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A re-evaluation of the initial yield of the hydrated electron in the picosecond time range

Abstract

The yield of the hydrated electron in the picosecond time range has been re-evaluated with an ultrafast pulse radiolysis system using a laser photocathode RF-gun in combination with a conventional one, and a value of 4.1{+-}0.2 per 100 eV of absorbed energy at 20 ps was derived. This is consistent with recent experimental results using a time correlation method [Bartels et al., J. Phys. Chem. A 104, 1686-1691 (2000)] and with Monte-Carlo calculations [Muroya et al., Can. J. Chem. 80 1367-1374 (2002)].
Authors:
Muroya, Yusa; [1]  Mingzhang, Lin; [1]  Wu, Guozhong; [1]  Iijima, Hokuto; [1]  Yoshii, Koji; [1]  Ueda, Toru; [1]  Kudo, Hisaaki; [1]  Katsumura, Yosuke [1] 
  1. Nuclear Engineering Research Laboratory, Graduate School of Engineering, University of Tokyo, 2-22 Shirakata-shirane, Tokai-mura, Naka-gun, Ibaraki 319-1188 (Japan)
Publication Date:
Feb 01, 2005
Product Type:
Journal Article
Resource Relation:
Journal Name: Radiation Physics and Chemistry (1993); Journal Volume: 72; Journal Issue: 2-3; Other Information: DOI: 10.1016/j.radphyschem.2004.09.011; PII: S0969-806X(04)00492-X; Copyright (c) 2004 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved; Country of input: International Atomic Energy Agency (IAEA); PBD: Feb 2005
Subject:
38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY; EV RANGE 10-100; EVALUATION; HYDRATION; LASERS; MONTE CARLO METHOD; PHOTOCATHODES; PULSES; RADIOLYSIS; SOLVATED ELECTRONS
OSTI ID:
20620236
Country of Origin:
United Kingdom
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0969-806X; RPCHDM; TRN: GB05R3058063886
Submitting Site:
GBN
Size:
page(s) 169-172
Announcement Date:
Aug 28, 2005

Citation Formats

Muroya, Yusa, Mingzhang, Lin, Wu, Guozhong, Iijima, Hokuto, Yoshii, Koji, Ueda, Toru, Kudo, Hisaaki, and Katsumura, Yosuke. A re-evaluation of the initial yield of the hydrated electron in the picosecond time range. United Kingdom: N. p., 2005. Web. doi:10.1016/j.radphyschem.2004.09.011.
Muroya, Yusa, Mingzhang, Lin, Wu, Guozhong, Iijima, Hokuto, Yoshii, Koji, Ueda, Toru, Kudo, Hisaaki, & Katsumura, Yosuke. A re-evaluation of the initial yield of the hydrated electron in the picosecond time range. United Kingdom. https://doi.org/10.1016/j.radphyschem.2004.09.011
Muroya, Yusa, Mingzhang, Lin, Wu, Guozhong, Iijima, Hokuto, Yoshii, Koji, Ueda, Toru, Kudo, Hisaaki, and Katsumura, Yosuke. 2005. "A re-evaluation of the initial yield of the hydrated electron in the picosecond time range." United Kingdom. https://doi.org/10.1016/j.radphyschem.2004.09.011.
@misc{etde_20620236,
title = {A re-evaluation of the initial yield of the hydrated electron in the picosecond time range}
author = {Muroya, Yusa, Mingzhang, Lin, Wu, Guozhong, Iijima, Hokuto, Yoshii, Koji, Ueda, Toru, Kudo, Hisaaki, and Katsumura, Yosuke}
abstractNote = {The yield of the hydrated electron in the picosecond time range has been re-evaluated with an ultrafast pulse radiolysis system using a laser photocathode RF-gun in combination with a conventional one, and a value of 4.1{+-}0.2 per 100 eV of absorbed energy at 20 ps was derived. This is consistent with recent experimental results using a time correlation method [Bartels et al., J. Phys. Chem. A 104, 1686-1691 (2000)] and with Monte-Carlo calculations [Muroya et al., Can. J. Chem. 80 1367-1374 (2002)].}
doi = {10.1016/j.radphyschem.2004.09.011}
journal = []
issue = {2-3}
volume = {72}
journal type = {AC}
place = {United Kingdom}
year = {2005}
month = {Feb}
}