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The decomposition behavior of as-received and oxidized TiH{sub 2} foaming-agent powder

Abstract

The decomposition behavior of as-received and oxidized TiH{sub 2} powder has been studied using differential scanning calorimetry and X-ray diffraction. It was found that the decomposition of TiH{sub 2} in argon occurs in two stages, firstly the reduction in the stoichiometry of the hydride to {delta}-TiH{sub 1.5}, and secondly, with progressive heating, decomposition of the hydride to form the {beta}- and {alpha}-phases. When heating in air, at low temperatures, oxidation of the hydride to form an oxyhydride occurs and with progressive heating, the oxidation products Ti{sub 3}O and TiO{sub 2} are formed in increasing quantities. Heat treatment, to reduce the stoichiometry of the hydride and form an oxide layer, does delay the evolution of gas when re-heated in argon. A balance between the delay in gas evolution and detrimental gas loss is best achieved for pre-heat treating to between 530 and 630 deg. C.
Publication Date:
Sep 25, 2003
Product Type:
Journal Article
Resource Relation:
Journal Name: Materials Science and Engineering. A, Structural Materials: Properties, Microstructure and Processing; Journal Volume: 357; Journal Issue: 1-2; Other Information: DOI: 10.1016/S0921-5093(03)00211-9; PII: S0921509303002119; Copyright (c) 2003 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved; Country of input: International Atomic Energy Agency (IAEA)
Subject:
36 MATERIALS SCIENCE; AIR; ARGON; CALORIMETRY; DECOMPOSITION; FOAMS; HEAT; HEAT TREATMENTS; HEATING; LAYERS; OXIDATION; POWDERS; REDUCTION; STOICHIOMETRY; TITANIUM HYDRIDES; TITANIUM OXIDES; X-RAY DIFFRACTION
OSTI ID:
20907820
Country of Origin:
Netherlands
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0921-5093; MSAPE3; TRN: NL05S7562070113
Submitting Site:
NLN
Size:
page(s) 258-263
Announcement Date:
Sep 20, 2007

Citation Formats

Kennedy, A R, and Lopez, V H. The decomposition behavior of as-received and oxidized TiH{sub 2} foaming-agent powder. Netherlands: N. p., 2003. Web. doi:10.1016/S0921-5093(03)00211-9.
Kennedy, A R, & Lopez, V H. The decomposition behavior of as-received and oxidized TiH{sub 2} foaming-agent powder. Netherlands. https://doi.org/10.1016/S0921-5093(03)00211-9
Kennedy, A R, and Lopez, V H. 2003. "The decomposition behavior of as-received and oxidized TiH{sub 2} foaming-agent powder." Netherlands. https://doi.org/10.1016/S0921-5093(03)00211-9.
@misc{etde_20907820,
title = {The decomposition behavior of as-received and oxidized TiH{sub 2} foaming-agent powder}
author = {Kennedy, A R, and Lopez, V H}
abstractNote = {The decomposition behavior of as-received and oxidized TiH{sub 2} powder has been studied using differential scanning calorimetry and X-ray diffraction. It was found that the decomposition of TiH{sub 2} in argon occurs in two stages, firstly the reduction in the stoichiometry of the hydride to {delta}-TiH{sub 1.5}, and secondly, with progressive heating, decomposition of the hydride to form the {beta}- and {alpha}-phases. When heating in air, at low temperatures, oxidation of the hydride to form an oxyhydride occurs and with progressive heating, the oxidation products Ti{sub 3}O and TiO{sub 2} are formed in increasing quantities. Heat treatment, to reduce the stoichiometry of the hydride and form an oxide layer, does delay the evolution of gas when re-heated in argon. A balance between the delay in gas evolution and detrimental gas loss is best achieved for pre-heat treating to between 530 and 630 deg. C.}
doi = {10.1016/S0921-5093(03)00211-9}
journal = []
issue = {1-2}
volume = {357}
place = {Netherlands}
year = {2003}
month = {Sep}
}