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Isolation of lanthanide and hafnium radioisotopes from a massive Ta-target

Abstract

Production of radioactive isotopes of rare Earth elements (REE) is relevant for their application in systematic chemical, environmental and nuclear medical investigations. In particular, among the lanthanides the number of isotopes with different nuclear characteristics is very high, while their chemical properties are quite similar. As a source of radiolanthanides, in this experiment a massive 195 g tantalum target was used, which has been irradiated with 1 GeV protons at CERN accelerator in 2002, totally receiving about 10{sup 19} protons. A rough estimate of the overall REE mass in the target yielded 100 {mu}g. Due to significant radiation dose (200 {mu}Sv at 100 cm distance), excess of the chemical matrix (Ta) and the complex radioelement distribution in the target, a sophisticated radiochemical separation procedure was developed. (orig.)
Authors:
Korolev, N A; Novgorodov, A F; Filosofov, D V; Lebedev, N A; [1]  Zhernosekov, K; Korobeinikov, A; Roesch, F; [2]  Beyer, G J [3] 
  1. Joint Institute for Nuclear Research, DLNP, Dubna (Russian Federation)
  2. Mainz Univ. (Germany). Inst. fuer Kernchemie
  3. CERN, ISOLDE, Geneva (Switzerland)
Publication Date:
Jul 01, 2004
Product Type:
Conference
Report Number:
INIS-DE-0228
Reference Number:
TRN: DE07F8775
Resource Relation:
Conference: NRC 6: 6. international conference on nuclear and radiochemistry, Aachen (Germany), 29 Aug - 3 Sep 2004; Other Information: PBD: 2004; Related Information: In: Advances in nuclear and radiochemistry. Extended abstracts, Schriften des Forschungszentrums Juelich. Reihe Allgemeines und Interdisziplinaeresv. 3, by Qaim, S.M.; Coenen, H.H. (eds.), 831 pages.
Subject:
38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY; 73 NUCLEAR PHYSICS AND RADIATION PHYSICS; RARE EARTHS; HAFNIUM ISOTOPES; TANTALUM 181 TARGET; SEPARATION PROCESSES; NUCLEAR REACTION YIELD; PROTON REACTIONS
OSTI ID:
20896355
Research Organizations:
Forschungszentrum Juelich GmbH (Germany). Inst. fuer Nuklearchemie
Country of Origin:
Germany
Language:
English
Other Identifying Numbers:
Other: ISBN 3-89336-362-9; ISSN 1433-5565; TRN: DE07F8775
Availability:
Commercial reproduction prohibited; INIS; OSTI as DE20896238; www.osti.gov/servlets/purl/20896238-kbAkpi/
Submitting Site:
DEN
Size:
page(s) 321-322
Announcement Date:
Jan 08, 2009

Citation Formats

Korolev, N A, Novgorodov, A F, Filosofov, D V, Lebedev, N A, Zhernosekov, K, Korobeinikov, A, Roesch, F, and Beyer, G J. Isolation of lanthanide and hafnium radioisotopes from a massive Ta-target. Germany: N. p., 2004. Web.
Korolev, N A, Novgorodov, A F, Filosofov, D V, Lebedev, N A, Zhernosekov, K, Korobeinikov, A, Roesch, F, & Beyer, G J. Isolation of lanthanide and hafnium radioisotopes from a massive Ta-target. Germany.
Korolev, N A, Novgorodov, A F, Filosofov, D V, Lebedev, N A, Zhernosekov, K, Korobeinikov, A, Roesch, F, and Beyer, G J. 2004. "Isolation of lanthanide and hafnium radioisotopes from a massive Ta-target." Germany.
@misc{etde_20896355,
title = {Isolation of lanthanide and hafnium radioisotopes from a massive Ta-target}
author = {Korolev, N A, Novgorodov, A F, Filosofov, D V, Lebedev, N A, Zhernosekov, K, Korobeinikov, A, Roesch, F, and Beyer, G J}
abstractNote = {Production of radioactive isotopes of rare Earth elements (REE) is relevant for their application in systematic chemical, environmental and nuclear medical investigations. In particular, among the lanthanides the number of isotopes with different nuclear characteristics is very high, while their chemical properties are quite similar. As a source of radiolanthanides, in this experiment a massive 195 g tantalum target was used, which has been irradiated with 1 GeV protons at CERN accelerator in 2002, totally receiving about 10{sup 19} protons. A rough estimate of the overall REE mass in the target yielded 100 {mu}g. Due to significant radiation dose (200 {mu}Sv at 100 cm distance), excess of the chemical matrix (Ta) and the complex radioelement distribution in the target, a sophisticated radiochemical separation procedure was developed. (orig.)}
place = {Germany}
year = {2004}
month = {Jul}
}