Ghidini, M; De Renzi, R [2] 
  1. L-NESS, Dipartimento di Fisica del Politecnico di Milano, via Anzani 42, 22100 Como (Italy)
  2. Dipartimento di Fisica Universita di Parma, Parco Area delle Scienze 7/A, 43100 Parma (Italy)
Publication Date:
Nov 25, 2007
Product Type:
Journal Article
Resource Relation:
Journal Name: Materials Science and Engineering. B, Solid-State Materials for Advanced Technology; Journal Volume: 144; Journal Issue: 1-3; Conference: EMRS 2007 - Symposium H: Nanoscale tailoring of defect structures for optimized functional and multifunctional oxide films, Strasbourg (France), 28 May - 1 Jun 2007; Other Information: DOI: 10.1016/j.mseb.2007.07.084; PII: S0921-5107(07)00318-2; Copyright (c) 2007 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved; Country of input: International Atomic Energy Agency (IAEA)
Subject:
36 MATERIALS SCIENCE; CHEMICAL REACTIONS; CURIE POINT; ELECTRIC CONTACTS; ENERGY BEAM DEPOSITION; FERROMAGNETISM; GOLD; INJECTION; INTERFACES; LANTHANUM COMPOUNDS; LASER RADIATION; LAYERS; MANGANATES; PERTURBATION THEORY; PULSED IRRADIATION; STRAINS; STRONTIUM COMPOUNDS; THICKNESS; THIN FILMS; WORK FUNCTIONS
OSTI ID:
21090255
Country of Origin:
Netherlands
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0921-5107; MSBTEK; TRN: NL08R3636100465
Availability:
Available from http://dx.doi.org/10.1016/j.mseb.2007.07.084;INIS
Submitting Site:
NLN
Size:
page(s) 93-96
Announcement Date:
Nov 13, 2008

Citation Formats

Brivio, S, Cantoni, M, Petti, D, Cattoni, A, Bertacco, R. , E-mail: riccardo.bertacco@polimi.it, Finazzi, M, Ciccacci, F, Sidorenko, A, Allodi, G, Ghidini, M, and De Renzi, R. Decrease of the Curie temperature in La{sub 0.67}Sr{sub 0.33}MnO{sub 3} thin films induced by Au capping. Netherlands: N. p., 2007. Web. doi:10.1016/j.mseb.2007.07.084.
Brivio, S, Cantoni, M, Petti, D, Cattoni, A, Bertacco, R. , E-mail: riccardo.bertacco@polimi.it, Finazzi, M, Ciccacci, F, Sidorenko, A, Allodi, G, Ghidini, M, & De Renzi, R. Decrease of the Curie temperature in La{sub 0.67}Sr{sub 0.33}MnO{sub 3} thin films induced by Au capping. Netherlands. https://doi.org/10.1016/j.mseb.2007.07.084
Brivio, S, Cantoni, M, Petti, D, Cattoni, A, Bertacco, R. , E-mail: riccardo.bertacco@polimi.it, Finazzi, M, Ciccacci, F, Sidorenko, A, Allodi, G, Ghidini, M, and De Renzi, R. 2007. "Decrease of the Curie temperature in La{sub 0.67}Sr{sub 0.33}MnO{sub 3} thin films induced by Au capping." Netherlands. https://doi.org/10.1016/j.mseb.2007.07.084.
@misc{etde_21090255,
title = {Decrease of the Curie temperature in La{sub 0.67}Sr{sub 0.33}MnO{sub 3} thin films induced by Au capping}
author = {Brivio, S, Cantoni, M, Petti, D, Cattoni, A, Bertacco, R. , E-mail: riccardo.bertacco@polimi.it, Finazzi, M, Ciccacci, F, Sidorenko, A, Allodi, G, Ghidini, M, and De Renzi, R}
abstractNote = {Ferromagnetism of La{sub 0.67}Sr{sub 0.33}MnO{sub 3} is extremely sensitive to external perturbations like substrate-induced strain, charge injection and chemical interactions with neighbour layers. In this paper we discuss the perturbation induced by the presence of a metallic overlayer, typically deposited for electric contacts, in the prototypical case of the Au/La{sub 0.67}Sr{sub 0.33}MnO{sub 3} interface. In particular we found a sizable decrease of the Curie temperature in thin films of La{sub 0.67}Sr{sub 0.33}MnO{sub 3} after gold capping: 65 K for 5 nm thickness of the manganite. Apart from chemical reactions at the interface, charge injection-depletion induced by the difference in the work function between Au and La{sub 0.67}Sr{sub 0.33}MnO{sub 3} could partially explain this phenomenon.}
doi = {10.1016/j.mseb.2007.07.084}
journal = []
issue = {1-3}
volume = {144}
place = {Netherlands}
year = {2007}
month = {Nov}
}