You need JavaScript to view this

High resolution and high precision absorption spectroscopy using high finesse cavities: application to the study of molecules with atmospheric interest; Cavites de haute finesse pour la spectroscopie d'absorption haute sensibilite et haute precision: application a l'etude de molecules d'interet atmospherique

Abstract

High finesse cavities are used to measure very weak absorption features. Two different methodologies are investigated and applied to the study of molecules with atmospheric interest. First, Continuous Wave - Cavity Ring Down Spectroscopy (CW-CRDS) is used to study the atmospheric spectra of water vapour in the near infrared range. These measurements are performed for temperature and pressure of atmospheric relevance for DIAL applications (Differential Absorption Lidar). This study, financed by the European Space Agency (ESA), goes with the WALES mission (Water Vapour Lidar Experiment in Space). The experimental setup was conceived in order to control pressure, temperature and relative humidity conditions. A particular attention is done to characterize and describe the spectrometer. Then, measurements of red Oxygen B band are performed to demonstrate the huge performance of Optical Feedback Cavity Enhanced Absorption Spectroscopy (OF-CEAS). The desired optical feedback is obtained by light injection into the high finesse cavity through a glass plate placed inside the cavity and closed to the Brewster angle. We show a measurement dynamical range of 5 orders of magnitude (10{sup -5} to 10{sup -10} /cm) and a sensitivity of 10{sup -10} /cm/{radical} Hz. Also, sampling absorption spectra by the super linear cavity frequency comb allows  More>>
Authors:
Publication Date:
Dec 15, 2005
Product Type:
Thesis/Dissertation
Report Number:
FRNC-TH-6565
Resource Relation:
Other Information: TH: These physique; 133 refs.; Also available from Universite Lyon 1.Bibliotheque universitaire Sciences, 43, boulevard du 11 Novembre 1918 BP 2215 Batiment 901, 69603 - Villeurbanne Cedex (France)
Subject:
47 OTHER INSTRUMENTATION; 54 ENVIRONMENTAL SCIENCES; CAVITY RESONATORS; ABSORPTION SPECTROSCOPY; LASER SPECTROSCOPY; WATER VAPOR; INFRARED SPECTRA; CROSS SECTIONS; CALIBRATION; SENSITIVITY; FABRY-PEROT INTERFEROMETER; TRANSFER FUNCTIONS; OPTICAL RADAR; OXYGEN
OSTI ID:
20823630
Research Organizations:
Universite Claude Bernard Lyon-1, 69 - Villeurbanne (France)
Country of Origin:
France
Language:
French
Other Identifying Numbers:
TRN: FR0604412
Availability:
Commercial reproduction prohibited; OSTI as DE20823630
Submitting Site:
FR
Size:
234 pages
Announcement Date:
Jan 04, 2007

Citation Formats

Motto-Ros, V. High resolution and high precision absorption spectroscopy using high finesse cavities: application to the study of molecules with atmospheric interest; Cavites de haute finesse pour la spectroscopie d'absorption haute sensibilite et haute precision: application a l'etude de molecules d'interet atmospherique. France: N. p., 2005. Web.
Motto-Ros, V. High resolution and high precision absorption spectroscopy using high finesse cavities: application to the study of molecules with atmospheric interest; Cavites de haute finesse pour la spectroscopie d'absorption haute sensibilite et haute precision: application a l'etude de molecules d'interet atmospherique. France.
Motto-Ros, V. 2005. "High resolution and high precision absorption spectroscopy using high finesse cavities: application to the study of molecules with atmospheric interest; Cavites de haute finesse pour la spectroscopie d'absorption haute sensibilite et haute precision: application a l'etude de molecules d'interet atmospherique." France.
@misc{etde_20823630,
title = {High resolution and high precision absorption spectroscopy using high finesse cavities: application to the study of molecules with atmospheric interest; Cavites de haute finesse pour la spectroscopie d'absorption haute sensibilite et haute precision: application a l'etude de molecules d'interet atmospherique}
author = {Motto-Ros, V}
abstractNote = {High finesse cavities are used to measure very weak absorption features. Two different methodologies are investigated and applied to the study of molecules with atmospheric interest. First, Continuous Wave - Cavity Ring Down Spectroscopy (CW-CRDS) is used to study the atmospheric spectra of water vapour in the near infrared range. These measurements are performed for temperature and pressure of atmospheric relevance for DIAL applications (Differential Absorption Lidar). This study, financed by the European Space Agency (ESA), goes with the WALES mission (Water Vapour Lidar Experiment in Space). The experimental setup was conceived in order to control pressure, temperature and relative humidity conditions. A particular attention is done to characterize and describe the spectrometer. Then, measurements of red Oxygen B band are performed to demonstrate the huge performance of Optical Feedback Cavity Enhanced Absorption Spectroscopy (OF-CEAS). The desired optical feedback is obtained by light injection into the high finesse cavity through a glass plate placed inside the cavity and closed to the Brewster angle. We show a measurement dynamical range of 5 orders of magnitude (10{sup -5} to 10{sup -10} /cm) and a sensitivity of 10{sup -10} /cm/{radical} Hz. Also, sampling absorption spectra by the super linear cavity frequency comb allows very precise frequency measurements. This is demonstrated by the determination of Oxygen pressure shifts with an absolute accuracy of around 5 x 10{sup -5} cm{sup -1}/atm. To our knowledge, we provide the highest accuracy ever reported for this parameter. (author)}
place = {France}
year = {2005}
month = {Dec}
}