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Ultrafast measurement of the optical properties of shocked nickel and laser heated gold

Abstract

We have used high-resolution Frequency Domain Interferometry (FDI) to make the first ultrafast measurement of shock-induced changes in the optical properties of thin nickel ({approx}500 nm) targets. Data taken at several angles of incidence allowed the separation of optical effects from material motion, yielding an effective complex index for the shocked material. In contrast to our previous studies of aluminum, measurements with an 800 nm probe wavelength found a phase shift attributable to optical property changes with the same sign as that due to surface motion, during an 11.5 GPa shock breakout. A similar experiment was attempted with thin gold films ({approx}180 nm) using Ultrafast Spatial Interferometry (USI). However, since the electron-phonon coupling in gold is extremely weak, a shock is observed as it forms'. Ballistic electrons and electron-electron equilibrium cause fast heating of the electrons in the entire thickness of the thin film, followed by lattice excitation through electron-phonon coupling, eventually leading to melt and frustrated thermal expansion yielding the observed surface motion. We suggest that these experiments offer a new path for observation of phase changes or for temperature measurements, by allowing a determination of the complex index under dynamic loading conditions and comparing the measured values to  More>>
Authors:
Funk, David J; Moore, D S; Reho, J H; Gahagan, K T; McGrane, S D; Rabie, R L [1] 
  1. Dynamic Experimentation Division, Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)
Publication Date:
Jul 08, 2002
Product Type:
Journal Article
Resource Relation:
Journal Name: AIP Conference Proceedings; Journal Volume: 620; Journal Issue: 1; Conference: 12. APS topical conference on shock compression of condensed matter, Atlanta, GA (United States), 24-29 Jun 2001; Other Information: DOI: 10.1063/1.1483760; (c) 2002 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA); PBD: 8 Jul 2002
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; ALUMINIUM; DYNAMIC LOADS; ELECTRON-PHONON COUPLING; ELECTRONS; EXCITATION; GOLD; INTERFEROMETRY; NICKEL; OPTICAL PROPERTIES; PHASE SHIFT; PRESSURE RANGE GIGA PA; SHOCK WAVES; SURFACES; TEMPERATURE MEASUREMENT; THERMAL EXPANSION; THIN FILMS
OSTI ID:
20620945
Country of Origin:
United States
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0094-243X; APCPCS; TRN: US03C4090064595
Submitting Site:
INIS
Size:
page(s) 1227-1230
Announcement Date:
Aug 28, 2005

Citation Formats

Funk, David J, Moore, D S, Reho, J H, Gahagan, K T, McGrane, S D, and Rabie, R L. Ultrafast measurement of the optical properties of shocked nickel and laser heated gold. United States: N. p., 2002. Web. doi:10.1063/1.1483760.
Funk, David J, Moore, D S, Reho, J H, Gahagan, K T, McGrane, S D, & Rabie, R L. Ultrafast measurement of the optical properties of shocked nickel and laser heated gold. United States. https://doi.org/10.1063/1.1483760
Funk, David J, Moore, D S, Reho, J H, Gahagan, K T, McGrane, S D, and Rabie, R L. 2002. "Ultrafast measurement of the optical properties of shocked nickel and laser heated gold." United States. https://doi.org/10.1063/1.1483760.
@misc{etde_20620945,
title = {Ultrafast measurement of the optical properties of shocked nickel and laser heated gold}
author = {Funk, David J, Moore, D S, Reho, J H, Gahagan, K T, McGrane, S D, and Rabie, R L}
abstractNote = {We have used high-resolution Frequency Domain Interferometry (FDI) to make the first ultrafast measurement of shock-induced changes in the optical properties of thin nickel ({approx}500 nm) targets. Data taken at several angles of incidence allowed the separation of optical effects from material motion, yielding an effective complex index for the shocked material. In contrast to our previous studies of aluminum, measurements with an 800 nm probe wavelength found a phase shift attributable to optical property changes with the same sign as that due to surface motion, during an 11.5 GPa shock breakout. A similar experiment was attempted with thin gold films ({approx}180 nm) using Ultrafast Spatial Interferometry (USI). However, since the electron-phonon coupling in gold is extremely weak, a shock is observed as it forms'. Ballistic electrons and electron-electron equilibrium cause fast heating of the electrons in the entire thickness of the thin film, followed by lattice excitation through electron-phonon coupling, eventually leading to melt and frustrated thermal expansion yielding the observed surface motion. We suggest that these experiments offer a new path for observation of phase changes or for temperature measurements, by allowing a determination of the complex index under dynamic loading conditions and comparing the measured values to those obtained under static conditions.}
doi = {10.1063/1.1483760}
journal = []
issue = {1}
volume = {620}
journal type = {AC}
place = {United States}
year = {2002}
month = {Jul}
}